A quantum memory scheme with a frequency conversion interface has been proposed, where the processes of storage/retrieval of photons in a resonant polyatomic ensemble and single-photon frequency conversion in a nonlinear medium are combined in a single cavity. Compared to independent quantum memory and frequency converter, the proposed approach allows one to avoid unnecessary losses during radiation input/output and to completely overcome the need to match the operating wavelengths and bands of two devices. A solution of the Heisenberg–Langevin equations that describes the cycle of storage followed by retrieval of a single-photon wave packet has been obtained and used to formulate the conditions for achieving a high quantum memory efficiency, in particular, modified impedance matching conditions.
A quantum memory scheme with a frequency conversion interface has been proposed, where the processes of storage/retrieval of photons in a resonant polyatomic ensemble and single-photon frequency conversion in a nonlinear medium are combined in a single cavity. Compared to independent quantum memory and frequency converter, the proposed approach allows one to avoid unnecessary losses during radiation input/output and to completely overcome the need to match the operating wavelengths and bands of two devices. A solution of the Heisenberg–Langevin equations that describes the cycle of storage followed by retrieval of a single-photon wave packet has been obtained and used to formulate the conditions for achieving a high quantum memory efficiency, in particular, modified impedance matching conditions.
The ability to control the optical frequency of quantum state carriers (i.e. photons) is an important functionality for future quantum networks. It allows all matter quantum systems - nodes of the network - to be compatible with the telecommunication C-band, therefore enabling long distance fiber quantum communication between them. It also allows dissimilar nodes to be connected with each other, thus resulting in heterogeneous networks that can take advantage of the different capabilities offered by the diversity of its constituents. Quantum memories are one of the building blocks of a quantum network, enabling the storage of quantum states of light and the entanglement distribution over long distances. In our group, two different types of memories are investigated: a cold atomic ensemble and an ion-doped crystal. In this thesis I investigate the quantum frequency conversion of narrow-band photons, emitted or absorbed by optical quantum memories, with two different objectives: the first one is to connect quantum memories emitting or absorbing visible single photons with the telecommunication wavelengths, where fiber transmission loss is minimum. The second and main goal is to study the compatibility between disparate quantum nodes, emitting or absorbing photons at different wavelengths. More precisely the objective is to achieve a quantum connection between the two optical memories studied using quantum frequency conversion techniques. The main core of this work is the quantum frequency conversion interface that bridges the gap between the cold ensemble of Rubidium atoms, emitting photons at 780nm, and the Praseodymium ion doped crystal, absorbing photons at 606nm. This interface is composed of two different frequency conversion devices, where a cascaded conversions takes place: the first one converts 780nm photons to the telecommunication C-band, and the second one converts them back to visible, at 606nm. This comes with several challenges such as conversion efficiency, phase stability and parasitic noise reduction, which are important considerations to show the conservation of quantum behaviors through the conversion process. This work can be divided in three parts. In a first one, we built a quantum frequency conversion interface between 606nm and the C-band wavelength, capable of both up and down-conversion of single photon level light. We also characterized the noise processes involved in this specific conversion. In the down-conversion case we showed that memory compatible heralded single photons emitted from a photon pair source preserve their non-classical properties through the conversion process. In the up-conversion case, we showed the storage of converted telecom photons in the praseodymium doped crystal, and their retrieval with high signal to noise ratio. The second part of the work was devoted to the conversion of photons from an emissive Rubidium atomic quantum memory to the telecom C band. In this work we converted the heralding photons from the atomic ensemble and measured non-classical correlations between a stored excitation and a C-band photon, necessary for quantum repeater applications. In the last part of the thesis, we setup the full frequency conversion interface and showed that heralded photons emitted by the atomic ensemble are converted, stored in the solid state memory and retrieved with high signal to noise ratio. We demonstrated that a single collective excitation stored in the atomic ensemble is transfered to the crystal by mean of a single photon at telecom wavelength. We also showed time-bin qubit transfer between the two quantum memories. This work represents the first proof of principle of a photonic quantum connection between disparate quantum memory nodes. The results presented in this thesis pave the way towards the realization of modular and hybrid quantum networks.
We demonstrate the storage and retrieval of heralded single photons in a fiber-based cavity quantum memory. The photons are stored, and retrieved, from the memory using quantum frequency conversion which switches the photon into, and out of, resonance with the cavity. The photons, generated in the telecom O-band with a bandwidth of 81 GHz, are retrieved from the memory with a 1/ e lifetime of 1.64 µs, or 32.8 cavity round trips. We show that non-classical photon statistics remain for 70 round trips. The internal memory efficiency after 0.5 µs of storage is 10.9 ± 0.5%; a coupling efficiency of 60% into the memory cavity yields a total efficiency of 6.0 ± 0.3%. These results mark a crucial step forward in the development of fiber-based quantum memories, and high-bandwidth memories operating at telecom wavelengths, with applications to photon source multiplexing and fiber-based quantum networking.
High-speed long-range quantum communication requires combining frequency multiplexed photonic channels with quantum memories. We experimentally demonstrate an integrated quantum frequency conversion protocol that can convert between wavelength division multiplexing channels in the telecom range with an efficiency of 55±8% and a noise subtracted Hong-Ou-Mandel (HOM) dip visibility of 84.5%. This protocol is based on a cascaded second order nonlinear interaction and can be used to interface a broad spectrum of frequencies with narrowband quantum memories, or alternatively as a quantum optical transponder, efficiently interfacing different regions of a frequency-multiplexed spectrum.
Single-photon frequency conversion for quantum interface plays an important role in quantum communications and networks, which is crucial for the realization of quantum memory, faithful entanglement swapping and quantum teleportation. In this talk, I will present our recent experiments about single-photon frequency conversion based on quadratic nonlinear processes. Firstly, we demonstrated spectrum compression of broadband single photons at the telecom wavelength to the near-visible window. A positively chirped single-photon-level laser pulse and a negatively chirped classical one are converted to a narrowband single-photon pulse, with a spectrum compression factor of 58, through sum-frequency generation (SFG), marking a critical step towards coherent photonic interface. Secondly, we demonstrated the nonlinear interaction between two chirped broadband single-photon-level coherent states. A high SFG efficiency of 1.06 × 10−7 is realized, which may be utilized to achieve heralding entanglement at a distance. Finally, we theoretically introduced and experimentally demonstrated single-photon frequency conversion in the telecom band, enabling switching of single photons between dense wavelength-division multiplexing channels. Using cascaded quasi-phase matched sum/difference frequency generation, the signal photon of a photon pair from spontaneous down-conversion is precisely shifted to identically match its counterpart, i.e. idler photon, in frequency to manifest a clear non-classical dip in the Hong-Ou-Mandel interference. Moreover, quantum entanglement between the photon pair is maintained after the frequency conversion. Our researches have realized three significant quantum interfaces via single-photon frequency conversion, which hold great promise for the development of quantum communications and networks.
In this paper we experimentally demonstrated a broadband scheme of the multiresonator quantum memory-interface. The microwave photonic scheme consists of the system of mini-resonators strongly interacting with a common broadband resonator coupled with the external waveguide. We have implemented the impedance matched quantum storage in this scheme via controllable tuning of the mini-resonator frequencies and coupling of the common resonator with the external waveguide. Proof-of-principal experiment has been demonstrated for broadband microwave pulses when the quantum efficiency of 16.3% was achieved at room temperature. By using the obtained experimental spectroscopic data, the dynamics of the signal retrieval has been simulated and promising results were found for high-Q mini-resonators in microwave and optical frequency ranges. The results pave the way for the experimental implementation of broadband quantum memory-interface with quite high efficiency η > 0.99 on the basis of modern technologies, including optical quantum memory at room temperature.
The storage of single photons generated via nondegenerate spontaneous parametric down-conversion in a cavity with a PPKTP crystal in quantum memory based on an atomic frequency comb in a Eu:YSO crystal is demonstrated. A technique for preparing spectral profiles within the absorption line of a doped crystal that are matched to the spectrum of single-photon radiation is developed. For storage times of 250 and 166 ns, quantum memory efficiencies of 3 and 7% have been obtained with signal-to-noise ratios of 1/4 and 1/2, respectively.