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World Journal of Applied Physics

On the Reduction of Classical Spin in One-dimensional Heisenberg Magnets with Spin S>1/2

Farhod Rahimi

Published Feb 27, 2026• 0 citations
Publisher

Abstract

This paper develops a semiclassical framework for one-dimensional Heisenberg magnets with spin S>1/2, where classical approaches are reliable only as S→∞ and can miss quantum contributions from multipole moments. The aim is to construct a workable mathematical apparatus that connects the quantum lattice Hamiltonian to an effective classical field description while incorporating an effective reduction of the classical spin length. The analysis starts from an anisotropic Heisenberg chain with nearest-neighbour exchange and single-ion anisotropy. After outlining the continuum (long-wavelength) reduction, including factorization of slowly varying fields and replacement of commutators by Poisson brackets, the semiclassical limit is formulated using a Hartree product ansatz and generalized SU(N) coherent states for each lattice site. For spin S=1 the coherent state is built on the SU(3)/[SU(2)×U(1)] manifold. Two Euler angles define the orientation of the classical spin vector, an additional angle describes rotation of the quadrupole tensor about this vector, and a real parameter g controls the redistribution between dipolar and quadrupolar sectors. Averaging the spin operators yields explicit classical components and shows that the standard constraint |S|^2=1 is violated. Instead, an identity relates the reduced spin length to a combination of double correlators, demonstrating that quadrupolar degrees of freedom quantitatively produce a measurable renormalization of the effective classical spin. For spin S=3/2 the construction is generalized to SU(4) coherent states, where both quadrupole and octupole moments arise naturally. The averaged spin operators again violate spin-length conservation and, moreover, simple projection sum rules. The corresponding SU(4) identities involve combinations of triple correlators and introduce parameters g and k that quantify reductions due to quadrupolar and octupolar sectors, respectively; the SU(3) case is recovered when k=0. The framework provides a transparent route to include multipolar physics in semiclassical dynamics and is relevant for interpreting nonlinear collective excitations, including soliton-like modes, in quantum spin chains.

DOI
10.11648/j.wjap.20261101.12

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This paper develops a semiclassical framework for one-dimensional Heisenberg magnets with spin S>1/2, where classical approaches are reliable only as S→∞ and can miss quantum contributions from multipole moments. The aim is to construct a workable mathematical apparatus that connects the quantum lattice Hamiltonian to an effective classical field description while incorporating an effective reduction of the classical spin length. The analysis starts from an anisotropic Heisenberg chain with nearest-neighbour exchange and single-ion anisotropy. After outlining the continuum (long-wavelength) reduction, including factorization of slowly varying fields and replacement of commutators by Poisson brackets, the semiclassical limit is formulated using a Hartree product ansatz and generalized SU(N) coherent states for each lattice site. For spin S=1 the coherent state is built on the SU(3)/[SU(2)×U(1)] manifold. Two Euler angles define the orientation of the classical spin vector, an additional angle describes rotation of the quadrupole tensor about this vector, and a real parameter g controls the redistribution between dipolar and quadrupolar sectors. Averaging the spin operators yields explicit classical components and shows that the standard constraint |S|^2=1 is violated. Instead, an identity relates the reduced spin length to a combination of double correlators, demonstrating that quadrupolar degrees of freedom quantitatively produce a measurable renormalization of the effective classical spin. For spin S=3/2 the construction is generalized to SU(4) coherent states, where both quadrupole and octupole moments arise naturally. The averaged spin operators again violate spin-length conservation and, moreover, simple projection sum rules. The corresponding SU(4) identities involve combinations of triple correlators and introduce parameters g and k that quantify reductions due to quadrupolar and octupolar sectors, respectively; the SU(3) case is recovered when k=0. The framework provides a transparent route to include multipolar physics in semiclassical dynamics and is relevant for interpreting nonlinear collective excitations, including soliton-like modes, in quantum spin chains.
On the basis of the method of generalized coherent states (GCS) of the SU(2) group we formulate the reduction procedure of the quantum lattice Heisenberg XYZ model to the continuum Landau-Lifshitz model. The choice of the GCS representation is determined (i) by their proximity to the corresponding classical states and (ii) by similarity of the geometric structure of the homogeneous spaces on which the SU(2) GCS and the vector of the magnetic moment of the corresponding Landau-Lifshitz model are defined. The present reduction procedure is allowed only in the case of weak anisotropy. Accounting for a weak one-ion anisotropy leads to the Landau-Lifshitz model with a renormalized anisotropy tensor. The contribution of such an anisotropy vanishes for the s = 1/2 case.
Effective nonlinear field theory for a semiclassical long-wavelength description of one-dimensional S=1/2 Heisenberg antiferromagnets with dimerized ground states is derived within an approach using two-site coherent states. The method is applied to bond-alternating anisotropic spin chains in presence of external magnetic field and next-nearest-neighbor interactions. Linear and nonlinear excitations in singlet and magnetic phases are studied. Soliton solutions are found and their properties under semiclassical quantization are discussed. \textcopyright{} 1996 The American Physical Society.
A variational estimate of the free energy of a quantum spin chain based on the stochastic behavior of the quantization axes is proposed. It allows a description of the nonlinear excitations and quantum spin waves within the same framework. For an easy-plane ferromagnet with an external field in the plane it reveals that the nonlinear excitations (solitons) are predominantly described by the classical degrees of freedom. Considerable effort has been devoted to the theoretical description1 and experimental verification of the existence of nonlinear excitations. In this field magnetic chain systems have played an important part.2 Chain systems with an easy-plane anisotropy, such as (C6 H11 NH3 )CuBr3 (CHAB) and CsNiF3 , which are subjected to a symmetry breaking field, were found to be soliton bearing.3 Theoretically the description of the nonlinear effect is based on the mapping of the spin dynamics on a sine-Gordon model. Further research4 indicated that the interpretation of the thermodynamical properties of real systems in terms of the sine-Gordon model required however quantum and anisotropy corrections. Since the dipolar interactions between the spins in the chain are considered to be negligible, the direction of the spin chain in configuration space with respect to any preferred direction in spin space does not enter explicitly in the Hamiltonian. This makes it interesting to define a site-dependent z direction in spin space which makes an angle (Θn ,φn ) with the z direction in configuration space. The model Hamiltonian can then be written in terms of the spin operators defined with respect to the site-dependent quantization axis. The representation with equal quantization axis for all the sites is related to the representation with different quantization axes at each site by a rotation in spin space. The unitary transformation that describes the rotation contains the angles (Θn ,φn ), which we have treated as random variables. Based on this observation we have proposed a new variational approach for the quantum spin chain. We will outline the main results here. A full account is published elsewhere.5 In our approach the free energy of the system can be separated in a quantum part and a classical part. The free energy F of the chain is then approximated by an upper bound F<Fcl +Fqm , where βFcl =−ln[E(exp−βVcl )] and βFqm =−ln Tr(exp−β〈Hqm 〉). The first part is a configurational classical free energy, depending on the choice of the probability distribution for the quantization axes via the expectation E. The second contribution is the free energy of a modified quantum chain, whose parameters are classical averages and can be obtained from the configurational classical free energy. For easy-plane ferromagnetic chains, the nonlinear excitations are comprised in the classical part, whereas the quantum part contains predominantly linear excitations. For those thermodynamical quantities that are insensitive to the contribution of the quantum excitations, the chain is thermodynamically equivalent with a classical sine-Gordon system. The out-of-plane corrections are incorporated in the quantum part of the free energy. This behavior is corroborated experimentally by measurements of the excess heat capacity of CHAB for different magnetic fields with the same in-plane component.6 The validity of our approach is, however, not restricted to easy-plane ferromagnetic chains. Also for more complex systems with, for example, an orthorhombic or helical symmetry, the introduction of stochastic quantization axes can shed new light on some of the thermodynamical properties of these quantum systems in terms of their classical equivalent.
Generalized Coherent States (GCS) are constructed (and discussed) in order to study quasiclassical behaviour of quantum spin models of the Heisenberg type. Several such models are taken to their semiclassical limits, whose form depends on the spin value as well as the Hamiltonian symmetry. In the continuum approximation, SU(2)/U(1) GCS when applied give rise to the well known Landau - Lifshitz classical phenomenology. For arbitrary spin values one obtains a lattice of coupled nonlinear oscillators. Corresponding classical continuum models are described as well.