This thesis investigates the concentration of solar light for the generation of entangled photons. Previous studies have demonstrated that pumping a nonlinear crystal with coherent laser light can produce entangled photons via spontaneous parametric down-conversion (SPDC). The objective of this work is to explore the feasibility of generating entangled photons using solar light as the pump source. An experimental setup is developed that efficiently collects approximately 1000 W/m² of sunlight and couples it into an optical fiber to pump a nonlinear ppKTP crystal. Primary focusing is achieved using a Fresnel lens with dimensions of 1 m × 1.4 m, while a secondary concentrator guides the focused light into a multimode optical fiber with a core diameter of 1500 µm. The efficiency of the secondary concentrator is identified as a key factor determining the usable pump power. Several concentrator designs are investigated through optical simulations and experimental testing. Initial approaches employing cascaded compound parabolic concentrators and conical segments yield low coupling efficiencies. To overcome these limitations, optimized geometries including a solid glass droplet and a single polished conical concentrator made of fused silica are developed. Simulations predict total efficiencies of up to 66.9 % for high-index materials. Outdoor experiments under real sunlight demonstrate that coupling solar light into an optical fiber is feasible, with up to 62 mW successfully coupled. The results provide a foundation for future solar-driven quantum optical systems and related free-space applications.
This thesis investigates the concentration of solar light for the generation of entangled photons. Previous studies have demonstrated that pumping a nonlinear crystal with coherent laser light can produce entangled photons via spontaneous parametric down-conversion (SPDC). The objective of this work is to explore the feasibility of generating entangled photons using solar light as the pump source. An experimental setup is developed that efficiently collects approximately 1000 W/m² of sunlight and couples it into an optical fiber to pump a nonlinear ppKTP crystal. Primary focusing is achieved using a Fresnel lens with dimensions of 1 m × 1.4 m, while a secondary concentrator guides the focused light into a multimode optical fiber with a core diameter of 1500 µm. The efficiency of the secondary concentrator is identified as a key factor determining the usable pump power. Several concentrator designs are investigated through optical simulations and experimental testing. Initial approaches employing cascaded compound parabolic concentrators and conical segments yield low coupling efficiencies. To overcome these limitations, optimized geometries including a solid glass droplet and a single polished conical concentrator made of fused silica are developed. Simulations predict total efficiencies of up to 66.9 % for high-index materials. Outdoor experiments under real sunlight demonstrate that coupling solar light into an optical fiber is feasible, with up to 62 mW successfully coupled. The results provide a foundation for future solar-driven quantum optical systems and related free-space applications.
Spontaneous parametric down-conversion (SPDC) can produce entangled photons from a nonlinear medium driven by a pump beam, and has thus been a key resource in photonic quantum technologies. Historically, the low efficiency of SPDC prompted the use of lasers, which are high-intensity light sources, as pump sources. However, the practical implementation of laser-driven systems faces an imminent energy bottleneck. Lasers typically have suboptimal energy efficiencies due to lasing thresholds and the technical demands of thermal management. As a result, laser-pumped entangled photon sources suffer from significant power overhead, rendering quantum devices less sustainable. Over the past few decades, light-emitting diodes (LEDs) have emerged as inexpensive and energy-efficient alternatives for high-intensity light sources. Since 2010, studies have shown that LEDs can drive SPDC and generate photon pairs. These results suggests the potential to replace lasers with ubiquitous and natural light sources to build environmentally friendly quantum devices. However, replacing lasers with other light sources entails a lack of coherence in all degrees of freedom (DoFs) of the pump beam, including spatial, temporal-spectral, and polarization, which may influence the resulting entanglement generated from SPDC. While earlier studies established that pump coherence in a specific DoF sets an upper bound for entanglement in that same DoF, the cross-influence between different DoFs has not been fully investigated. In this thesis, we study the influence of the pump's spatiotemporal coherence on the polarization entanglement generated from SPDC. First, we experimentally demonstrate that polarization-entangled two-photon states can be generated from SPDC pumped by spatiotemporally incoherent light emitted from an LED. Although the resulting entanglement appears lower than that of laser-pumped SPDC, we theoretically show that spatiotemporal incoherence does not fundamentally constrain polarization entanglement; rather, the reduction arises from a coupling between spatiotemporal and polarization DoFs introduced by the experimental setup. We determined experimentally that this cross-influence acts as a deterministic mapping from the spatial components of the pump to the two-photon polarization state. Because this mapping depends on technical aspects of the setup, we envisioned that it could be either (i) engineered to structure entanglement in higher dimensions, or (ii) compensated to reduce spatial distinguishability. Building on the latter, we show that by placing the nonlinear medium in a phase-compensated interferometric setup, SPDC pumped by spatially incoherent light can produce high polarization entanglement that violates local realism, even without postselecting the SPDC field for a single spatial mode. Finally, as a proof-of-principle demonstration of a truly environmentally friendly quantum light source, we demonstrate the generation of polarization-entangled two-photon states from SPDC pumped by a natural source - sunlight.
This thesis deals with the production of entangled photons using spontaneous parametric down-conversion (SPDC). We start with a short overview of some important theoretical concepts. First we provide a brief reminder of the theory of entanglement. We then discuss how the state of quantum systems can be determined using quantum state tomography. We also explain SPDC, the physical process which we use to produce entangled photons. Finally, we give an overview of the methods which have been used to produce entangled photons in the past, both for two- and three-photon entanglement. \n \nThe first experiment is the design of an efficient source of entangled photon pairs based on a polarizing Sagnac interferometer configuration. With this configuration, we can use quasi-phasematched materials which allow for higher efficiencies than standard bulk nonlinear materials. The source is pumped by a low-power continuous-wave laser diode, and produces degenerate photon pairs at 809nm. It has a spectral brightness of 87,500 pairs/(s mW nm), and the fidelity of the produced quantum states with a Bell state is 98.9%. The source is used for experiments in quantum key distribution, cluster state quantum computing, remote state preparation, state discrimination, and entanglement-enhanced classical communication. \n \nThe second experiment discussed in this thesis is the generation of photon triplets using cascaded SPDC. In this experiment, a primary SPDC source is pumped with a low-power, continuous-wave laser diode, producing photon pairs. Single photons from these pairs serve as the pump for a second down-conversion, resulting in photon triplets. This is the first demonstration of the direct production of photon triplets, and the first observation of SPDC at the single photon level. This method could potentially be used to produce entangled photon triplets without post-selection, and as a source of triggered Bell pairs.
We present an ultrabright polarization-entangled photon source that is optimally coupled into single-mode fibers (SMFs). This study theoretically and experimentally examines the characteristics of spontaneous parametric down-conversion (SPDC) photons, including their spectrum, bandwidth, emission angle, and intensity, as functions of crystal length, temperature and beam waist condition. Notably, we measure the collinear spatial modes of photon-pairs and collection optics under various beam waist conditions and analyze them using a collinear Gaussian approximation model. By employing a simple mode-matching optical setup, we optimize the SMF coupling and heralding efficiencies of the photon-pairs. Consequently, we achieve a spectral brightness exceeding 2.0 MHz/mW/nm from a fiber-coupled entangled photon source, utilizing a 30-mm ppKTP crystal inside a polarization Sagnac interferometer. This represents the highest spectral brightness of SPDC photons generated using a CW laser pumped bulk crystal to date. Polarization entanglement was verified by a quantum state tomography and a polarization-correlation measurement. The fidelity of the entangled state is measured to be 97.8 % and the Bell-CHSH value S = 2.782 +- 0.04. The results obtained here provide practical insights for designing high-performance SPDC sources for satellite-based communication and long-distance optical links with extremely high-photon loss.
We present a simple but highly efficient source of polarization-entangled photons based on spontaneous parametric down-conversion (SPDC) in bulk periodically poled potassium titanyl phosphate crystals (PPKTP) pumped by a 405 nm laser diode. Utilizing one of the highest available nonlinear coefficients in a non-degenerate, collinear type-0 phase-matching configuration, we generate polarization entanglement via the crossed-crystal scheme and detect 0.64 million photon pair events/s/mW, while maintaining an overlap fidelity with the ideal Bell state of 0.98 at a pump power of 0.025 mW.
We present a simple but highly efficient source of polarization-entangled photons based on spontaneous parametric down-conversion (SPDC) in bulk periodically poled potassium titanyl phosphate crystals (PPKTP) pumped by a 405 nm laser diode. Utilizing one of the highest available nonlinear coefficients in a non-degenerate, collinear type-0 phase-matching configuration, we generate polarization entanglement via the crossed-crystal scheme and detect 0.64 million photon pair events/s/mW, while maintaining an overlap fidelity with the ideal Bell state of 0.98 at a pump power of 0.025 mW.
Both correlated-mode coupling efficiency and photon pair flux (brightness) of spontaneous parametric down-conversion (SPDC) coupled into single-mode fibers are key parameters for various quantum information science applications. We present an experimental investigation on the optimization of the correlated-mode coupling efficiency and the brightness of frequency-degenerated SPDC photon pairs into single-mode optical fibers. Using photon pairs generated from a type-I phase-matched bulk $\ensuremath{\beta}$-barium borate crystal pumped by a continuous-wave laser, we carefully evaluated both the correlated-mode coupling efficiency and the brightness of SPDC light coupled to a single-mode optical fiber, while continuously changing the focusing of the pump and collection modes, experimenting with Rayleigh lengths from 3 to 280 (for the pump) and 0.2 to 20 (for the collection) times the crystal length. The measured data suggest that the correlated-mode coupling efficiency can be close to unity for any pump focus, however, the optimal Rayleigh length of the collection mode depends on the pump focus parameter, and the brightness can be increased by tightening the pump focus, provided that the Rayleigh length of the collection mode is precisely adjusted. A maximal correlated-mode coupling efficiency of $99.0\ifmmode\pm\else\textpm\fi{}1.3%$ was experimentally achieved. These results will be useful for photonic quantum science and technology using SPDC sources with high heralding efficiencies.