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Electric Stern-Gerlach Interferometer with Rydberg Atoms

Nick Siegner

Published Jun 30, 2025• 0 citations
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We show that superficially similar implementations of Stern-Gerlach Interferometers (SGIs) are expected to differ dramatically in their sensitivity to fields transverse to the primary acceleration direction. These transverse fields unavoidably accompany any static magnetic or electric field gradients, and have been shown by Comparat [Phys. Rev. A 101, 023606 (2020)] to limit the precision application of SGIs. As a concrete example, we consider SGIs with ultracold Rb Rydberg atoms accelerated by spatially-varying electric fields. We find that the deleterious effect of transverse fields imply that only some implementations (sequences of field gradients, internal state swaps, and so-on) may exhibit fringes with high visibility.

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A coherent electric analogue of the Stern-Gerlach experiment has been performed with helium atoms in Rydberg states. The atoms, travelling in pulsed supersonic beams, were prepared in superpositions of Rydberg states with different static electric dipole polarisabilities using pulses of microwave radiation. State-dependent forces were then exerted on them, transverse to their direction of propagation, using inhomogeneous electric fields. These fields were generated between a pair of electrodes in a wedge configuration. The forces applied resulted in the coherent evolution of each atomic wavepacket into a superposition of spatially separated momentum states. The classical paths of least action associated with these momentum states evolved over time up to a separation of ∼2 nm. The coherent evolution of the atoms, and hence the superposition of atomic wavepackets in this ‘half-loop’ electric Rydberg-atom interferometer, was monitored by measuring the internal Rydberg state populations at the end of each measurement cycle. The experimental data are in good quantitative agreement with the results of semiclassical calculations of the phase evolution of the atomic superposition states which account for contributions from Stark shifts, the momentum differences between the classical paths of least action through the apparatus, and the spatial separation of the atomic wavepackets.

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An electric analogue of the longitudinal Stern-Gerlach matter-wave interferometer has been realized for atoms in Rydberg states with high principal quantum number n. The experiments were performed with He atoms prepared in coherent superpositions of the n=55 and n=56 circular Rydberg states in a zero electric field by a π/2 pulse of resonant microwave radiation. These atoms were subjected to a pulsed inhomogeneous electric field to generate a superposition of momentum states before a π pulse was applied to invert the internal states. The same pulsed inhomogeneous electric field was then reapplied for a second time to transform the motional states to have equal momenta before a further π/2 pulse was employed to interrogate the final Rydberg state populations. This Hahn-echo microwave pulse sequence, interspersed with a pair of equivalent inhomogeneous electric field pulses, yielded two spatially separated matter waves. Interferences between these matter waves were observed as oscillations in the final Rydberg state populations as the amplitude of the pulsed electric field gradients was adjusted.

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Some New Effects in Atom Stern-Gerlach Interferometry

Renaud Mathevet, K. Brodsky, F. Perales +5 more

Springer eBooks•Jan 1, 2001•2 citations
We show that superficially similar implementations of Stern-Gerlach Interferometers (SGIs) are expected to differ dramatically in their sensitivity to fields transverse to the primary acceleration direction. These transverse fields unavoidably accompany any static magnetic or electric field gradients, and have been shown by Comparat [Phys. Rev. A 101, 023606 (2020)] to limit the precision application of SGIs. As a concrete example, we consider SGIs with ultracold Rb Rydberg atoms accelerated by spatially-varying electric fields. We find that the deleterious effect of transverse fields imply that only some implementations (sequences of field gradients, internal state swaps, and so-on) may exhibit fringes with high visibility.
A coherent electric analogue of the Stern-Gerlach experiment has been performed with helium atoms in Rydberg states. The atoms, travelling in pulsed supersonic beams, were prepared in superpositions of Rydberg states with different static electric dipole polarisabilities using pulses of microwave radiation. State-dependent forces were then exerted on them, transverse to their direction of propagation, using inhomogeneous electric fields. These fields were generated between a pair of electrodes in a wedge configuration. The forces applied resulted in the coherent evolution of each atomic wavepacket into a superposition of spatially separated momentum states. The classical paths of least action associated with these momentum states evolved over time up to a separation of ∼2 nm. The coherent evolution of the atoms, and hence the superposition of atomic wavepackets in this ‘half-loop’ electric Rydberg-atom interferometer, was monitored by measuring the internal Rydberg state populations at the end of each measurement cycle. The experimental data are in good quantitative agreement with the results of semiclassical calculations of the phase evolution of the atomic superposition states which account for contributions from Stark shifts, the momentum differences between the classical paths of least action through the apparatus, and the spatial separation of the atomic wavepackets.
An electric analogue of the longitudinal Stern-Gerlach matter-wave interferometer has been realized for atoms in Rydberg states with high principal quantum number n. The experiments were performed with He atoms prepared in coherent superpositions of the n=55 and n=56 circular Rydberg states in a zero electric field by a π/2 pulse of resonant microwave radiation. These atoms were subjected to a pulsed inhomogeneous electric field to generate a superposition of momentum states before a π pulse was applied to invert the internal states. The same pulsed inhomogeneous electric field was then reapplied for a second time to transform the motional states to have equal momenta before a further π/2 pulse was employed to interrogate the final Rydberg state populations. This Hahn-echo microwave pulse sequence, interspersed with a pair of equivalent inhomogeneous electric field pulses, yielded two spatially separated matter waves. Interferences between these matter waves were observed as oscillations in the final Rydberg state populations as the amplitude of the pulsed electric field gradients was adjusted.