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Frontiers in Optics

On Quantifying the Degree of Coherence in Qubits

Debabrata Goswami

Published Jan 1, 2025• 0 citations
Publisher

Abstract

We specifically define the amount of coherence that a specific state holds. We quantify the "quantum character" of qubits by considering their temporal evolution of the coherent character through off-diagonal density matrix elements.
DOI
10.1364/fio.2025.jv5a.3

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Being the key resource in quantum physics, the proper quantification of coherence is of utmost importance. Amid complex-looking functionals in quantifying coherence, we set forth a simple and easy-to-evaluate approach: principal diagonal difference of coherence (CPDD), which we prove to be non-negative, self-normalized, and monotonic (under any incoherent operation). In an attempt to extend CPDD in the domain of mixed states, we propose a simple, generic expression (applicable to other pure state coherence measures as well). To validate this theory, we consider a fictitious two-qubit system (both interacting and non-interacting) and, through the laser pulse–system interaction (semi-classical approach), compare the coherence evolution of CPDD with the relative entropy of coherence (Cr⋅e) and the l1-norm of coherence (Cl1), in both pure- and mixed-state regimes. The results from both the numerical and analytical (for a two-level system) studies clearly demonstrate a better sensitivity of CPDD in the close proximity of the maximally coherent states (MCS) than Cr⋅e or Cl1. To the best of our knowledge, CPDD is the only quantifier (among all existing coherence quantifiers) that is a linear function of density-matrix elements.
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The conditions under which quantum-classical Liouville dynamics may be reduced to a master equation are investigated. Systems that can be partitioned into a quantum-classical subsystem interacting with a classical bath are considered. Starting with an exact non-Markovian equation for the diagonal elements of the density matrix, an evolution equation for the subsystem density matrix is derived. One contribution to this equation contains the bath average of a memory kernel that accounts for all coherences in the system. It is shown to be a rapidly decaying function, motivating a Markovian approximation on this term in the evolution equation. The resulting subsystem density matrix equation is still non-Markovian due to the fact that bath degrees of freedom have been projected out of the dynamics. Provided the computation of nonequilibrium average values or correlation functions is considered, the non-Markovian character of this equation can be removed by lifting the equation into the full phase space of the system. This leads to a trajectory description of the dynamics where each fictitious trajectory accounts for decoherence due to the bath degrees of freedom. The results are illustrated by computations of the rate constant of a model nonadiabatic chemical reaction.