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Light Science & Applications

Non-Hermitian quantum walks uncover dynamical quantum phase transitions under self-normal and biorthogonal bases

Guangzhen Li, Luqi Yuan

Published Jan 4, 2026• 2 citations
Publisher

Abstract

The differences in critical times and critical momenta between self-normal and biorthogonal dynamical quantum phase transitions are revealed. The theoretical analysis is experimentally validated through multiple quench processes using a one-dimensional discrete-time non-Hermitian quantum walks.
DOI
10.1038/s41377-025-02069-5

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Dynamical quantum phase transitions (DQPTs), characterized by non-analytic behavior in rate function and abrupt changes in dynamic topological order parameters (DTOPs) over time, have garnered enormous attention in recent decades. However, in non-Hermitian systems, the special biorthogonality of the bases makes the definition of DQPTs complex. In this work, we delve into the comprehensive investigation of self-normal DQPTs (originally used in Hermitian systems) to compare them with their biorthogonal counterpart, within the context of non-Hermitian quantum walks (QWs). We present a detailed analysis of the behaviors of Loschmidt rate functions and DTOPs under these two distinct theoretical approaches. While both self-normal and biorthogonal methods can be used to detect DQPTs in quench dynamics between different topological phases, we theoretically present their differences in the definition of critical momenta and critical times by analyzing the Fisher zeros and fixed points. Finally, we present an experiment that observes both types of DQPTs using one-dimensional discrete-time QWs with single photons.
Non-Hermitian dynamical quantum phase transitions (DQPTs) are intrinsically sensitive to the choice of inner product under nonunitary time evolution. Although the biorthogonal formulation based on associated states provides a normalized Loschmidt echo with a probabilistic interpretation, previous studies have found biorthogonal and self-normal DQPTs to occur in the same parameter regimes, suggesting that the two forms of dynamical criticality are concomitant. Here we demonstrate that this is not the case. In an exactly solvable periodically driven non-Hermitian Su-Schrieffer-Heeger chain, we uncover a finite biorthogonal-only Floquet DQPT regime, where the biorthogonal Loschmidt rate becomes nonanalytic while the self-normal Loschmidt rate remains smooth. The critical conditions are obtained analytically, showing that the onset of biorthogonal Floquet DQPTs is locked to the exceptional lines of the effective Floquet Hamiltonian, whereas self-normal criticality has no corresponding spectral boundary. Moreover, for each critical momentum, the biorthogonal DQPT exhibits a pair of critical times within every driving period, whereas the self-normal DQPT exhibits only one. Our results establish a fundamental distinction between biorthogonal and self-normal DQPTs, thereby opening a route toward new nonequilibrium quantum phenomena in non-Hermitian systems.
Dynamical quantum phase transitions in non-Hermitian systems pose fundamental challenges due to the intrinsic biorthogonality of their eigenstates. In this work, we extend a biorthogonal framework to investigate dynamical quantum phase transitions in non-Hermitian topological superconductors. Taking the non-Hermitian Kitaev chain as a prototypical model, we construct an associated-state formalism and reformulate the Loschmidt rate function, dynamical topological order parameter, and dynamical Fisher zeros. Within this framework, we find that the critical times at which dynamical quantum phase transitions occur differ from those based on the conventional self-normal approaches. We further analyze momentum-resolved subsystems at critical momenta and demonstrate the robustness of the biorthogonal framework. Our work highlights the essential role of biorthogonality in nonequilibrium dynamics and establishes a consistent theoretical framework for dynamical quantum phase transitions in non-Hermitian topological superconductors.
We establish a unified framework for dynamical quantum phase transitions (DQPTs) in non-Hermitian systems that encompasses both biorthogonal and self-norm nonbiorthogonal formulations for pure and mixed states under quantum quench protocols. Our framework provides explicit expressions for the Loschmidt amplitude, Loschmidt echo, and rate function, revealing a universal geometric signature of DQPTs in the two-band model: orthogonality of two related vectors in two-dimensional real space. Strikingly, we demonstrate that nonbiorthogonal quenches from non-Hermitian to Hermitian Hamiltonians under chiral symmetry exhibit emergent topological characteristics of DQPTs, unveiling their fundamental features beyond conventional Hermitian regimes. This work establishes fundamental geometric and topological principles governing quantum criticality in open systems, with implications for quantum sensing and many-body physics in dissipative environments.
By utilizing biorthogonal bases, we develop a comprehensive framework for studying biorthogonal dynamical quantum phase transitions in non-Hermitian systems. With the help of the previously overlooked associated state, we define the automatically normalized biorthogonal Loschmidt echo. This approach is capable of handling arbitrary non-Hermitian systems with complex eigenvalues and naturally eliminates the negative value of Loschmidt rate obtained without the biorthogonal bases. Taking the non-Hermitian Su-Schrieffer-Heeger model as a concrete example, a 1/2 change of dynamical topological order parameter in biorthogonal bases is observed which is not shown in self-normal bases. Furthermore, we discover that the periodicity of biorthogonal dynamical quantum phase transitions depends on whether the two-level subsystem at the critical momentum oscillates or reaches a steady state.
Fisher zero lines of the Loschmidt amplitude in non-Hermitian quenches can exhibit anomalous structures in the complex time plane, such as divergence, separation, and the restriction of all branches or a specific branch to the real or imaginary axis. Here, we use the biorthogonal framework to reveal the origin of these structures and determine the corresponding critical momentum conditions by analyzing the values of mk=h^0⋅h^1m_k=\hat{\mathbf{h}}_0\cdot\hat{\mathbf{h}}_1mk​=h^0​⋅h^1​, the dot product between the normalized prequench and postquench complex Bloch vectors. When Fisher zeros continuously cover the real-time axis, the density of Fisher zeros is further introduced to identify the critical times within these critical regions, at which the rate function becomes nonanalytic. We verify our results in a generalized non-Hermitian SSH model by quenching the Peierls phase and the non-Hermitian gain-loss strength, and also use the Jordan form to analyze the dynamics at postquench exceptional points, where the conventional Fisher zero formula is not applicable.