This thesis details the complete upgrade and renovation of an existing experimental platform into a high-resolution quantum gas microscope for ultracold 87Rb atoms. Quantum gas microscopes enable site-resolved imaging, providing unprecedented access to quantum statistical effects and many-body phenomena. While such instruments are often employed to study physics in optical lattices, we have innovatively adapted our apparatus to investigate bulk system behavior. A major part of this project involved upgrading the scientific apparatus and retrofitting the previous system. We introduced new optical components, including a high-NA objective, and improved the vacuum system for better optical access. Extensive lab renovations, from upgrading the optical table to reorganizing the laser and imaging setups, were carried out to enhance mechanical and thermal stability. Rigorous optical benchmarking confirmed that the objective achieves diffractionlimited imaging, which is critical for resolving single atoms. This capability allowed us to detect density fluctuations at the scale of the thermal de Broglie wavelength in a quasi-two-dimensional gas of 87Rb atoms. In an experiment resembling Hanbury Brown and Twiss interferometry, we measured a 30% enhancement in the second-order correlation function in situ, demonstrating strong bosonic bunching. This outcome underscores the microscope’s precision and the importance of high-resolution imaging in capturing subtle quantum statistical effects. The successful realization of this apparatus demonstrates the utility of quantum gas microscopes in probing bulk systems. With this new platform in place, future studies can explore critical phenomena, many-body correlations, matter-wave emission, and quantum simulations with cold atoms.
This thesis details the complete upgrade and renovation of an existing experimental platform into a high-resolution quantum gas microscope for ultracold 87Rb atoms. Quantum gas microscopes enable site-resolved imaging, providing unprecedented access to quantum statistical effects and many-body phenomena. While such instruments are often employed to study physics in optical lattices, we have innovatively adapted our apparatus to investigate bulk system behavior. A major part of this project involved upgrading the scientific apparatus and retrofitting the previous system. We introduced new optical components, including a high-NA objective, and improved the vacuum system for better optical access. Extensive lab renovations, from upgrading the optical table to reorganizing the laser and imaging setups, were carried out to enhance mechanical and thermal stability. Rigorous optical benchmarking confirmed that the objective achieves diffractionlimited imaging, which is critical for resolving single atoms. This capability allowed us to detect density fluctuations at the scale of the thermal de Broglie wavelength in a quasi-two-dimensional gas of 87Rb atoms. In an experiment resembling Hanbury Brown and Twiss interferometry, we measured a 30% enhancement in the second-order correlation function in situ, demonstrating strong bosonic bunching. This outcome underscores the microscope’s precision and the importance of high-resolution imaging in capturing subtle quantum statistical effects. The successful realization of this apparatus demonstrates the utility of quantum gas microscopes in probing bulk systems. With this new platform in place, future studies can explore critical phenomena, many-body correlations, matter-wave emission, and quantum simulations with cold atoms.
Imagine a new generation of computers that dramatically surpasses the most powerful supercomputers, being able to tackle the most challenging of computational problems. These problems arise, for example, in quantum physics where the computational power required to model a many-particle system increases exponentially with the number of its constituents, and as a consequence the calculations become prohibitively time-consuming. Nobel laureate Richard Feynman proposed this new type of computer in the early 1980s: ‘Let the computer itself be built of quantum mechanical elements which obey quantum mechanical laws.’ Such a quantum simulator would allow researchers to tackle challenging problems in condensed-matter physics. In particular many-body fermionic quantum systems are very difficult to compute due to the antisymmetric nature of the wave function, and the resulting sign problem for quantum Monte Carlo methods. This is why a quantum simulator will be an excellent test bed to investigate phenomena and properties of strongly correlated fermionic quantum systems. A powerful experimental platform to realize a quantum simulator is laser-cooled atoms [1] held in an artificial crystal of light, generated by superimposing laser beams. The atoms are kept in this optical lattice similar to marbles in the hollows of an egg carton, and they can mimic the behaviour of electrons in a real crystal. These systems interface atomic physics with condensed matter physics in a new way, as the tools of atomic physics allow for exquisite control of many experimental parameters, which are often inaccessible in solid state experiments. In-situ imaging techniques [2] using ‘quantum-gas microscopes’ constitute a new approach to the study of many-body quantum systems in an optical lattice with unprecedented resolution at the single-particle and single-site level [3,4]. This new method is complementary to earlier optical lattice experiments measuring distributions in momentum space after a time-of-flight expansion. A quantum-gas microscope uses an optical imaging system (Fig. 1a) for collecting the fluorescence light of ultracold atoms in an optical lattice with high spatial resolution comparable to the lattice spacing of ≈ 500 nm. (a) Atoms in optical lattice atoms are imaged with a high-resolution microscope objective [4]. (b) Single-site addressing is achieved by focussing a laser beam through the microscope onto selected atoms, bringing them into resonance with microwave radiation which produces spin flips [12]. (c) and (d) Single-atom-resolved fluorescence images of bosonic Mottinsulators [4,9]. (e) Deterministically prepared atom distribution using single-site addressing [12]. (f) Direct observation of single-atom quantum walks [15]. Fluorescence imaging of atoms in a quantum-gas microscope has made it possible to directly observe bosonic Mott insulators with single-atom resolution [4–6], giving access to in-situ measurements of temperature and entropy distributions. Subsequently, ground-breaking experiments in many-body quantum dynamics have been performed, such as the first direct observation of correlation spreading after quenches of the system to lower lattice depths [7]. Other experiments include the quantum simulation of an antiferromagnetic spin-1/2 chain [8], the realization of algorithmic cooling [9], the direct measurement of correlations across the superfluid-to-Mott-insulator transition [10], or the observation of the ‘Higgs’ amplitude mode [11]. The high-resolution imaging system is also capable of optically addressing individual atoms with sub-diffraction-limited resolution. For this purpose, a laser beam is focussed though the microscope objective onto selected lattice sites, bringing the atoms into resonance with microwave radiation which produces spin flips [12,13]. The preparation of arbitrary atom distributions in the lattice not only opens perspectives for neutral-atom quantum information processing, but also allows the deterministic creation of specific out-of-equilibrium situations, and their ensuing system dynamics can be studied with single-atom resolution. Examples include the creation of spin impurities and the study of their dynamics in a many-body system [14], the observation of quantum walks [15] and magnon-bound states [16], and the measurement of entanglement entropy [17]. The technique used for single-site-resolved detection of individual atoms in the optical lattice is fluorescence imaging. It requires laser cooling of the atoms to sub-Doppler temperatures while detecting the fluorescence photons emitted during this process. A challenge is to achieve a low particle loss rate and to prevent the atoms from hopping between lattice sites. In the case of the first quantum-gas microscopes, this has been implemented with bosonic rubidium-87 atoms, and also recently for ytterbium-174. However, it has proven more challenging for fermionic alkaline species such as potassium-40 and lithium-6, as their low mass and small excited state hyperfine splitting-prevented standard sub-Doppler cooling from working. As a result, it took several years to extend the quantum-gas microscope technique to fermionic species, and in 2015 several groups have demonstrated single-atom-resolved imaging of fermions [18]. In these setups, the direct observation of band insulators [19], fermionic Mott insulators [20,21] and even antiferromagnetic correlations [22] has been reported most recently. These developments provide fascinating opportunities to study many-body fermionic quantum systems with single-particle access. The fermionic nature of the electron is vital to understanding a range of phenomena within solid-state physics, such as electron pairing in superconductivity, and quantum magnetism. In this context, the quantum simulator will allow, e.g. for direct measurement of ordered quantum phases and out-of-equilibrium dynamics, with access to quantities such as spin--spin correlation functions and the growth of many-body entanglement. The high-resolution imaging systems could also be used to project tailored time-varying light fields onto the atoms, allowing the removal of high-entropy regions by locally modifying the confining potential to attain very low-entropy states. Attaining these low-entropy many-particle states is one of the key challenges in our field. In summary, quantum-gas microscopes offer unprecedented access to many-body quantum systems, and they will allow us to gain an even deeper insight into the intriguing world of quantum physics that governs the properties of strongly correlated materials. Using a well-controlled quantum system to simulate other quantum systems could help resolve some of the most challenging problems scientists face in condensed matter physics and materials science, but it will also provide new insights in quantum chemistry, high-energy physics and biology. SK acknowledges funding from the EU (ERC FERMILATT, SIQS, QuProCs) and SUPA.
Atom-based quantum simulators offer a unique platform that enables the imaging of each particle in a many-body system. Until now, however, this capability has been limited to quantum systems in discretized space such as optical lattices and tweezers, where spatial degrees of freedom are quantized. Here, we introduce a novel method for imaging atomic quantum many-body systems in the continuum, allowing for in situ resolution of every particle. We demonstrate the capabilities of our approach on a two-dimensional atomic Fermi gas. We probe the density correlation functions, resolving their full spatial functional form, and reveal the shape of the Fermi hole arising from Pauli exclusion as a function of temperature. Our method opens the door to probing strongly correlated quantum gases in the continuum with unprecedented spatial resolution, providing in situ access to spatially resolved correlation functions of arbitrarily high order across the entire system.
In this thesis, I present experiments on making and probing strongly correlated gases of ultracold atoms in an optical lattice with engineered potentials and dynamics. The quantum gas microscope first developed in our lab enables single-site resolution imaging and manipulation of atoms in a two-dimensional lattice, offering an ideal platform for quantum simulation of condensed matter systems. Here we demonstrate our abilities to generate optical potential with high precision and high resolution, and engineer coherent dynamics using photon assisted tunneling. We also create a system of bilayer quantum gases that brings new imaging capabilities and extends the possible range of our quantum simulation.
We report the first direct in situ observation of density fluctuations on the scale of the thermal de Broglie wavelength in an ultracold gas of bosons. Bunching of ^{87}Rb atoms in a quasi-two-dimensional system is observed by single-atom imaging using a quantum gas microscope. Compared to a classical ensemble, we observe a 30% enhancement of the second-order correlation function. We show the spatial and thermal dependence of these correlations. The reported method of detecting in situ correlations can be applied to interacting many-body systems and to the study of critical phenomena near phase transitions.
Cold atom experiments have traditionally employed bulk imaging techniques, such as absorption imaging, to measure atomic sample densities. However, in recent years, single-atom imaging methods have emerged as powerful tools to probe and manipulate quantum many-body systems at the level of individual particles. This work focuses specifically on quantum gas microscopy using Raman sideband cooling in an optical lattice. This technique, which has been used extensively in several cold atoms groups, has mostly been applied in the context of discrete systems, such as the celebrated Bose- and Fermi-Hubbard models and their generalization. In this thesis, we show how quantum gas microscopy can be extended beyond its original scope to probe continuous many-body systems in a quantitative manner. Our proposed protocol consists in a rapid ramp of the pinning lattice intensity, projecting atoms from the continuum onto discrete lattice sites, followed by a Raman sideband cooling stage that confines atoms near the motional ground state and prevents them from escaping during imaging. To validate the effectiveness of this new method, we characterize the pinning and imaging processes by using continuous quantum gas microscopy to reconstruct the wavefunction of a single-atom Gaussian wave packet during its free expansion. Under optimal conditions, we achieve an imaging fidelity in excess of 95%, defined as the probability of projecting an atom from the continuum to the nearest lattice site and successfully imaging it. We also apply this technique to a quasi-two-dimensional non-interacting Fermi gas, enabling us to extract two- and three-body correlation functions, g2 and g3, with unprecedented spatial resolution and finding an excellent agreement with the theoretical prediction. In particular, our measurements reveal a 90% reduction in the probability of finding two atoms in close proximity for the coldest samples, offering one of the most pristine in situ observations of the Pauli exclusion principle in a continuous system. Finally, we propose a thermometry method based on atom number fluctuations, which are readily obtained from our imaging procedure. Crucially, this thermometry technique could be generalized to strongly interacting systems, where temperature estimation is typically challenging. The quantum gas microscopy technique developed here opens new avenues for studying continuous many-body systems with unprecedented resolution, offering a powerful tool for future cold atom experiments.
Abstract Imaging is central to gaining microscopic insight into physical systems, and new microscopy methods have always led to the discovery of new phenomena and a deeper understanding of them. Ultracold atoms in optical lattices provide a quantum simulation platform, featuring a variety of advanced detection tools including direct optical imaging while pinning the atoms in the lattice1,2. However, this approach suffers from the diffraction limit, high optical density and small depth of focus, limiting it to two-dimensional (2D) systems. Here we introduce an imaging approach where matter wave optics magnifies the density distribution before optical imaging, allowing 2D sub-lattice-spacing resolution in three-dimensional (3D) systems. By combining the site-resolved imaging with magnetic resonance techniques for local addressing of individual lattice sites, we demonstrate full accessibility to 2D local information and manipulation in 3D systems. We employ the high-resolution images for precision thermodynamics of Bose–Einstein condensates in optical lattices as well as studies of thermalization dynamics driven by thermal hopping. The sub-lattice resolution is demonstrated via quench dynamics within the lattice sites. The method opens the path for spatially resolved studies of new quantum many-body regimes, including exotic lattice geometries or sub-wavelength lattices3–6, and paves the way for single-atom-resolved imaging of atomic species, where efficient laser cooling or deep optical traps are not available, but which substantially enrich the toolbox of quantum simulation of many-body systems.