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Frontiers in Optics

Efficient Bi-Photon State Characterisation and Its Applications in Quantum Technologies

Ebrahim Karimi

Published Jan 1, 2025• 0 citations
Publisher

Abstract

High-dimensional photonic entangled states are key resources for advancing quantum imaging, quantum sensing, secure communication, and quantum computation. The most common method for generating such states is spontaneous parametric down-conversion (SPDC), in which a pump photon splits into two daughter photons that share correlations across multiple photonic degrees of freedom. Characterising these high-dimensional states, however, is highly challenging, as it scales quadratically with the state dimensionality and usually requires large sets of projective measurements within the framework of positive operator-valued measures (POVMs).

DOI
10.1364/fio.2025.fth3e.2

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High-dimensional photonic entangled states are key resources for advancing quantum imaging, quantum sensing, secure communication, and quantum computation. The most common method for generating such states is spontaneous parametric down-conversion (SPDC), in which a pump photon splits into two daughter photons that share correlations across multiple photonic degrees of freedom. Characterising these high-dimensional states, however, is highly challenging, as it scales quadratically with the state dimensionality and usually requires large sets of projective measurements within the framework of positive operator-valued measures (POVMs).
Quantum states of light, such as single photons, pairs of entangled photons, and squeezed light are a key resource for photonic quantum technologies. All these states can be obtained via the nonlinear optical effect of spontaneous parametric down-conversion (SPDC). In SPDC, a higher-energy photon of a coherent beam (pump) splits in two lower-energy daughter photons, called signal and idler. The photons of such a pair can be entangled in polarization, time/frequency, and position/momentum. Efficient generation of photon pairs requires a high second-order susceptibilityχ(2)\chi^{(2)}χ(2)of the material where it occurs, and the phase matching between the pump and the down-converted photons.
Spontaneous parametric down-conversion (SPDC) is the most widely-used source of high-dimensional entangled two-photon states, and the entanglement in the spatial degree of freedom is considered best suited for harnessing high-dimensional advantages. Although the Schmidt basis provides a natural choice for state characterisation of entangled two-photon states in any degree of freedom, there is currently no technique that can measure the Schmidt basis of an entangled two-photon field. The existing techniques can only reconstruct the Schmidt spectrum when the Schmidt basis is known a priori. In contrast, we present a technique that measures the complete set of spatial Schmidt modes without any prior knowledge. Using this technique, we report measurement of states with over 3000 Schmidt modes -- highest reported yet -- with up to 98%\%% fidelity. We expect our work to significantly advance the harnessing of high-dimensional advantages in SPDC-based systems.
Quantum correlations, such as those existing between photons produced by spontaneous parametric down-conversion (SPDC), are ubiquitous in quantum photonic technologies. To develop applications, they must be precisely tailored and efficiently measured, which is often challenging in practice. This article presents an image encoding-decoding method based on the quantum correlations of photon pairs, highlighting recent advances in detecting and controlling these correlations for imaging and sensing applications.
Spontaneous parametric down-conversion in quantum optics is an invaluable resource for the realization of high-dimensional qudits with spatial modes of light. One of the main open challenges is how to directly generate a desirable qudit state in the SPDC process. This problem can be addressed through advanced computational learning methods; however, due to difficulties in modeling the SPDC process by a fully differentiable algorithm that takes into account all interaction effects, progress has been limited. Here, we overcome these limitations and introduce a physically-constrained and differentiable model, validated against experimental results for shaped pump beams and structured crystals, capable of learning every interaction parameter in the process. We avoid any restrictions induced by the stochastic nature of our physical model and integrate the dynamic equations governing the evolution under the SPDC Hamiltonian. We solve the inverse problem of designing a nonlinear quantum optical system that achieves the desired quantum state of down-converted photon pairs. The desired states are defined using either the second-order correlations between different spatial modes or by specifying the required density matrix. By learning nonlinear volume holograms as well as different pump shapes, we successfully show how to generate maximally entangled states. Furthermore, we simulate all-optical coherent control over the generated quantum state by actively changing the profile of the pump beam. Our work can be useful for applications such as novel designs of high-dimensional quantum key distribution and quantum information processing protocols. In addition, our method can be readily applied for controlling other degrees of freedom of light in the SPDC process, such as the spectral and temporal properties, and may even be used in condensed-matter systems having a similar interaction Hamiltonian.
Spontaneous parametric downconversion (SPDC) in quantum optics is an invaluable resource for the realization of high-dimensional qudits with spatial modes of light. One of the main open challenges is how to directly generate a desirable qudit state in the SPDC process. This problem can be addressed through advanced computational learning methods; however, due to difficulties in modeling the SPDC process by a fully differentiable algorithm, progress has been limited. Here, we overcome these limitations and introduce a physically constrained and differentiable model, validated against experimental results for shaped pump beams and structured crystals, capable of learning the relevant interaction parameters in the process. We avoid any restrictions induced by the stochastic nature of our physical model and integrate the dynamic equations governing the evolution under the SPDC Hamiltonian. We solve the inverse problem of designing a nonlinear quantum optical system that achieves the desired quantum state of downconverted photon pairs. The desired states are defined using either the second-order correlations between different spatial modes or by specifying the required density matrix. By learning nonlinear photonic crystal structures as well as different pump shapes, we successfully show how to generate maximally entangled states. Furthermore, we simulate all-optical coherent control over the generated quantum state by actively changing the profile of the pump beam. Our work can be useful for applications such as novel designs of high-dimensional quantum key distribution and quantum information processing protocols. In addition, our method can be readily applied for controlling other degrees of freedom of light in the SPDC process, such as spectral and temporal properties, and may even be used in condensed-matter systems having a similar interaction Hamiltonian.
The field of high-dimensional quantum photonics involves the use of multimode photonic degrees-of-freedom such as the spatial, temporal, or spectral structure of light to encode multi-level quantum states. Recent years have seen rapid progress in the development of methods to generate, manipulate, and distribute such quantum states of light and their use in a range of quantum technology applications that offer practical advantages over conventional qubit-based approaches. High-dimensional quantum states of light encoded in photonic time-bins, frequency-bins, transverse-spatial modes, waveguide paths, and temporal modes have enabled noise-robust fundamental tests of quantum mechanics, error-resilient and high-capacity quantum communication protocols, andas well as efficient approaches for quantum information processing, to name just a few examples. However, research in this field has progressed fairly independently, with little exchange across different photonic degrees-of-freedom or between experiment and theory and no comprehensive comparison between degrees-of-freedom. This roadmap aims to bridge this gap by surveying progress in each area and identifying shared challenges and opportunities that cut across two or more photonic degrees-of-freedoms. We review early work and state-of-the-art experimental techniques under development for high-dimensional quantum states encoded in single and entangled photons, as well as theoretical tools for their measurement and certification. We outline the main outstanding challenges for theory and each experimental degree-of-freedom, identifying promising future directions of research that may enable these to be overcome. We end by discussing interconnections and shared challenges centered around their distribution, measurement, and manipulation, with a view towards their integration into next-generation quantum technology platforms and applications.