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Supplement 1: Broadband-tunable LP01 mode frequency shifting by Raman coherence waves in a H2-filled hollow-core photonic crystal fiber

S. T. Bauerschmidt, David Novoa, A. Abdolvand, P. St. J. Russell

Published Jan 1, 2015• 0 citations
Publisher

Abstract

Originally published in Optica on 20 June 2015 (optica-2-6-536)
DOI
10.6084/m9.figshare.4921868

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Efficient quantum frequency conversion (QFC) across large spectral gaps remains a challenge for quantum networking. We theoretically investigate a cascaded QFC in hydrogen-filled hollow-core photonic crystal fiber (HC-PCF) to convert telecom photons (1550 nm) to the visible spectrum (676 nm) via two anti-Stokes Raman shifts. Although simultaneous phase matching is impractical across such a wide window, operating in a high-pressure regime overcomes phase mismatches because the high-gain Raman coherence wave has a shorter spatial extent than the nonlinear coherence length. Maxwell-Bloch simulations show conversion efficiencies exceeding 50%. This approach offers a flexible, low-loss path for integrating disparate quantum technologies in a single fiber platform.
We report on the efficient, tunable, and selective frequency up-conversion of a supercontinuum spectrum via molecular modulation in a hydrogen-filled hollow-core photonic crystal fiber. The vibrational Q(1) Raman transition of hydrogen is excited in the fiber by a pump pre-pulse, enabling the excitation of a synchronous, collective oscillation of the molecules. This coherence wave is then used to up-shift the frequency of an arbitrarily weak, delayed probe pulse. Perfect phase-matching for this process is achieved by using higher order fiber modes and adjusting the pressure of the filling gas. Conversion efficiencies of ~50% are obtained within a tuning range of 25 THz.