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Randomness in Dissipative and Chaotic Quantum Dynamics

MARTINEZ AZCONA, Pablo

Published Sep 17, 2025• 0 citations
OpenAlex

Abstract

This thesis studies randomness in quantum dissipative and chaotic dynamics. We first focus on a detailed study of the effect of noise in the Hamiltonian of a quantum system, going beyond the noise-average and characterizing higher moments. The main quantity we introduce is the Stochastic Operator Variance (SOV), which is an observable characterizing the spread of trajectories around the average evolution. Interestingly, this quantity fulfills different types of uncertainty relations and is related to quantum information scrambling through out-of-time-order correlators (OTOC). We illustrate the SOV-OTOC connection in a stochastic version of the Lipkin-Meshkov-Glick (LMG) model, which shows a positive Lyapunov exponent from an unstable saddle point. We find that under the action of the noise, this Lyapunov exponent can change sign, thus stabilizing the unstable phase of the model while destabilizing the stable one. We then study the interplay between noise and decay in a non-Hermitian Hamiltonian. The noise-average evolution follows an antidephasing master equation beyond Lindblad form. We characterize the purity dynamics and the steady states of this master equation, and study this new evolution in a stochastically driven version of the Dissipative Qubit. By characterizing its spectral and steady state properties, we find that there are three phases: the PT unbroken, PT broken, and a novel Noise Induced (NI) phase where the qubit converges to the lossy state. We further investigate the validity of our model to explain experimental data, such as the residual damping rate of the PT unbroken phase. In the last Chapter, we study randomness as a model for chaotic dynamics. In particular, leveraging a Wigner-like surmise for the k-th neighbor level spacing distribution, we compute analytically the k-th neighbor Spectral Form Factor (knSFF), which characterizes the contribution of the k-th neighbor spacings to the Spectral Form Factor (SFF). We study the properties of the individual knSFF and characterize their role in building the universal ramp of the SFF. Interestingly, we find that the very short-range and very long-range spacings are the ones that contribute the most to the extent of the ramp. We finish by discussing our results and possible pathways for further research.

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We study generic open quantum systems with Markovian dissipation, focusing on a class of stochastic Liouvillian operators of Lindblad form with independent random dissipation channels (jump operators) and a random Hamiltonian. We perform a thorough numerical study, focusing on global spectral features, the spectral gap, and the steady-state purity and statistics. We establish that all properties follow three different regimes as a function of the dissipation strength, whose boundaries depend on the particular observable. Within each regime, we determine the scaling exponents with the dissipation strength and system size. On the analytical side, we compute the average spectral gap at arbitrary dissipation and provide simple closed-form expressions for the asymptotic values at strong and weak dissipation strength. We also consider spectral correlations in generic complex spectra, such as that of the Liouvillian. We introduce and study, both analytically and numerically, the complex ratio of the nearest-neighbor spacing by next-to-nearest-neighbor spacing. Besides the usual level repulsion, we find that complex spacing ratios have a nontrivial angular dependence which offers a distinct signature of quantum chaos. It distinguishes integrable systems, which support the flat ratio distribution characteristic of Poisson statistics, and chaotic dissipative quantum systems, which conform to Random Matrix Theory statistics. We apply this new signature of quantum chaos to random Liouvillians and boundary-driven dissipative spin-chains. The results of this thesis can help understand the long-time dynamics, steady-state properties, and spectral correlations of generic dissipative systems.

arXiv:1911.02136•Nov 5, 2019•0 citations

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Minimal models of quantum chaotic many-body systems

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Phenomena in quantum chaotic systems such as spectral fluctuations are known to be described remarkably well by the random matrix theory (RMT) in small energy intervals and over large time scales. However, in exchange for analytical tractability, RMT has been constructed to leave out an important element of realistic physical systems { the notion of locality. Since quantum information propagates at a finite speed in a spatially-extended quantum chaotic system, there exists time scales before which RMT is effective. How do we describe the non-equilibrium quantum dynamics at intermediate timescales which are much longer than the local relaxation time but too short for RMT to apply? What are the signatures of many-body quantum chaotic systems beyond the description of RMT? In this thesis, we address these questions by analysing minimal models that incorporate a notion of locality and at the same time retain some analytical tractability of RMT. More specifically, we study Floquet quantum circuits that are random in space but periodic in time. These circuits consist of local and random quantum gates that act on a q-state `spin' at each site. After a brief review of classical chaos, quantum chaos, and quantum circuits in Chapter 1, we present three main results. In Chapter 2, we formulate a diagrammatical approach for computing ensemble averages of observables over random unitary circuits, and derive exact results on spectral statistics and dynamical observables for a Floquet circuit in the large-q limit. In Chapter 3, we further investigate the spectral statistics in spatiallyextended many-body quantum chaotic systems by computing the spectral form factor K(t) analytically and numerically. We show that K(t) follows the RMT description at times longer than the Thouless time tTh and identify the scaling of tTh at the large-q limit of a Floquet circuit. In Chapter 4, we discuss eigenstate correlations for spatially-extended many-body quantum chaotic systems, in terms of the statistical properties of matrix elements of local observables. While the eigenstate thermalization hypothesis (ETH) is known to give an excellent description of these quantities, the phenomenon of scrambling and the butterfly effect imply structure beyond ETH. We determine analytically and verify numerically the universal form of this structure at long distances and small eigenvalue separations for Floquet systems.

•Jan 1, 2019•0 citations

Imposing Structure on Chaos in Complex Quantum Systems: Theoretical Predictions to Experimental Validation

Suchsland, Lucien Philippe Leonard

At the heart of physics lies the human fascination with natural phenomena and the wish to understand the underlying principles. A well-known example is the butterfly effect. It describes how small changes in the initial state can cause significantly different measurement outcomes at later times. Such sensitivity to initial conditions is a key signature of chaotic systems and reflects their instability under small perturbations. The principle underlying this phenomenon is information spreading: with time, information about the perturbation propagates through the system, changing measurement results even at distant locations. In quantum systems, information not only spreads but can also scramble, meaning that the precise details about the perturbation are hidden in highly nonlocal correlations. Information scrambling has emerged as a universal feature of quantum chaos and, together with other universal features, serves as an organizing principle for quantum systems. 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We then approximately restore energy conservation by considering trotterized systems, ranging from unstructured and chaotic to highly structured and integrable ones. We find these systems to thermalize on a scale set by the trotterization step, slowly approaching the universal linear Krylov complexity growth regime. Approaching the linear growth regime is a fundamental property of trotterized systems with an unbounded spectrum, while systems with a bounded energy spectrum can evade thermalization as probed by Krylov complexity. Instead, they have a nonanalytic transition as the Trotter step size increases. Our study of Krylov complexity establishes its universal properties for discrete time evolution. The presented results deepen our understanding of the thermalizing behavior of different classes of systems in relation to their spectral properties by introducing an intuitive notion of a bath with chaotic characteristics. 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This shows that no direct, universal relation exists between the two. Finally, we discuss the effects of breaking the integrable structure of the TFIM. Our results show that for short times, chaotic systems in proximity of integrability can retain signatures of integrability. In contrast, we observe significant changes at large times. This suggests that information scrambling, as a universal feature of chaotic systems, is restored at large times—even in systems near integrability that exhibit order. Following the analysis of information spreading close to integrable regimes, we study the stability of information spreading in more generic systems. First, we consider charge-conserving random circuits. In these systems, charge-charge correlators exhibit large fluctuations across different circuit instances with a slow polynomial decay in time. At the same time, they remain stable against fine-tuned perturbations, which can be interpreted as dephasing noise in the eigenbasis of the charge density operators. Equivalently, charge-charge correlators are mostly insensitive to decoherence, with interference effects contributing only subleading corrections. In this sense, the charge information spreading probed by charge-charge correlators is effectively classical. We perform a detailed analysis and quantify the dephasing insensitivity of these correlators. This suggests that circuit-to-circuit fluctuations can be captured by considering small regions where “quantum” effects are included, embedded within otherwise “classical” dynamics. This observation motivates the development of an algorithm to compute charge-charge correlators for individual circuits on classical computers with high accuracy. We quantitatively relate the algorithm’s performance to the dephasing analysis. We demonstrate the algorithm’s accuracy numerically for charge-charge correlators. Then, we argue that in generic circuits without conservation laws, the information spreading, as probed by OTOCs, follows similar principles. We conclude by comparing OTOC values measured on quantum devices with up to 95 superconducting qubits and 1000 gates to predictions from the approximate algorithm. This cross-validates experimental measurements and theoretical predictions. In this thesis, we explore the implications of adding structure to chaotic quantum systems, contributing to a deeper understanding of the organizing principles governing quantum chaos. We establish that entanglement can be suppressed in the semiclassical limit and that Krylov complexity behaves differently in thermalizing or integrable time-dependent systems. We show that the phenomenon information scrambling is also present in chaotic quantum systems even in the vicinity of a quantum phase transition. Conversely, when charge conservation is added, information spreading is stabilized and becomes reminiscent of that in classical systems. This work opens up further research directions towards a better understanding of the quantum nature of chaotic quantum systems and the development of probes of chaos in time dependent systems with different types of structure.

•Jan 1, 2025•0 citations
This thesis studies randomness in quantum dissipative and chaotic dynamics. We first focus on a detailed study of the effect of noise in the Hamiltonian of a quantum system, going beyond the noise-average and characterizing higher moments. The main quantity we introduce is the Stochastic Operator Variance (SOV), which is an observable characterizing the spread of trajectories around the average evolution. Interestingly, this quantity fulfills different types of uncertainty relations and is related to quantum information scrambling through out-of-time-order correlators (OTOC). We illustrate the SOV-OTOC connection in a stochastic version of the Lipkin-Meshkov-Glick (LMG) model, which shows a positive Lyapunov exponent from an unstable saddle point. We find that under the action of the noise, this Lyapunov exponent can change sign, thus stabilizing the unstable phase of the model while destabilizing the stable one. We then study the interplay between noise and decay in a non-Hermitian Hamiltonian. The noise-average evolution follows an antidephasing master equation beyond Lindblad form. We characterize the purity dynamics and the steady states of this master equation, and study this new evolution in a stochastically driven version of the Dissipative Qubit. By characterizing its spectral and steady state properties, we find that there are three phases: the PT unbroken, PT broken, and a novel Noise Induced (NI) phase where the qubit converges to the lossy state. We further investigate the validity of our model to explain experimental data, such as the residual damping rate of the PT unbroken phase. In the last Chapter, we study randomness as a model for chaotic dynamics. In particular, leveraging a Wigner-like surmise for the k-th neighbor level spacing distribution, we compute analytically the k-th neighbor Spectral Form Factor (knSFF), which characterizes the contribution of the k-th neighbor spacings to the Spectral Form Factor (SFF). We study the properties of the individual knSFF and characterize their role in building the universal ramp of the SFF. Interestingly, we find that the very short-range and very long-range spacings are the ones that contribute the most to the extent of the ramp. We finish by discussing our results and possible pathways for further research.
We study generic open quantum systems with Markovian dissipation, focusing on a class of stochastic Liouvillian operators of Lindblad form with independent random dissipation channels (jump operators) and a random Hamiltonian. We perform a thorough numerical study, focusing on global spectral features, the spectral gap, and the steady-state purity and statistics. We establish that all properties follow three different regimes as a function of the dissipation strength, whose boundaries depend on the particular observable. Within each regime, we determine the scaling exponents with the dissipation strength and system size. On the analytical side, we compute the average spectral gap at arbitrary dissipation and provide simple closed-form expressions for the asymptotic values at strong and weak dissipation strength. We also consider spectral correlations in generic complex spectra, such as that of the Liouvillian. We introduce and study, both analytically and numerically, the complex ratio of the nearest-neighbor spacing by next-to-nearest-neighbor spacing. Besides the usual level repulsion, we find that complex spacing ratios have a nontrivial angular dependence which offers a distinct signature of quantum chaos. It distinguishes integrable systems, which support the flat ratio distribution characteristic of Poisson statistics, and chaotic dissipative quantum systems, which conform to Random Matrix Theory statistics. We apply this new signature of quantum chaos to random Liouvillians and boundary-driven dissipative spin-chains. The results of this thesis can help understand the long-time dynamics, steady-state properties, and spectral correlations of generic dissipative systems.
We study the quantum dynamics generated by a non-Hermitian Hamiltonian subject to stochastic perturbations in its anti-Hermitian part, describing fluctuating gains and losses. The dynamics averaged over the noise is described by an "antidephasing" master equation. We characterize the resulting state evolution and analyze its purity. The properties of such dynamics are illustrated in a stochastic dissipative qubit. Our analytical results show that adding noise allows for a rich control of the dynamics, stabilizing the lossy state and making state purification possible to a greater variety of steady states.
The out-of-time order correlator (OTOC) has been widely studied in closed quantum systems. However, there are very few studies for open systems and they are mainly focused on isolating the effects of scrambling from those of decoherence. Adopting a different point of view, we study the interplay between these two processes. This proves crucial in order to explain the OTOC behavior when a phase space contracting dissipation is present, ubiquitous not only in real life quantum devices but in the dynamical systems area. The OTOC decay rate is closely related to the classical Lyapunov exponent-with some differences-and more sensitive in order to distinguish the chaotic from the regular behavior than other measures. On the other hand, it is revealed as a generally simple function of the longest lived eigenvalues of the quantum evolution operator. We find no simple connection with the Ruelle-Pollicott resonances, but by adding Gaussian noise of ℏ_{eff} size to the classical system we recover the OTOC decay rate, which is a consequence of the correspondence principle put forward in Phys. Rev. Lett. 108, 210605 (2012)10.1103/PhysRevLett.108.210605 and Phys. Rev. E 99, 042214 (2019)10.1103/PhysRevE.99.042214.
Dissipative quantum chaos plays a central role in the characterization and control of information scrambling, nonunitary evolution, and thermalization, but it still lacks a precise definition. The Grobe-Haake-Sommers conjecture, which links Ginibre level repulsion to classical chaotic dynamics, was recently shown to fail [Phys. Rev. Lett. 133, 240404 (2024)PRLTAO0031-900710.1103/PhysRevLett.133.240404]. We properly restore the quantum-classical correspondence through a dynamical approach based on the von Neumann entropy (VNE) and out-of-time-order correlators (OTOCs), which reveal signatures of chaos beyond spectral statistics. Focusing on the open anisotropic Dicke model, we identify two distinct regimes: transient chaos, marked by rapid early-time growth of VNE and OTOCs followed by low saturation values, and steady-state chaos, characterized by high long-time values. We introduce a random matrix toy model and show that Ginibre spectral statistics signals short-time chaos rather than steady-state chaos. Our results establish VNE dynamics and OTOCs as reliable diagnostics of dissipative quantum chaos across different timescales.
Phenomena in quantum chaotic systems such as spectral fluctuations are known to be described remarkably well by the random matrix theory (RMT) in small energy intervals and over large time scales. However, in exchange for analytical tractability, RMT has been constructed to leave out an important element of realistic physical systems { the notion of locality. Since quantum information propagates at a finite speed in a spatially-extended quantum chaotic system, there exists time scales before which RMT is effective. How do we describe the non-equilibrium quantum dynamics at intermediate timescales which are much longer than the local relaxation time but too short for RMT to apply? What are the signatures of many-body quantum chaotic systems beyond the description of RMT? In this thesis, we address these questions by analysing minimal models that incorporate a notion of locality and at the same time retain some analytical tractability of RMT. More specifically, we study Floquet quantum circuits that are random in space but periodic in time. These circuits consist of local and random quantum gates that act on a q-state `spin' at each site. After a brief review of classical chaos, quantum chaos, and quantum circuits in Chapter 1, we present three main results. In Chapter 2, we formulate a diagrammatical approach for computing ensemble averages of observables over random unitary circuits, and derive exact results on spectral statistics and dynamical observables for a Floquet circuit in the large-q limit. In Chapter 3, we further investigate the spectral statistics in spatiallyextended many-body quantum chaotic systems by computing the spectral form factor K(t) analytically and numerically. We show that K(t) follows the RMT description at times longer than the Thouless time tTh and identify the scaling of tTh at the large-q limit of a Floquet circuit. In Chapter 4, we discuss eigenstate correlations for spatially-extended many-body quantum chaotic systems, in terms of the statistical properties of matrix elements of local observables. While the eigenstate thermalization hypothesis (ETH) is known to give an excellent description of these quantities, the phenomenon of scrambling and the butterfly effect imply structure beyond ETH. We determine analytically and verify numerically the universal form of this structure at long distances and small eigenvalue separations for Floquet systems.
At the heart of physics lies the human fascination with natural phenomena and the wish to understand the underlying principles. A well-known example is the butterfly effect. It describes how small changes in the initial state can cause significantly different measurement outcomes at later times. Such sensitivity to initial conditions is a key signature of chaotic systems and reflects their instability under small perturbations. The principle underlying this phenomenon is information spreading: with time, information about the perturbation propagates through the system, changing measurement results even at distant locations. In quantum systems, information not only spreads but can also scramble, meaning that the precise details about the perturbation are hidden in highly nonlocal correlations. Information scrambling has emerged as a universal feature of quantum chaos and, together with other universal features, serves as an organizing principle for quantum systems. This motivates imposing structure like locality on quantum systems in order to probe the capabilities and limits of such organizing principles. There have been significant advances in both theoretical and experimental directions in recent years. The newly gained flexibility in designing experiments and simulations also inspires the analytical study of quantum systems from the bottom up, where tractable models offer insights into the generic features of quantum mechanics. In this thesis we build upon these advances to explore the implications of adding structure to chaotic quantum systems for the behavior of such features. In particular, we consider the measures entanglement entropy and Krylov complexity as probes of structure. These quantities are closely connected to information spreading. This motivates us to study the influence of structure on information spreading in the second part. In the first part, we begin with a detailed discussion of the behavior of entanglement in chaotic systems. We impose a minimal amount of local structure by separating the system into two parts, each modeled as a single spin. We validate the predicted entanglement for typical states in such systems and show that it saturates the Page limit as the Hilbert space dimension increases. We then study how different initially unentangled product states approach the Page limit under time evolution. We consider three types of product states, each representing a distinct case. Random product states represent generic states only restricted by the absence of entanglement. Random dipole and quadrupolar states represent two distinct types of semi-classical structure. The results on the entanglement generation in the three different types of states refine our earlier conclusion, demonstrating that the semi-classical limit can suppress the generation of extensive entanglement. This suppression does not occur for random product or quadrupolar states; where the imposed structure is insufficient. We conclude the second chapter by presenting two protocols that can stabilize the dynamics at finite spin sizes, similar to the semi-classical limit. In the following chapter, we move from measuring the complexity of time-evolved states using entanglement entropy to investigating time-evolved operators through the lens of Krylov complexity. After a short introduction to Krylov complexity for Hamiltonian dynamics, we generalize the framework for discrete time evolution. We identify the linear growth of Krylov complexity as a universal feature of generic systems and analyze its behavior as we transition from chaotic to increasingly structured systems. Dual-unitary circuits converge toward this universal behavior at rates that can be as fast as exponential, consistent with their classification as maximally chaotic. We then approximately restore energy conservation by considering trotterized systems, ranging from unstructured and chaotic to highly structured and integrable ones. We find these systems to thermalize on a scale set by the trotterization step, slowly approaching the universal linear Krylov complexity growth regime. Approaching the linear growth regime is a fundamental property of trotterized systems with an unbounded spectrum, while systems with a bounded energy spectrum can evade thermalization as probed by Krylov complexity. Instead, they have a nonanalytic transition as the Trotter step size increases. Our study of Krylov complexity establishes its universal properties for discrete time evolution. The presented results deepen our understanding of the thermalizing behavior of different classes of systems in relation to their spectral properties by introducing an intuitive notion of a bath with chaotic characteristics. We link this thermalization behavior to information spreading, which we explore in the second part of this thesis. Information scrambling, along with the associated spreading, is a key phenomenon in chaotic systems with local structure. In the fourth chapter, we investigate information spreading in proximity to an integrable system exhibiting spontaneous symmetry breaking, the transverse field Ising model (TFIM). As expected, integrability prevents the scrambling of information. At the same time, information spreading probed by quenched out-of-time ordered correlators (OTOCs) exhibits features reminiscent of the quantum phase transition present in the TFIM. We unravel the intricate behavior of these OTOCs and identify the underlying mechanism that stabilizes the long-time values of OTOCs: dynamical relocalization. We provide two variations of the TFIM in which the relocalization phenomenon is not directly related to the presence of a quantum phase transition. This shows that no direct, universal relation exists between the two. Finally, we discuss the effects of breaking the integrable structure of the TFIM. Our results show that for short times, chaotic systems in proximity of integrability can retain signatures of integrability. In contrast, we observe significant changes at large times. This suggests that information scrambling, as a universal feature of chaotic systems, is restored at large times—even in systems near integrability that exhibit order. Following the analysis of information spreading close to integrable regimes, we study the stability of information spreading in more generic systems. First, we consider charge-conserving random circuits. In these systems, charge-charge correlators exhibit large fluctuations across different circuit instances with a slow polynomial decay in time. At the same time, they remain stable against fine-tuned perturbations, which can be interpreted as dephasing noise in the eigenbasis of the charge density operators. Equivalently, charge-charge correlators are mostly insensitive to decoherence, with interference effects contributing only subleading corrections. In this sense, the charge information spreading probed by charge-charge correlators is effectively classical. We perform a detailed analysis and quantify the dephasing insensitivity of these correlators. This suggests that circuit-to-circuit fluctuations can be captured by considering small regions where “quantum” effects are included, embedded within otherwise “classical” dynamics. This observation motivates the development of an algorithm to compute charge-charge correlators for individual circuits on classical computers with high accuracy. We quantitatively relate the algorithm’s performance to the dephasing analysis. We demonstrate the algorithm’s accuracy numerically for charge-charge correlators. Then, we argue that in generic circuits without conservation laws, the information spreading, as probed by OTOCs, follows similar principles. We conclude by comparing OTOC values measured on quantum devices with up to 95 superconducting qubits and 1000 gates to predictions from the approximate algorithm. This cross-validates experimental measurements and theoretical predictions. In this thesis, we explore the implications of adding structure to chaotic quantum systems, contributing to a deeper understanding of the organizing principles governing quantum chaos. We establish that entanglement can be suppressed in the semiclassical limit and that Krylov complexity behaves differently in thermalizing or integrable time-dependent systems. We show that the phenomenon information scrambling is also present in chaotic quantum systems even in the vicinity of a quantum phase transition. Conversely, when charge conservation is added, information spreading is stabilized and becomes reminiscent of that in classical systems. This work opens up further research directions towards a better understanding of the quantum nature of chaotic quantum systems and the development of probes of chaos in time dependent systems with different types of structure.