This thesis addresses challenges in the experimental realisation of optical quantum computing with atom-cavity platforms and develops techniques for experimental quantum control that generalise across a range of quantum modalities. Within the framework of cavity quantum electrodynamics (cQED), methods are developed and numerically validated for fast and precise control of single atoms to generate photonic states of interest. In particular, we consider the generation of high-repetition-rate n-photon bursts and time-bin entangled states. These photonic resources are essential for applications such as boson sampling, multi-photon interference, optical quantum computing, and quantum-enhanced metrology. Experimental improvements in coherent population transfer are demonstrated using adaptive pulse shaping with acousto-optic modulators. Beyond photon generation, the thesis introduces general-purpose pulse-level techniques, including pulse distortion correction, memory-efficient pulse compression, and machine learning-based optimisation. These methods are shown to be transferable to other platforms, such as neutral atom arrays and superconducting qubits. A particular contribution is the implementation of scalable pulse generation using fixed-point compressed pulse representations on FPGA hardware, achieving substantial memory savings while maintaining high fidelity in simulations of quantum operations. Additionally, reinforcement learning is presented as a powerful tool for optimising complex quantum dynamics, with state-of-the-art results demonstrated across various simulated systems. Throughout the thesis, theoretical developments are supported by numerical simulations and partial experimental validation, providing important insights for the development of future quantum technologies.
This thesis addresses challenges in the experimental realisation of optical quantum computing with atom-cavity platforms and develops techniques for experimental quantum control that generalise across a range of quantum modalities. Within the framework of cavity quantum electrodynamics (cQED), methods are developed and numerically validated for fast and precise control of single atoms to generate photonic states of interest. In particular, we consider the generation of high-repetition-rate n-photon bursts and time-bin entangled states. These photonic resources are essential for applications such as boson sampling, multi-photon interference, optical quantum computing, and quantum-enhanced metrology. Experimental improvements in coherent population transfer are demonstrated using adaptive pulse shaping with acousto-optic modulators. Beyond photon generation, the thesis introduces general-purpose pulse-level techniques, including pulse distortion correction, memory-efficient pulse compression, and machine learning-based optimisation. These methods are shown to be transferable to other platforms, such as neutral atom arrays and superconducting qubits. A particular contribution is the implementation of scalable pulse generation using fixed-point compressed pulse representations on FPGA hardware, achieving substantial memory savings while maintaining high fidelity in simulations of quantum operations. Additionally, reinforcement learning is presented as a powerful tool for optimising complex quantum dynamics, with state-of-the-art results demonstrated across various simulated systems. Throughout the thesis, theoretical developments are supported by numerical simulations and partial experimental validation, providing important insights for the development of future quantum technologies.
As quantum computers advance toward larger, more powerful systems, scaling beyond a single quantum processing unit (QPU) will require the development of fast, high-fidelity interconnections between QPUs. One of the most promising strategies for achieving this is coupling qubits to optical cavities. Strong atom-cavity interactions enable the generation of atom-photon entanglement at rates orders of magnitude faster than alternative approaches, offering a critical advantage for scalable architectures. This thesis investigates the use of nanophotonic and microscale cavities to achieve exceptional atom-photon coupling while maintaining compatibility with state-of-the-art neutral atom QPUs. The experiments presented in this thesis demonstrate coherent transport between a free-space atom array and an optical cavity, coherent Rydberg excitations and interactions in the presence of the cavity interface, fast high-fidelity readout and cavity-mediated operations, and novel fabrication techniques for improved microcavities that further enhance system performance. Together, these advances outline a pathway toward utility-scale quantum computing.
Neutral atoms, trapped in optical tweezers and lattices, have gained significant attention owing to advances in laser technologies, control hardware, and innovative experimental techniques. These systems offer unique advantages such as long coherence times, natural homogeneity, and scalability, while also presenting challenges related to gate speed limitations, atom loss, slow measurements, and other imperfections. Quantum control theory has emerged as a crucial tool for advancing these technologies by enabling precise manipulation of atoms. In this thesis, we review the foundational concepts in quantum control theory, outlining both analytical approaches and numerical optimization techniques, including methods to account for experimental imperfections. A concise overview of neutral atom platforms follows, covering two distinct operational regimes: Rydberg atoms in optical tweezers and fermionic atoms in optical superlattices. The core of the thesis is dedicated to our work addressing practical control problems in neutral atom systems. First, we develop a platform-independent method for estimating and compensating nonlinear pulse distortions in experimental setups and demonstrate its use numerically for Rydberg atom excitations. Next, we tackle the challenge of implementing fast and robust gates in fermionic atom systems trapped in superlattices by optimizing lattice depths. Finally, we explore the application of Rydberg-based analog quantum simulators for variational quantum eigensolvers, using Lie-algebraic tools to analyze symmetry restrictions. This work highlights the essential role of quantum control methods in enhancing the fidelity, robustness, and applicability of neutral atom quantum technologies. It also demonstrates how combining theoretical tools, numerical optimization, and experimental considerations leads to practical solutions for scalable and high-performance quantum systems. The methods and insights developed here also offer transferable strategies for other quantum hardware architectures.
Neutral atom arrays have rapidly emerged as a leading platform for quantum computing, boasting scalable, configurable arrays of single atoms trapped in optical tweezers, fast, high-fidelity entangling gates through Rydberg interactions, and programmable, parallelized control of qubit operations. Coupling an atom array to an optical cavity opens a new frontier. Leveraging enhanced light-atom interactions in cavity quantum electrodynamics, cavity- coupled atom arrays acquire capabilities that can further expand the neutral atom toolbox, including cavity-enhanced atom readouts, atom-photon entanglement, and photon-mediated interactions between distant atoms. This thesis presents a quantum hardware platform that integrates an array of neutral atoms with a high-finesse optical cavity. After describing the design and development of the experimental apparatus, I demonstrate high-fidelity atom state readout through the cavity, achieving improved speed and atom survival compared to conventional free-space imaging methods. I then introduce a new technique for selectively controlling atom-cavity coupling on arbitrary subsets of the array, using local AC Stark shifts on the excited states of the atoms. Building on these tools, I demonstrate fast, non-destructive cavity-based readout of atom arrays, a crucial bottleneck of atom array platforms. I also showcase real-time measurement and feedback capabilities with a demonstration of classical error correction, using a register of atomic bits. Finally, I describe progress toward implementing single- and two-qubit gates within the cavity-coupled system. By combining coherent control, tunable interactions, and high-fidelity, non-destructive readout integrated and real-time feedback, the cavity-coupled Rydberg atom array offers a promising path toward fault-tolerant quantum computing.
The discovery of quantum mechanics in the 20th century forms the basis of many of the technologies that define our lives today. The ability to engineer and manipulate individual quantum systems -- even create artificial atoms -- promises a similar revolutionary leap in technology. A quantum technology of particular interest is quantum computing, which has the potential to solve problems that are intractable for classical computers, opening up new domains of computation. Meanwhile, an attractive approach to creating engineered quantum systems is circuit quantum electrodynamics (cQED). Where research initially focused on understanding the physics of cQED devices, focus has shifted to building systems capable of performing useful computations. However, this remains extremely challenging, in part due to the inherently fragile nature of the individual quantum bits, but also due to difficulties in controlling and scaling up these systems. This thesis focuses on the control aspects of building an extensible full-stack quantum computer based on superconducting transmon qubits. We define the demonstration of quantum fault-tolerance as our target application to give focus to our efforts. The QuSurf architecture for a full-stack quantum computer presented in this thesis is designed with this application in mind. We provide a detailed study of the error sources present in this system and give an overview of the relevant characterization techniques. In the second part of this thesis, we address several key challenges in the control of a quantum computer. To realize high-fidelity coherence limited gates, we present a novel tuneup protocol that achieves a tenfold speedup over the state-of-the-art. This is realized by eliminating the need for qubit initialization. We demonstrate this protocol by calibrating single-qubit gates to a coherence limited Clifford fidelity of 99.9% in one minute. Performing repeated parity checks, as is required for quantum error correction, requires reusing qubits quickly after they have been measured. By introducing a numerically optimized depletion pulse we are able to speeds up the depletion of measurement photons in a readout resonator without having to rely on specific symmetry conditions. Using this technique speed up photon depletion by more than six inverse resonator linewidths, reducing the error rate in an emulated ancilla parity check by a factor 75. Flux-pulsing based two-qubit gates are the fastest two-qubit gates. However, they are also very technically demanding. The key challenge in performing these gates is addressing the distortions that control signals experience as they traverse various electrical components. We have developed Cryoscope (short for cryogenic oscilloscope) to characterize and correct these distortions. Cryoscope is an in-situ technique that uses the qubit to sample control pulses of arbitrary shape. Even when correcting distortions to within sim0.1 two-qubit gates are history-dependent due to the long timescale upon which some of these distortions act. We have invented Net-Zero, a new type of flux-pulsing based two-qubit gate, to address this problem. It makes use of a symmetry condition of the transmon to have net-zero integral, making the gate resilient to long-timescale distortions. The gate suppresses leakage out of the computational subspace to 0.1% by making use of leakage interference and has a built-in echo effect that enhances the coherence of the gate, achieving a two-qubit gate fidelity of 99.1%. Custom software is required to perform the physics experiments needed to build and operate a quantum computer. PycQED is an open-source software framework we have developed for this purpose. We discuss the design choices and concepts of PycQED before turning our focus to characterization and calibration. Here we introduced dependency graphs as a useful abstraction and system emulation as an essential development tool for automating the characterization and calibration process. We conclude the thesis by reflecting on the limitations of our architecture and providing an outlook on the grand challenges of building a useful kilo-qubit sized quantum computer. We define these challenges as The Application Problem, The Fabrication Problem, and The Calibration Problem.
The prospect of a universal quantum computer is alluring, yet formidable. Smaller scale quantum information processing, however, has been demonstrated. Quantum networks, interlinking flying and stationary qubits, and linear optical quantum computing (LOQC) are both good candidates for scaling up such computations. A strongly coupled atom-cavity system is a promising approach for applications in these fields, both as a node in a quantum network, and as a source of photons for LOQC. This thesis demonstrates the versatile capabilities of an atom-cavity system comprising a single 87Rb atom within a macroscopic high-finesse Fabry-Pérot cavity. It operates intermittently for periods of up to 100 μs, with single-photon repetition rates of 1 MHz and an intra-cavity production efficiency of up to 85%. Exploiting the long coherence time of around 500 ns, the photons are subdivided into d time bins, with arbitrary amplitudes and phases, thus encoding arbitrary qudits. High fidelity quantum logic is shown, operating a controlled-NOT gate integrated into a photonic chip with a classical fidelity of 95.9+1.4-1.7 %. Additionally, the generation of entanglement is verified and non-classical correlations between events separated by periods exceeding the travel time across the chip by three orders of magnitude are observed. Photonic quantum simulation is performed, using temporally encoded qudits to mimic the correlation statistics of both fermions and anyons, in addition to bosons. Finally measurement-based quantum feedback is demonstrated and used to actively control the routing of temporal qubits.
A frontier challenge in quantum science and technology is the construction of scalable quantum systems which can operate in regimes beyond classical simulatability. Such systems can be used as tools for simulating and exploring complex phenomena in quantum physics; they can also be used to benchmark and test quantum algorithms. Several experimental platforms, based on a variety of quantum mechanical building blocks, are currently being pursued with these goals in mind, with state-of-the-art systems capable of controlling up to around fifty particles. In this thesis, we present the development of a new platform based on individually controlled neutral atoms. In this approach, hundreds of individual atoms are trapped in an array of optical tweezers, and they are sorted in real-time into programmable geometries in one and two dimensions. After initialization of an array, atom interactions are switched on by coherent excitation to highly excited Rydberg states, resulting in a rich spin Hamiltonian. We experimentally advance several key aspects of this platform, developing new tools for controlling strongly interacting atom arrays and probing novel quantum phases and non-equilibrium dynamics. We additionally utilize Rydberg interactions to entangle atoms, demonstrating high fidelity universal quantum logic gates as well as the preparation of fully entangled Schrödinger cat states. This work highlights the prospects for scalable quantum simulation and quantum information processing beyond the limit of classical computation using neutral atom arrays.