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Modèles efficaces de systèmes quantiques ouverts bipartis

Angela Riva

Published Feb 2, 2026• 0 citations
OpenAlex

Abstract

This thesis develops model reduction methods for open quantum system dynamics, yielding efficient models for bipartite systems, with direct application to circuit QED and broader applicability beyond this platform. First, we consider dissipative dynamics characterized by timescale separation, which translates to a gap on the real axis of the spectrum of the Liouvillian generating it. This allows to compute the reduced evolution for a target subsystem by adiabatically eliminating fast-decaying degrees of freedom. A Sylvester equation integral representation yields closed forms for the reduced generators and explicit reconstruction maps to arbitrary order without a preliminary interaction-picture averaging step, providing a linear center manifold description that separates long-lived from fast-decaying modes by the real parts of the spectrum. The reduced dynamics takes place on the center manifold, that is, the spectral subspace associated with eigenvalues whose real parts are small (long-lived modes), while placing no restriction on imaginary parts, thus allowing for fast unitary dynamics on the target subsystem. We further demonstrate the equivalence of such a geometric approach to adiabatic elimination with the time-convolutionless master equation framework, by showing that the maps defining the reduced model satisfy the same invariance equation in both frameworks. The time-convolutionless formulation of adiabatic elimination extends to cases where the target system undergoes fast unitary dynamics and retains explicit time dependence in the reduced model, hence capturing initial transients that are neglected in time-independent geometric reductions. Second, we apply a unitary chain mapping of microscopic system–environment Hamiltonians to a nearest-neighbor form, enabling efficient time evolution exploiting tensor network time evolution algorithms based on the time dependent variational principle. Accuracy of the tensor network representation, and thus the size of the reduced model, is controlled by entanglement entropy growth, which we quantify numerically. While the methods are general and apply beyond the specific platform considered, we focus on dispersive readout in circuit QED (a qubit dipolarly coupled to a driven, lossy cavity). We quantify the dependence of the relaxation time $T_1$ of the qubit on intracavity photon number $\bar n$ (and thus on the drive amplitude) and on the spectral structure of the environment, and compute the emission spectrum directly from environmental observables. Simulations including a Purcell notch filter predict a decrease of $T_1$ with increasing drive power, a qualitatively different behavior with respect to Born–Markov–secular GKSL predictions but consistent with experimental trends, indicating that explicit filter modeling is required in this case. Together, the results specify when reduced Liouvillian models under a dissipative gap are reliable and when microscopic, non-perturbative simulations are required.

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In open quantum systems theory, reduced models are invaluable for conceptual understanding and computational efficiency. Adiabatic elimination is a useful model reduction method for systems with separated timescales, where a reduced model is derived by discarding rapidly decaying degrees of freedom. So far, adiabatic elimination has been formulated using a geometric approach, which provides a versatile and general framework. This article introduces a reformulation of adiabatic elimination through the framework of the time-convolutionless (TCL) master equation, a widely recognized tool for computing projected time evolution in open quantum systems. We show that the TCL master equation formulation yields results equivalent to those obtained from the geometric formulation. By applying the TCL master equation formulation to typical examples, we demonstrate a practical methodology for performing adiabatic elimination calculation. This study not only bridges two previously independent approaches, thereby making the adiabatic elimination method accessible to a broader audience, but also enables the analysis of complex cases that are challenging within the geometric formulation. Additionally, it reveals a geometric interpretation of the TCL master equation formalism.

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This thesis develops model reduction methods for open quantum system dynamics, yielding efficient models for bipartite systems, with direct application to circuit QED and broader applicability beyond this platform. First, we consider dissipative dynamics characterized by timescale separation, which translates to a gap on the real axis of the spectrum of the Liouvillian generating it. This allows to compute the reduced evolution for a target subsystem by adiabatically eliminating fast-decaying degrees of freedom. A Sylvester equation integral representation yields closed forms for the reduced generators and explicit reconstruction maps to arbitrary order without a preliminary interaction-picture averaging step, providing a linear center manifold description that separates long-lived from fast-decaying modes by the real parts of the spectrum. The reduced dynamics takes place on the center manifold, that is, the spectral subspace associated with eigenvalues whose real parts are small (long-lived modes), while placing no restriction on imaginary parts, thus allowing for fast unitary dynamics on the target subsystem. We further demonstrate the equivalence of such a geometric approach to adiabatic elimination with the time-convolutionless master equation framework, by showing that the maps defining the reduced model satisfy the same invariance equation in both frameworks. The time-convolutionless formulation of adiabatic elimination extends to cases where the target system undergoes fast unitary dynamics and retains explicit time dependence in the reduced model, hence capturing initial transients that are neglected in time-independent geometric reductions. Second, we apply a unitary chain mapping of microscopic system–environment Hamiltonians to a nearest-neighbor form, enabling efficient time evolution exploiting tensor network time evolution algorithms based on the time dependent variational principle. Accuracy of the tensor network representation, and thus the size of the reduced model, is controlled by entanglement entropy growth, which we quantify numerically. While the methods are general and apply beyond the specific platform considered, we focus on dispersive readout in circuit QED (a qubit dipolarly coupled to a driven, lossy cavity). We quantify the dependence of the relaxation time T1T_1T1​ of the qubit on intracavity photon number nˉ\bar nnˉ (and thus on the drive amplitude) and on the spectral structure of the environment, and compute the emission spectrum directly from environmental observables. Simulations including a Purcell notch filter predict a decrease of T1T_1T1​ with increasing drive power, a qualitatively different behavior with respect to Born–Markov–secular GKSL predictions but consistent with experimental trends, indicating that explicit filter modeling is required in this case. Together, the results specify when reduced Liouvillian models under a dissipative gap are reliable and when microscopic, non-perturbative simulations are required.
We provide model reduction formulas for open quantum systems consisting of a target component which weakly interacts with a strongly dissipative environment. The time-scale separation between the uncoupled dynamics and the interaction allows to employ tools from center manifold theory and geometric singular perturbation theory to eliminate the variables associated to the environment (adiabatic elimination) with high-order accuracy. An important specificity is to preserve the quantum structure: reduced dynamics in (positive) Lindblad form and coordinate mappings in Kraus form. We provide formulas of the reduced dynamics. The main contributions of this paper are (i) to show how the decomposition of the environment into KKK components enables its efficient treatment, avoiding the quantum curse of dimension; and (ii) to extend the results to the case where the target component is subject to Hamiltonian evolution at the fast time-scale. We apply our theory to a microwave superconducting quantum resonator subject to material losses, and we show that our reduced-order model can explain the transmission spectrum observed in a recent pump probe experiment.
Modèles efficaces de systèmes quantiques ouverts bipartites Cette thèse développe des méthodes de réduction de modèles pour la dynamique des systèmes quantiques ouverts, conduisant à des modèles efficaces pour les systèmes bipartites, avec une application directe à la QED en circuit et une portée plus large au-delà de cette plateforme. Nous considérons tout d'abord des dynamiques dissipatives caractérisées par une séparation d'échelles de temps, qui se traduit par un écart spectral (gap) sur l'axe réel du spectre du Liouvillien générateur. Cela permet de calculer l'évolution réduite d'un sous-système cible en éliminant adiabatiquement les degrés de liberté à décroissance rapide. Une représentation intégrale sous forme d'équation de Sylvester fournit des expressions fermées pour les générateurs réduits ainsi que des applications de reconstruction explicites à tout ordre, sans étape préalable de moyennisation dans l'image d'interaction, ce qui donne une description linéaire en variété centrale séparant les modes de longue durée de vie des modes à décroissance rapide au moyen des parties réelles du spectre. La dynamique réduite se déroule sur la variété centrale, c'est-à-dire le sous-espace spectral associé aux valeurs propres dont les parties réelles sont petites (modes de longue durée de vie), sans imposer de restriction sur les parties imaginaires, ce qui autorise une dynamique unitaire rapide sur le sous-système cible. Nous démontrons en outre l'équivalence d'une telle approche géométrique de l'élimination adiabatique avec le formalisme des équations maîtresses sans mémoire (time-convolutionless), en montrant que les applications définissant le modèle réduit satisfont la même équation d'invariance dans les deux cadres. La formulation sans mémoire de l'élimination adiabatique s'étend à des cas où le système cible subit une dynamique unitaire rapide et conserve une dépendance temporelle explicite dans le modèle réduit, ce qui permet de capturer les transitoires initiaux qui sont négligés dans les réductions géométriques indépendantes du temps. Dans un deuxième temps, nous appliquons une transformation unitaire en chaîne des Hamiltoniens microscopiques système-environnement vers une forme à interactions de voisinage immédiat, permettant une évolution temporelle efficace au moyen d'algorithmes de réseaux de tenseurs basés sur le principe variationnel dépendant du temps. La précision de la représentation en réseau de tenseurs, et donc la taille du modèle réduit, est contrôlée par la croissance de l'entropie d'intrication, que nous quantifions numériquement. Bien que les méthodes soient générales et s'appliquent au-delà de la plateforme spécifique considérée, nous nous concentrons sur la mesure dispersive en QED en circuit (un qubit couplé dipolairement à une cavité excitée et dissipative). Nous quantifions la dépendance du temps de relaxation T₁ du qubit au nombre moyen de photons intracavité n̄ (et donc à l'amplitude du drive) ainsi qu'à la structure spectrale de l'environnement, et calculons le spectre d'émission directement à partir d'observables de l'environnement. Des simulations incluant un filtre de Purcell à encoche prédisent une diminution de T₁ lorsque la puissance du drive augmente, un comportement qualitativement différent des prédictions de type GKSL dans l'approximation de Born-Markov-séculaire, mais cohérent avec les tendances expérimentales, ce qui indique qu'un modèle incluant explicitement le filtre est nécessaire dans ce cas. Pris ensemble, ces résultats précisent dans quels régimes les modèles liouvilliens réduits sous l'hypothèse d'un gap dissipatif sont fiables et dans quels cas des simulations microscopiques non perturbatives sont nécessaires.
Adiabatic elimination methods allow the reduction of the space dimension needed to describe systems whose dynamics exhibit separation of timescale. For open quantum systems, it consists in eliminating the fast part assuming it has almost instantaneously reached its steady state and obtaining an approximation of the evolution of the slow part. These methods can be applied to eliminate a linear subspace within the system Hilbert space or, alternatively, to eliminate a fast subsystem in a bipartite quantum system. In this work, we extend an adiabatic elimination method used for removing fast degrees of freedom within a system [Phys. Rev. A 101, 042102 (2020)] to eliminate a subsystem from an open bipartite quantum system. As an illustration, we apply our technique to a dispersively coupled two-qubit system and in the case of the open Rabi model.
Adiabatic elimination is a model reduction technique commonly used by physicists to eliminate quickly dissipating components from quantum physics equations. We revisit this technique when the target non-dissipating component is driven by Hamiltonian actuation at a fast timescale. Following center manifold theory, we can still write reduced dynamics for the target component, but there may be new conditions to ensure that it takes the standard structure of quantum dynamics, i.e. evolution equations of Lindblad type and coordinate changes in Kraus map form. We here propose various approaches to recover a Lindblad form up to third-order terms: without conditions for finite-dimensional systems, and under some finite set conditions for infinite-dimensional systems.
Simplifying composite open quantum systems through model reduction is central to enable their analytical and numerical understanding. In this work, we introduce a self-consistent approach to eliminate the cavity degrees of freedom of cavity quantum electrodynamics (CQED) devices in the non-adiabatic regime, where the cavity memory time is comparable with the timescales of the atom dynamics. To do so, we consider a CQED system consisting of a two-level atom coupled to a single-mode cavity, both subsystems interacting with the environment through an arbitrary number of ports, within the input-output formalism. A self-consistency equation is derived for the reduced atom dynamics. This allows retrieving an exact expression for the effective Purcell-enhanced emission rate and, under reasonable approximations, a set of self-consistent dynamical equations and input-output relations for the effective two level atom. The resulting reduced model captures non-Markovian features, characterized through an effective Lindblad equation exhibiting two decoherence rates, a positive and a negative one. In the continuous-wave excitation regime, we benchmark our approach by computing effective steady states and output flux expressions beyond the low-power excitation regime, for which a semi-classical treatment is usually applied. We also compute two-time correlations and spectral densities, showing an excellent agreement with full cavity quantum electrodynamics simulations, except in the strong-coupling, high-excitation regime. Our results provide a practical framework for reducing the size of CQED models, which could be generalized to more complex atom and cavity configurations.
In open quantum systems theory, reduced models are invaluable for conceptual understanding and computational efficiency. Adiabatic elimination is a useful model reduction method for systems with separated timescales, where a reduced model is derived by discarding rapidly decaying degrees of freedom. So far, adiabatic elimination has been formulated using a geometric approach, which provides a versatile and general framework. This article introduces a reformulation of adiabatic elimination through the framework of the time-convolutionless (TCL) master equation, a widely recognized tool for computing projected time evolution in open quantum systems. We show that the TCL master equation formulation yields results equivalent to those obtained from the geometric formulation. By applying the TCL master equation formulation to typical examples, we demonstrate a practical methodology for performing adiabatic elimination calculation. This study not only bridges two previously independent approaches, thereby making the adiabatic elimination method accessible to a broader audience, but also enables the analysis of complex cases that are challenging within the geometric formulation. Additionally, it reveals a geometric interpretation of the TCL master equation formalism.