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Elsevier eBooks

Single solid-state quantum emitters and optical tweezers

Pablo Camarero, Ana Dávila, Esther Rincón, Fengchan Zhang, Elisa Ortiz‐Rivero, Patricia Haro‐González

Published Jan 1, 2026• 0 citations
Publisher
DOI
10.1016/b978-0-323-88660-4.00001-6

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Single-photon emitters based on individual atoms or individual atomic-like defects are highly sought-after components for future quantum technologies. A key challenge in this field is how to isolate just one such emitter; the best approaches still have an active emitter yield of only 50% so that deterministic integration of single active emitters is not yet possible. Here, we demonstrate the ability to isolate individual erbium emitters embedded in 20 nm nanocrystals of NaYF 4 using plasmonic aperture optical tweezers. The optical tweezers capture the nanocrystal, whereas the plasmonic aperture enhances the emission of the Er and allows the measurement of discrete emission rate values corresponding to different numbers of erbium ions. Three separate synthesis runs show near-Poissonian distribution in the discrete levels of emission yield that correspond to the expected ion concentrations, indicating that the yield of active emitters is approximately 80%. Fortunately, the trap allows for selecting the nanocrystals with only a single emitter, and so this gives a route to isolating and integrating single emitters in a deterministic way. This demonstration is a promising step toward single-photon quantum information technologies that utilize single ions in a solid-state medium, particularly because Er emits in the low-loss fiber-optic 1550 nm telecom band.
Quantum technologies require sources of single photons, which can be created by isolating individual atoms or ions. Erbium ions are a promising choice for single photon sources as it emits photons at low-loss fiber optic wavelengths. However, erbium has a low emission rate and it is challenging to isolate single emitters reliably. Here, we isolate singly Er3+-doped nanocrystals using optical tweezers in a gold double nanohole aperture. The double nanohole geometry enhances the emission rate from the nanocrystals. With this additional enhancement we observe emission at 1550 nm. Discrete levels of emission from dilutely Er3+-doped nanocrystals are observed—corresponding to the number of active erbium emitters present. Nanocrystals with single active emitters were identified and isolated with this technique, demonstrating a path towards single emitter sources at 1550 nm.
Single photon sources are desired for quantum computing and communication applications. Ideally, these sources would provide single photons on demand at the low-loss fiber optical communication wavelength of 1550 nm. Single Erbium ions provide a good candidate for such sources because they emit at the right wavelength and they are very stable, however, the challenges remain of isolating a single emitter, coupling its emission to optical fiber and enhancing its emission rate. Nanoaperture optical tweezers provide a pathway to solving these issues by trapping and identifying single emitters, enhancing their emission rate and providing efficient coupling to an optical fiber. Recently, we have made progress in each of these areas (trapping, enhancing and coupling), which will be reviewed in this talk.