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Optics Letters

Hyperspectral imaging of downconverted photons in angle phase-matched nonlinear crystals

Evan J. Kumar, Lorenzo Uboldi, Cristian Manzoni, Giulio Cerullo, Ajay Ram Srimath Kandada

Published Jan 20, 2026• 2 citations
Publisher

Abstract

Spontaneous Parametric Down-Conversion (SPDC) is key to generating broadband spectrally entangled photons for quantum optical spectroscopy. Here we use a common-path birefringent interferometer to experimentally map the spatial-spectral distribution of SPDC in Type I and II β-barium borate crystals using hyperspectral k-space imaging. Under broadband pulsed pumping, we observe strong spatial variations in the spectra, with distinct features for each phase-matching type. Simulations based on biphoton amplitudes and phase-matching conditions qualitatively match our results. This spatial-spectral mapping enables control over biphoton entanglement entropy, paving the way for optimized quantum light sources for material spectroscopy.

DOI
10.1364/ol.587889

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Spontaneous Parametric Down-Conversion (SPDC) is key to generating broadband spectrally entangled photons for quantum optical spectroscopy. Here we use a common-path birefringent interferometer to experimentally map the spatial-spectral distribution of SPDC in Type I and II β-barium borate crystals using hyperspectral k-space imaging. Under broadband pulsed pumping, we observe strong spatial variations in the spectra, with distinct features for each phase-matching type. Simulations based on biphoton amplitudes and phase-matching conditions qualitatively match our results. This spatial-spectral mapping enables control over biphoton entanglement entropy, paving the way for optimized quantum light sources for material spectroscopy.
Spontaneous Parametric Down-Conversion (SPDC) is key to generating broadband spectrally entangled photons for quantum optical spectroscopy. Here we use a a common-path birefringent interferometer to experimentally map the spatial-spectral mode structure of SPDC in Type I and II β\betaβ-barium borate crystals using hyperspectral k-space imaging. Under broadband pulsed pumping, we observe strong spatial variations in the spectra, with distinct features for each phase-matching type. Simulations based on biphoton amplitudes and phase-matching conditions qualitatively match our results. This spatial-spectral mapping enables control over biphoton entanglement entropy, paving the way for optimized quantum light sources for material spectroscopy.
Spontaneous parametric down-conversion (SPDC) is one of the most widely used sources of polarization-entangled photon pairs, and understanding the generated biphoton state is essential for realizing high-brightness and high-purity entangled-photon sources. In particular, Type-II SPDC produces a biphoton wavefunction with a complex coupling between the spatial and polarization degrees of freedom owing to birefringence. In this study, we calculate the real-space distribution of the two-photon polarization state from the biphoton wavefunction of Type-II SPDC generated in a \b{eta}-barium borate (BBO) crystal. By identifying the spatial correlation direction between polarization and real-space coordinates, we designed aperture shapes that restrict the collection along this correlation direction. Through both numerical simulations and experiments, we demonstrate that such correlation-aligned apertures simultaneously achieve higher entanglement purity and improved photon collection efficiency. These results establish a practical design principle for optimizing aperture geometries based on the real-space biphoton wavefunction, providing a new approach to realizing high-purity and high-brightness SPDC entangled-photon sources.
Abstract Spontaneous parametric down-conversion (SPDC) is the most widely used process for generating photon pairs entangled in various degrees of freedom such as polarization, time-energy, position-transverse momentum, and angle-orbital angular momentum (OAM). In SPDC, a pump photon interacts with a non-linear optical crystal and splits into two entangled photons called the signal and the idler photons. The SPDC process has been studied extensively in the last few decades for various pump and crystal configurations, and the entangled photon pairs produced by SPDC have been used in numerous experimental studies on quantum entanglement and entanglement-based real-world quantum-information applications. In this tutorial article, we present a thorough study of phase matching in BBO crystals for spontaneous parametric down-conversion and thereby also investigate the generation of entangled photons in such crystals. First, we present a theoretical derivation of two-photon wavefunction produced by SPDC in the frequency and transverse momentum bases. We then discuss in detail the effects due to various crystal and pump parameters including the length of the crystal, the angle between the optic axis and the pump propagation direction, the pump incidence angle on the crystal surface, the refraction at the crystal surfaces, and the pump propagation direction inside the crystal. These effects are extremely relevant in experimental situations. We then present our numerical and experimental results in order to illustrate how various experimental parameters affect the phase matching and thus the generation of entangled photons. Finally, using the two-photon wavefunction in the transverse wave-vector basis, we show how to derive the two-photon wavefunction in the OAM basis and thereby calculate the two-photon angular Schmidt spectrum. We expect this article to be useful for researchers working in various capacities with entangled photons generated by SPDC in BBO crystals.
We demonstrate a broadband entangled photon source based on a single-pass, type-0 phase-matched, non-collinear spontaneous parametric down-conversion (SPDC) process. By spatially multiplexing the intrinsically random transverse momentum states of biphotons emitted in an annular spatial distribution from a single-frequency-pumped, 2-mm-long periodically poled KTP crystal, we generate polarization-entangled pair photons with a spectral bandwidth of ∼130 nm centered at 810 nm. The negligible group-velocity mismatch of the co-polarized near-degenerate photons in single-pass and low birefringence of standard optical components preserves indistinguishability across the broadband emission without phase compensation, enabling high-quality polarization entanglement over the entire emission bandwidth. The source achieves a brightness of 0.57 Mpairs/s/mW and a two-photon coherence length of 6.97 μm, while exhibiting an interference visibility exceeding 95%, a Bell–CHSH parameter of 2.526 ± 0.005 that remains stable over 12 h of continuous operation and violates the Bell inequality by more than 100 standard deviations, and a state fidelity of 96.3%. The generic scheme providing the broadest bandwidth entangled biphotons at 810 nm, to our knowledge, can readily be used for other wavelengths as required for multiparty quantum networks and quantum sensing applications.
Here we investigate the all-optical control of spectral correlations in spontaneous parametric down-conversion. We show that when photon pairs are projected onto high-order spatial modes, the spatial structure of the pump field defines the phase-matching function of the nonlinear interaction. Thus, by structuring the pump field in both space and spectrum, the biphoton spectral correlations are fully controlled. Considering a standard periodically-poled crystal as the nonlinear medium, we show that the Gouy phase matching method proposed here can generate both spectrally uncorrelated and high-dimensional spectrally entangled photon pairs, similarly to what is achieved with aperiodically-poled crystals. Furthermore, we show that our method can generate a wider class of quantum states if the pump field is a spatiotemporal wavepacket, that is, if its spatial and spectral structures are correlated.