The evolution of a closed quantum system is described by a unitary operator generated by a Hermitian Hamiltonian. However, when certain degrees of freedom are coupled to an environment, the relevant dynamics can be captured by non-unitary evolution operators, arising from non-Hermitian Hamiltonians. Here we introduce a photonic platform that implements non-unitary quantum walks, commonly used to emulate open-system dynamics, in the synthetic space of light transverse momentum. These walks are realized by propagating light through a series of dichroic liquid-crystal metasurfaces that impart polarization-dependent momentum shifts. The non-unitary behavior stems from dichroic dye molecules with polarization-dependent absorption, whose orientation is coupled to that of the liquid crystals. We demonstrate multiple walks up to five time steps, with adjustable levels of dichroism set by the metasurface voltage, which is controlled remotely. This discrete-time process maps onto two-band tight-binding models with reciprocal yet non-Hermitian nearest-neighbor couplings, corresponding to a less-studied class of non-Hermitian systems. Our platform broadens the range of optical simulators for controlled investigations of non-Hermitian quantum dynamics.
The evolution of a closed quantum system is described by a unitary operator generated by a Hermitian Hamiltonian. However, when certain degrees of freedom are coupled to an environment, the relevant dynamics can be captured by non-unitary evolution operators, arising from non-Hermitian Hamiltonians. Here we introduce a photonic platform that implements non-unitary quantum walks, commonly used to emulate open-system dynamics, in the synthetic space of light transverse momentum. These walks are realized by propagating light through a series of dichroic liquid-crystal metasurfaces that impart polarization-dependent momentum shifts. The non-unitary behavior stems from dichroic dye molecules with polarization-dependent absorption, whose orientation is coupled to that of the liquid crystals. We demonstrate multiple walks up to five time steps, with adjustable levels of dichroism set by the metasurface voltage, which is controlled remotely. This discrete-time process maps onto two-band tight-binding models with reciprocal yet non-Hermitian nearest-neighbor couplings, corresponding to a less-studied class of non-Hermitian systems. Our platform broadens the range of optical simulators for controlled investigations of non-Hermitian quantum dynamics.
The possibility of fine-tuning the couplings between optical modes is a key requirement in photonic circuits for quantum simulations. In these architectures, emulating the long-time evolution of particles across large lattices requires sophisticated setups that are often intrinsically lossy. Here we report ultra-long photonic quantum walks across several hundred optical modes, obtained by propagating a light beam through very few closely stacked liquid-crystal metasurfaces. By exploiting spin–orbit effects, these implement space-dependent polarization transformations that mix circularly polarized optical modes carrying quantized transverse momentum. As each metasurface implements long-range couplings between distant modes, by using only a few of them we simulate quantum walks up to 320 discrete steps without any optical amplification, far beyond state-of-the-art experiments. To showcase the potential of this method, we experimentally demonstrate that in the long time limit a quantum walk affected by dynamical disorder generates maximal entanglement between two system partitions. Our platform grants experimental access to large-scale unitary evolutions while keeping optical losses at a minimum, thereby paving the way to massive multi-photon multi-mode quantum simulations.
Photonic implementations of unitary processes on lattice structures, such as quantum walks, have been demonstrated across various architectures. However, few platforms offer the combined advantages of scalability, reconfigurability, and the ability to simulate dynamics on lattices with periodic boundary conditions. Here, we employ a recently developed platform that enables the implementation of arbitrary translation-invariant unitary operations on one- and two-dimensional lattices, and demonstrate a mechanism for introducing periodic boundary conditions. Our approach leverages the possibility of shaping the evolution operator directly in the reciprocal lattice, where discrete sampling of the unitary effectively enforces the desired topology. We program our platform to realize quantum walks on one-dimensional cyclic lattices and two-dimensional lattices with cylindrical or toroidal topologies. The lattice size is controlled by adjusting the sampling density in reciprocal space. We investigate the dynamics of localized states and wavepackets, observing refocusing behavior, breathing modes modulated by reciprocal-space discretizations, and wavepacket trajectories that reflect the underlying topology. Finally, we demonstrate a form of dimensional reduction by mapping a two-dimensional quantum walk on a cylinder to a one-dimensional walk with a high-dimensional coin. These results establish a novel paradigm for realizing a broad class of optical mode transformations within bounded Hilbert spaces.
The evolution of a quantum system interacting with an environment can be described as a unitary process acting on both the system and the environment. In this framework, the system's evolution can be predicted by tracing out the environmental degrees of freedom. Here, we establish a precise mapping between the global unitary dynamics and the quantum operation involving the system, wherein the system is a single qubit, and the environment is modeled as a discrete lattice space. This approach enables the implementation of arbitrary noise operations on single-polarization qubits using a minimal set of three liquid-crystal metasurfaces, whose transverse distribution of the optic axes can be patterned to reproduce the target process. We experimentally validate this method by simulating common noise processes, such as phase errors and depolarization. Besides providing a practical solution for quantum state purification, this work demonstrates a versatile approach for the simulation of open qubit dynamics, with potential implications for quantum error correction and environment-induced quantum phase transitions.
Abstract Photonic implementations of unitary processes on lattice structures, such as quantum walks, have been demonstrated across various architectures. However, few platforms offer the combined advantages of scalability, reconfigurability, and the ability to simulate dynamics on lattices with periodic boundary conditions, such as cyclic or toroidal geometries. Here, we employ a recently developed platform that enables the implementation of arbitrary translationally invariant unitary operations on one- and two-dimensional lattices, and demonstrate a natural mechanism for introducing periodic boundary conditions. Our approach leverages direct access to the reciprocal lattice, where discrete sampling of the unitary evolution effectively enforces the desired topology. We program our platform to realize quantum walks on 1D cyclic lattices and 2D lattices with cylindrical or toroidal topologies. The lattice size can be readily tuned by adjusting the sampling density in reciprocal space. By controlling reciprocal-space occupancy, we investigate the dynamics of localized states and wavepackets, observing refocusing behavior, breathing modes modulated by reciprocal-space discretizations, and wavepacket trajectories that reflect the underlying topology. We further demonstrate a form of dimensional reduction by mapping a 2D quantum walk on a cylinder to a 1D walk with a high-dimensional coin. These results establish a versatile platform for realizing a broad class of optical mode transformations within bounded Hilbert spaces.
Open quantum systems generally do not perfectly preserve phase coherence: coupling to uncontrolled environments requires a density-matrix description based on the Liouvillian framework beyond pure-state wave evolution. Realizing and probing such dynamics in a programmable platform is therefore essential for connecting coherent physics to realistic dissipative settings. Here we implement a tunable open-system quantum walk in a photonic mesh lattice, where controlled phase noise produces adjustable dephasing and non-reciprocal gain-loss imbalance provides an independently tunable non-Hermitian drive. This allows us to continuously interpolate between coherent quantum walks and incoherent classical walks, and to observe how directional transport evolves in the Liouvillian regime. Using non-Hermitian skin dynamics as a probe, we measure the center-of-mass drift over both the coherence and non-Hermiticity parameters, revealing a crossover from coherence-enhanced to decoherence-enhanced transport in quantitative agreement with quantum-channel simulations. We further program spatial and temporal interfaces to demonstrate interface accumulation and a long-time drift governed by the instantaneous channel. Our results establish a controllable photonic platform for simulating open quantum dynamics and show that decoherence can actively reshape non-Hermitian transport.
The observation of extreme dynamics within quantum simulators based on photonic circuits is typically precluded by optical losses, exponentially increasing with the system depth or, equivalently, with the number of optical components. This is a natural consequence of the standard approach to photonic simulations of quantum dynamics, where the complexity of the setup grows with the extension of the evolution in time. By focusing on simple protocols of discrete-time quantum walks, we show that it is possible to compress homogeneous evolutions within only three liquid-crystal metasurfaces, encompassing up to a few hundreds of time steps. By exploiting spin-orbit effects, these devices implement space-dependent polarization transformations that mix circularly polarized optical modes carrying quantized transverse momentum, mimicking the target quantum dynamics with high efficiency and accuracy. Being extremely versatile, our compact platform will pave the way to the simulations of extreme regimes of more exotic dynamics.