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Roadmap on atomically-engineered quantum platforms

Phark, Soo-hyon, Bent Weber, Yoshida, Yasuo, Forrester, Patrick R., R. J. G. Elbertse, Stroscio, Joseph A., Wang, Hao, Yang, Kai, Gross, Leo, Mishra, Shantanu, Paschke, Fabian, Katharina Kaiser, Fatayer, Shadi, Repp, Jascha, Harry L. Anderson, Diego Peña, Albrecht, Florian, Giessibl, Franz J., Fasel, Roman, Fernández-Rossier, Joaquín, Kawai, Shigeki, L. Limot, Nicolás Lorente, Berthold Jäck, Huang, Haonan, Joachim Ankerhold, Christian R. Ast, Trahms, Martina, Clemens B. Winkelmann, Franke, Katharina J., Soldini, Martina O., Glenn Wagner, Titus Neupert, Küster, Felix, Das, Souvik, S. Parkin, Sessi, Paolo, Wang, Zhenyu, Vidya Madhavan, Huber, Rupert, Singh, Gagandeep, Donati, Fabio, Rusponi, Stefano, Brune, Harald, Eufemio Moreno Pineda, Mario Ruben, Wolfgang Wernsdorfer, Huang, Wantong, Au-Yeung, Kwan Ho, Philip Willke, Heinrich, Andreas J., Baumann, Susanne, Sebastian Loth, Lukas M. Veldman, Alexander F. Otte, Wolf, Christoph, Joris Gerhard Keizer, Michelle Yvonne Simmons

Published Sep 1, 2025• 0 citations
Publisher

Abstract

Matter at the atomic-scale is inherently governed by the laws of quantum mechanics. This makes charges and spins confined to individual atoms—and interactions among them—an invaluable resource for fundamental research and quantum technologies alike. However, harnessing the inherent ‘quantumness’ of atomic-scale objects requires that they can be precisely engineered and addressed at the individual atomic level. Since its invention in the 1980s, scanning tunnelling microscopy (STM) has repeatedly demonstrated the unrivalled ability to not only resolve but manipulate matter at atomic length scales. Over the past decades, this has enabled the design and investigation of bottom-up tailored nanostructures as reliable and reproducible platforms to study designer quantum physics and chemistry, band topology, and collective phenomena. The vast range of STM-based techniques and modes of operation, as well as their combination with electromagnetic fields from the infrared to microwave spectral range, has even allowed for the precise control of individual charge and spin degrees of freedom. This roadmap reviews the most recent developments in the field of atomically-engineered quantum platforms and explores their potential in future fundamental research and quantum technologies.

DOI
10.3929/ethz-c-000786536

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Matter at the atomic-scale is inherently governed by the laws of quantum mechanics. This makes charges and spins confined to individual atoms—and interactions among them—an invaluable resource for fundamental research and quantum technologies alike. However, harnessing the inherent ‘quantumness’ of atomic-scale objects requires that they can be precisely engineered and addressed at the individual atomic level. Since its invention in the 1980s, scanning tunnelling microscopy (STM) has repeatedly demonstrated the unrivalled ability to not only resolve but manipulate matter at atomic length scales. Over the past decades, this has enabled the design and investigation of bottom-up tailored nanostructures as reliable and reproducible platforms to study designer quantum physics and chemistry, band topology, and collective phenomena. The vast range of STM-based techniques and modes of operation, as well as their combination with electromagnetic fields from the infrared to microwave spectral range, has even allowed for the precise control of individual charge and spin degrees of freedom. This roadmap reviews the most recent developments in the field of atomically-engineered quantum platforms and explores their potential in future fundamental research and quantum technologies.
Matter at the atomic-scale is inherently governed by the laws of quantum mechanics. This makes charges and spins confined to individual atoms—and interactions among them—an invaluable resource for fundamental research and quantum technologies alike. However, harnessing the inherent ‘quantumness’ of atomic-scale objects requires that they can be precisely engineered and addressed at the individual atomic level. Since its invention in the 1980s, scanning tunnelling microscopy (STM) has repeatedly demonstrated the unrivalled ability to not only resolve but manipulate matter at atomic length scales. Over the past decades, this has enabled the design and investigation of bottom-up tailored nanostructures as reliable and reproducible platforms to study designer quantum physics and chemistry, band topology, and collective phenomena. The vast range of STM-based techniques and modes of operation, as well as their combination with electromagnetic fields from the infrared to microwave spectral range, has even allowed for the precise control of individual charge and spin degrees of freedom. This roadmap reviews the most recent developments in the field of atomically-engineered quantum platforms and explores their potential in future fundamental research and quantum technologies.
Matter at the atomic-scale is inherently governed by the laws of quantum mechanics. This makes charges and spins confined to individual atoms—and interactions among them—an invaluable resource for fundamental research and quantum technologies alike. However, harnessing the inherent ‘quantumness’ of atomic-scale objects requires that they can be precisely engineered and addressed at the individual atomic level. Since its invention in the 1980s, scanning tunnelling microscopy (STM) has repeatedly demonstrated the unrivalled ability to not only resolve but manipulate matter at atomic length scales. Over the past decades, this has enabled the design and investigation of bottom-up tailored nanostructures as reliable and reproducible platforms to study designer quantum physics and chemistry, band topology, and collective phenomena. The vast range of STM-based techniques and modes of operation, as well as their combination with electromagnetic fields from the infrared to microwave spectral range, has even allowed for the precise control of individual charge and spin degrees of freedom. This roadmap reviews the most recent developments in the field of atomically-engineered quantum platforms and explores their potential in future fundamental research and quantum technologies.
Quantum phenomena are typically observable at length and time scales smaller than those of our everyday experience, often involving individual particles or excitations. The past few decades have seen a revolution in the ability to structure matter at the nanoscale, and experiments at the single particle level have become commonplace. This has opened wide new avenues for exploring and harnessing quantum mechanical effects in condensed matter. These quantum phenomena, in turn, have the potential to revolutionize the way we communicate, compute and probe the nanoscale world. Here, we review developments in key areas of quantum research in light of the nanotechnologies that enable them, with a view to what the future holds. Materials and devices with nanoscale features are used for quantum metrology and sensing, as building blocks for quantum computing, and as sources and detectors for quantum communication. They enable explorations of quantum behaviour and unconventional states in nano- and opto-mechanical systems, low-dimensional systems, molecular devices, nano-plasmonics, quantum electrodynamics, scanning tunnelling microscopy, and more. This rapidly expanding intersection of nanotechnology and quantum science/technology is mutually beneficial to both fields, laying claim to some of the most exciting scientific leaps of the last decade, with more on the horizon.
Since the invention of the scanning tunnelling microscope (STM) in the early 1980s atomic level microscopy has taken on a new dimension. The STM and the atomic force microscope (AFM) have become key instruments in the study of phenomena in the smallest dimensions ranging from magnetism in ultra-thin films, through the understanding of how atoms and molecules organise themselves, to insights into the propagation of electron waves. A good understanding of these issues will facilitate the manufacture of components or devices that are a few atomic dimensions in size and this will have far-reaching implications in fields ranging from medicine through to consumer electronics. As early as the 1970s, the scientific community was discussing the possibility of embedding a few molecules, or even a single molecule, between electrodes to perform the basic switching function. This is now possible in the case of individual components but key challenges lie with the economic commercial fabrication of whole devices. A key challenge lies in determining whether such quantum computers will work and how quantum effects can be used to perform variety of previously unsuspected and potentially useful schemes of information processing.
Electron spin resonance in scanning tunneling microscopy enabled the study of electronic transitions of magnetic impurities on surfaces at the atomic scale. This ESR-STM technique allows to spectroscopically probe and coherently manipulate spins using an all-electrical method without oscillating external magnetic driving fields. Here, we aim to review recent advancements in ESR-STM. We will discuss possible fundamental mechanisms by which the electric field drives spin resonance based on Heisenberg exchange, Kondo scattering, and Anderson impurity models. We validate theoretical predictions against experimental observations, to understand how electronic correlations, spin exchange, and many-body effects manifest in ESR-STM signals. After reviewing coherent spin control in the STM junction, we discuss potential applications of the ESR-STM method for coherent multi-spin control which enables multiple-qubit operations. Finally, we address recent developments in coupled electron-nuclear spin systems, including hyperfine-resolved ESR spectroscopy, and the driving and polarization of nuclear spins in ESR-STM.
Achieving time-domain control of quantum states with atomic-scale spatial resolution in nanostructures is a long-term goal in quantum nanoscience and spintronics. Here, we demonstrate coherent spin rotations of individual atoms on a surface at the nanosecond time scale, using an all-electric scheme in a scanning tunneling microscope (STM). By modulating the atomically confined magnetic interaction between the STM tip and surface atoms, we drive quantum Rabi oscillations between spin-up and spin-down states in as little as ~20 nanoseconds. Ramsey fringes and spin echo signals allow us to understand and improve quantum coherence. We further demonstrate coherent operations on engineered atomic dimers. The coherent control of spins arranged with atomic precision provides a solid-state platform for quantum-state engineering and simulation of many-body systems.