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Quantum Review Letters

On-chip quantum frequency conversion of 2μm photon in thin-film lithium niobate waveguide

Zishuo Gu, Chenyu Wang, Mengwen Chen, Zikang Wang, Hua-Ying Liu, Xiao-Hui Tian, Kunpeng Jia, Yong Zhang, S. Konrad Zhu, Zhenda Xie

Published Jan 1, 2026• 0 citations
Publisher

Abstract

Quantum frequency conversion (QFC) plays a critical role in practical quantum information technology as it provides a bridge among different quantum devices, which usually operate at different optimal wavelength. Photons with longer wavelength feature lower propagation loss and lower solar radiation noise in free space, hence hold promise for daylight long distance quantum communication. Besides, wavelength over 2 μ m also overlap with the absorption band of many important molecules, hence is of great importance for gases and molecules detection. Yet development of technology in this region has been hindered primarily by the spectral mismatch with other quantum devices, notably quantum detection and memories, which optimally operate in the visible band. Here, we demonstrate the first QFC of 2 μ m photons to the visible region on domain-engineered thin-film lithium niobate (TFLN) platform. Benefiting from the strong nonlinearity in such integrated platform, the highest internal quantum conversion efficiency of 42% is achieved at an exceptionally low pump saturation power of only 58 mW . This work provides an efficient interconnection between photons operating at the visible and 2 μ m bands in the integrated platform, pushing forward the development of practical quantum chips for application of quantum communication, sensing and metrology in the future. • Strong mode confinement and domain-engineered thin film lithium niobate (TFLN), combined with large χ ( 2 ) , enable efficient on-chip nonlinear conversion. • First demonstration of quantum frequency conversion (QFC) of 2 μ m band photon on thin film lithium niobate.

DOI
10.1016/j.qrl.2026.01.002

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Quantum frequency conversion (QFC) plays a critical role in practical quantum information technology as it provides a bridge among different quantum devices, which usually operate at different optimal wavelength. Photons with longer wavelength feature lower propagation loss and lower solar radiation noise in free space, hence hold promise for daylight long distance quantum communication. Besides, wavelength over 2 μ m also overlap with the absorption band of many important molecules, hence is of great importance for gases and molecules detection. Yet development of technology in this region has been hindered primarily by the spectral mismatch with other quantum devices, notably quantum detection and memories, which optimally operate in the visible band. Here, we demonstrate the first QFC of 2 μ m photons to the visible region on domain-engineered thin-film lithium niobate (TFLN) platform. Benefiting from the strong nonlinearity in such integrated platform, the highest internal quantum conversion efficiency of 42% is achieved at an exceptionally low pump saturation power of only 58 mW . This work provides an efficient interconnection between photons operating at the visible and 2 μ m bands in the integrated platform, pushing forward the development of practical quantum chips for application of quantum communication, sensing and metrology in the future. • Strong mode confinement and domain-engineered thin film lithium niobate (TFLN), combined with large χ ( 2 ) , enable efficient on-chip nonlinear conversion. • First demonstration of quantum frequency conversion (QFC) of 2 μ m band photon on thin film lithium niobate.
Quantum frequency conversion (QFC) plays a crucial role in constructing seamless interconnection between quantum systems operating at different wavelengths. To advance future quantum technology, chip-scale integrated QFC components, featuring high efficiency, small footprint, low power consumption, and high scalability, are indispensable. In this work, we demonstrate the first hybrid integrated QFC chip on a thin-film lithium niobate platform that connects the telecom and visible bands. Benefiting from the periodically poled microring resonator with ultra-high normalized conversion efficiency of 386,000%/W, an ultra-low pump power of 360 μW is achieved, which is more than two orders of magnitude lower than the traditional straight waveguide scheme. By injecting current into the chip, an on-chip quantum efficiency of 57% and a noise count of ∼7000 counts per second are achieved. Such an electrically pumped, integrated, and scalable QFC chip would significantly advance the integration of quantum networks and the development of chip-scale quantum optical systems.
Within the last decade, thin-film lithium niobate (TFLN) has emerged as a leading integrated photonics platform with immediate applications in classical communications. Concurrently, TFLN components tailored to the requirements of photonic quantum information processing have also garnered considerable interest. Chief among these is the quasi-phase matched (QPM) nonlinear frequency mixer—implemented via periodic domain inversion in ferroelectric lithium niobate—which can be used to generate photon pairs, squeezed states of light, and to perform single photon frequency conversion. Here, we demonstrate progress towards realizing a spectrally separable photon pair source in lithium niobate via waveguide dispersion engineering—a technique uniquely enabled by sub-wavelength optical mode confinement in the thin-film platform. Subsequently, we design optimize a scalable fabrication process to produce QPM TFLN devices for applications that require strict adherence to a specified operating wavelength, such as quantum frequency conversion in a quantum communications network. Finally, we explore how high-performance electro-optic devices can be combined with these nonlinear optical devices to realize a multi-functional platform in which quantum states of light can be generated and manipulated within a single, compact photonic integrated circuit.
Quantum frequency conversion (QFC) is essential for bridging the spectral gap between stationary qubits and low-loss optical communication channels. In this work, we demonstrate a short-wavelength-pumping QFC with the first-order quasi-phase matching period of 3.07 um on thin-film lithium niobate, converting ultraviolet photons to the telecom C-band. By constructing a theoretical model that correlates the normalized conversion efficiency with domain defects in the short-period phase-matched waveguide, we found the critical tolerance of domain defects along the waveguide should be ≤2\le 2≤2 (excluding the ends). Based on this, we achieved a theoretical limit normalized conversion efficiency of 839%/(W*cm^2) for the fundamental guided mode through fabrication optimization. Furthermore, we propose a robust noise suppression strategy for short-wavelength pumping by utilizing the counter-tuning behaviors of difference-frequency generation and spontaneous parametric down-conversion. By combining these advances with ultra-narrowband filtering, we achieve a record-high external efficiency of 28.8% and an ultra-low noise of 35 counts per second. This high-performance QFC connecting ultraviolet and telecom bands satisfies the stringent requirements for long-lived remote ion-ion entanglement in scalable quantum networks [W.-Z. Liu et al., Nature (2026)].
Quantum frequency conversion (QFC) is essential for bridging the spectral gap between stationary qubits and low-loss optical communication channels. Practicable QFC interfaces connecting ultraviolet and telecommunication bands are of great significance but have remained elusive, constrained by the dual challenges of a high-performance frequency converter and effective noise suppression in short-wavelength pumping configurations. We address this by demonstrating the phase-matching mechanism with domain defects and differential-tuning behavior of the spontaneous parametric down-conversion noises. Based on a quantitative analysis of performance degradation induced by domain defects, we propose specific fabrication guidelines and experimentally achieve an ultrahigh normalized conversion efficiency of 839%/(W cm^{2}) for the fundamental guided mode in thin-film lithium niobate waveguides. Meanwhile, we reveal a new noise control mechanism for short-wavelength pumping by utilizing the differential-tuning behaviors of difference-frequency generation and spontaneous parametric down-conversion processes. Then a single-stage QFC from 393 nm to the telecom C band with a record-high external efficiency of 28.8% and an ultralow noise level of 35 counts per second is achieved experimentally. The proposed mechanisms would enable other QFCs with higher efficiency and lower noise, advancing the development of scalable quantum networks. Furthermore, it holds significant potential for driving progress in both classical and integrated nonlinear photonics.
In this work, we demonstrate a quantum pulse gate (QPG) in thin-film lithium niobate. QPGs enable the selective manipulation and detection of temporal modes of quantum light and form the basis of numerous applications in photonic quantum technologies. To date, their widespread adaption is held back by two main limitations: restricted wavelength and polarization combinations of the involved fields and low normalized conversion efficiencies. We overcome these limitations through developing a QPG in thin-film lithium niobate. We design a waveguide geometry that provides the required dispersion properties for a highly efficient type-0 sum-frequency generation.We verify our design through mapping of the phase matching intensity, and demonstrate high-quality QPG operation by measuring a temporal-mode selectivity of (96.8$\pm1.7)1.7)% on par with existing QPGs. Thanks to the strong confinement in thin-film lithium niobate, we succeed in demonstrating an internal conversion efficiency of (89.61.7)\pm0.1)0.1)% for a pump power of only 20mW in front of our sample. This yields a lower-bound estimate for the normalized conversion efficiency of (18100.1)\pm10)10)10)\mathrm{W}^{-1}\mathrm{cm}^{-2}$, three orders of magnitude higher than in previous QPGs. Our results establish thin-film lithium niobate as ideal platform for high-performance QPGs and are a major step towards practical QPGs for photonic quantum technologies.
Abstract The lithium niobate on insulator (LNOI) platform has revolutionized lithium niobate materials, and a series of quantum photonic chips have exhibited unprecedented performances. Quantum frequency conversion (QFC) that enables quantum state preservation during frequency conversion is crucial in quantum technology. This work demonstrates a low-noise QFC process on the LNOI nanophotonic platform, connecting telecom and near-visible bands. An internal conversion efficiency of 73% and an on-chip noise count of 900 counts per second (cps) are achieved. Furthermore, the preservation of quantum statistical properties is verified, indicating the QFC chip’s promise for extensive applications of LNOI integrated circuits in quantum information. Based on this chip, we constructed an upconversion single-photon detector with a detection efficiency of 8.7% and a noise of 300 cps, paving the way to integrated on-chip single-photon detection. The realization of a low-noise QFC device also provide a pathway for practical chip-scale QFC-based quantum systems in heterogeneous configurations.