The orbital angular momentum (OAM) of photons provides a pivotal resource for carrying out high-dimensional quantum Pauli-X operations due to its unique discrete infinite orthogonality, which opens enticing perspectives for high-capacity quantum communication and multi-parallel quantum computation. However, the state-of-the-art Pauli-X gates that require cyclic transformation of OAM modes are mostly limited to four modes, face scalability challenges owing to the system redundancy and fidelity degradation induced by increased processing modes. Here, we propose a general strategy to design scalable quantum Pauli-X gates in high-dimensional OAM space by taking full advantage of the order-correlated spatial divergence property of OAM modes. Leveraging the mechanism of balance mode filtering, partitioned phase is embedded between two structurally symmetric Q-plate elements that enable bidirectional mode shifting to filter out the highest-order OAM mode for spatially selective phase modulation. Derived from radial matching between modes and partitioned phase profiles, this design of parallel mode transformation underpins the extension to higher dimensions by merely adjusting filter parameters. We demonstrate the five-mode cyclic transformation with mode purity and diffraction efficiency higher than 92% and 92.7%, respectively. By incorporating polarization-entangled photon sources, we further realize five-dimensional quantum Pauli-X gates encoded on OAM space and experimentally verify the entanglement of output mode states. Low modulation loss and efficient quantum state tomography (QST) techniques endow the reconstructed density matrices with fidelities exceeding 92.3% ± 0.1%, indicating the well-performed entanglement preservation of output states. These results confirm that our approach achieves scalable quantum Pauli-X gate operations through a simple balanced architecture with high coherence, consolidating a theoretical and experimental foundation for large-scale quantum computation encoded on high-dimensional OAM space.
The orbital angular momentum (OAM) of photons provides a pivotal resource for carrying out high-dimensional quantum Pauli-X operations due to its unique discrete infinite orthogonality, which opens enticing perspectives for high-capacity quantum communication and multi-parallel quantum computation. However, the state-of-the-art Pauli-X gates that require cyclic transformation of OAM modes are mostly limited to four modes, face scalability challenges owing to the system redundancy and fidelity degradation induced by increased processing modes. Here, we propose a general strategy to design scalable quantum Pauli-X gates in high-dimensional OAM space by taking full advantage of the order-correlated spatial divergence property of OAM modes. Leveraging the mechanism of balance mode filtering, partitioned phase is embedded between two structurally symmetric Q-plate elements that enable bidirectional mode shifting to filter out the highest-order OAM mode for spatially selective phase modulation. Derived from radial matching between modes and partitioned phase profiles, this design of parallel mode transformation underpins the extension to higher dimensions by merely adjusting filter parameters. We demonstrate the five-mode cyclic transformation with mode purity and diffraction efficiency higher than 92% and 92.7%, respectively. By incorporating polarization-entangled photon sources, we further realize five-dimensional quantum Pauli-X gates encoded on OAM space and experimentally verify the entanglement of output mode states. Low modulation loss and efficient quantum state tomography (QST) techniques endow the reconstructed density matrices with fidelities exceeding 92.3% ± 0.1%, indicating the well-performed entanglement preservation of output states. These results confirm that our approach achieves scalable quantum Pauli-X gate operations through a simple balanced architecture with high coherence, consolidating a theoretical and experimental foundation for large-scale quantum computation encoded on high-dimensional OAM space.
The orbital angular momentum (OAM) of photons provides a pivotal resource for carrying out high-dimensional classical and quantum information processing due to its unique discrete high-dimensional nature. The cyclic transformation of a set of orthogonal OAM modes is an essential building block for universal high-dimensional information processing. Its realization in the quantum domain is the universal quantum Pauli-X gate. In this work, we experimentally demonstrate a cyclic transformation of six OAM modes with an averaged efficiency higher than 96% by exploiting a nonreciprocal Mach–Zehnder interferometer. Our system is simple and can, in principle, be scaled to more modes. By improving phase stabilization and inputting quantum photonic states, this method can perform universal single-photon quantum Pauli-X gate, thus paving the way for scalable high-dimensional quantum computation.
Unitary transformations are the fundamental building blocks of gates and operations in quantum information processing, allowing the complete manipulation of quantum systems in a coherent manner. In the case of photons, optical elements that can perform unitary transformations are readily available only for some degrees of freedom, e.g., wave plates for polarization. However, for high-dimensional states encoded in the transverse spatial modes of light, performing arbitrary unitary transformations remains a challenging task for both theoretical proposals and actual implementations. Following the idea of multi-plane light conversion, we show that it is possible to perform a broad variety of unitary operations at high quality by using only a few phase modulation planes. More importantly, we experimentally implement several high-dimensional quantum gates for up to five-dimensional states encoded in the full-field mode structure of photons. In particular, we realize cyclic and quantum Fourier transformations, known as Pauli X ^ -gates and Hadamard H ^ -gates, respectively, with an average visibility of more than 90%. In addition, we demonstrate near-perfect “unitarity” by means of quantum process tomography, unveiling a process purity of 99%. Last, we demonstrate the benefit of the two independent spatial degrees of freedom, i.e., azimuthal and radial, and implement a two-qubit controlled-NOT quantum operation on a single photon. Thus, our demonstrations open up new paths to implement high-dimensional quantum operations, which can be applied to various tasks in quantum communication, computation, and sensing schemes.
High-dimensional quantum computing has emerged as a recent alternative to conventional qubit-based approaches, offering advantages such as an increased information density and enhanced robustness against noise. In this work, we explore the use of the orbital angular momentum (OAM) of light as a degree of freedom in which high-dimensional quantum gates can be implemented. We present a theoretical and experimental study of structured light beams carrying OAM, with emphasis on Laguerre–Gauss modes, as a natural basis for high-dimensional quantum computing. We then describe the generation of OAM beams using computer-generated holograms and spatial light modulators, detailing practical methods for encoding arbitrary phase profiles. Building on this framework, we analyze the implementation of high-dimensional quantum logic gates, focusing on the generalized Pauli Z_d and X_d operations. Optical setups based on Dove prisms, Sagnac interferometers, spiral phase plates, and parity sorters are proposed and theoretically validated. Finally, we report experimental results demonstrating the generation of Laguerre–Gauss beams, the transformation properties of Dove prisms, and the operation of a parity sorter, which constitutes a building block for realizing high-dimensional quantum gates. These results establish a solid foundation for future implementations of high-dimensional quantum information processing using the orbital angular momentum of light.
The spatial modes of photons are one realization of a QuDit, a quantum system that is described in a D -dimensional Hilbert space. In order to perform quantum information tasks with QuDits, a general class of D -dimensional unitary transformations is needed. Among these, cyclic transformations are an important special case required in many high-dimensional quantum communication protocols. In this paper, we experimentally demonstrate a cyclic transformation in the high-dimensional space of photonic orbital angular momentum (OAM). Using simple linear optical components, we show a successful four-fold cyclic transformation of OAM modes. Interestingly, our experimental setup was found by a computer algorithm. In addition to the four-cyclic transformation, the algorithm also found extensions to higher-dimensional cycles in a hybrid space of OAM and polarization. Besides being useful for quantum cryptography with QuDits, cyclic transformations are key for the experimental production of high-dimensional maximally entangled Bell-states.
Structured light carrying Orbital Angular Momentum (OAM) enables high-dimensional photonic quantum information processing. In this work, we propose and theoretically demonstrate a four-dimensional controlledNOT (CNOT) quantum gate implemented using the radial (p) and azimuthal (l) degrees of freedom of Laguerre–Gaussian modes. Quantum information is encoded within a single photon, with the radial mode acting as the control qubit and the OAM mode as the target qubit. The gate is realized using fully linear and unitary optical transformations based on Fourier transform based radial mode sorting and OAM inversion within the architecture. This approach enables deterministic two-qubit logic in an expanded Hilbert space, providing a scalable pathway toward high-dimensional quantum gates using structured light.
High-dimensional degrees of freedom of photons can encode more quantum information than their two-dimensional counterparts. While the increased information capacity has advantages in quantum applications (such as quantum communication), controlling and manipulating these systems has been challenging. Here we show a method to perform deterministic arbitrary high-dimensional Pauli X gates for single photons carrying orbital angular momentum. The X gate consists of a cyclic permutation of qudit basis vectors and, together with the Z gate, forms the basis for performing arbitrary transformations. The proposed experimental setups only use two basic optical elements such as mode sorters and mode shifters and thus could be implemented in any system where these experimental tools are available. Furthermore the number of involved interferometers scales logarithmically with the dimension, which is important for practical implementation.