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Journal of the Physical Society of Japan

Numerical Calculation of the Quantum Phase Transition due to the Dzyaloshinskii–Moriya Interaction in the Kagome Lattice Antiferromagnet Using the Linked-Cluster Expansion Method

Tomoki Kobayashi, Yoshiyuki Fukumoto

Published Jan 28, 2026• 0 citations
Publisher
DOI
10.7566/jpsj.95.025003

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We argue that the S=1/2S=1/2S=1/2 kagome antiferromagnet undergoes a quantum phase transition when the Dzyaloshinskii-Moriya coupling is increased. For D<DcD<{D}_{c}D<Dc​ the system is in a moment-free phase, and for D>DcD>{D}_{c}D>Dc​ the system develops antiferromagnetic long-range order. The quantum critical point is found to be ${D}_{c}\ensuremath{\simeq}0.1J$ using exact diagonalizations and finite-size scaling. This suggests that the kagome compound ZnCu3(OH)6Cl3{\text{ZnCu}}_{3}{(\text{OH})}_{6}{\text{Cl}}_{3}ZnCu3​(OH)6​Cl3​ may be in a quantum critical region controlled by this fixed point.
We investigate the zero-temperature phase diagram of the nearest-neighbor kagome antiferromagnet in the presence of Dzyaloshinksii-Moriya interaction. We develop a theory for the transition between Z2{Z}_{2}Z2​ spin liquids with bosonic spinons and a phase with antiferromagnetic long-range order. Connections to recent numerical studies and experiments are discussed.
Motivated by experimental results for the thermodynamic properties of the Rb 2 Cu 3 SnF 12 material and the discovery of its valence-bond solid ground state, we utilize the numerical linked-cluster expansions (NLCEs) and devise an expansion tailored to solve the Heisenberg model on a pinwheel-distorted kagome lattice. Using the exchange interactions that are relevant to Rb 2 Cu 3 SnF 12 , we calculate its uniform spin susceptibility and find a very good agreement with experiment. Next, we focus on the ground state of a simplified model of the distorted kagome lattice and take advantage of a zero-temperature Lanczos-based NLCE to study the approach to the ground state of the uniform kagome lattice Heisenberg model using a tuning parameter. Together with results from exact diagonalization of finite clusters, we find evidence that a phase transition occurs before the uniform limit is reached.