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Deterministic preparation of a dual-species two-ion crystal

Zawierucha, Maximilian J., Rehmert, Till, Keller, Jonas, Mehlstäubler, Tanja E., Schmidt, Piet O., Wolf, Fabian

Published Jan 1, 2024• 0 citations
Publisher

Abstract

The demand for efficient preparation methods for dual-species ion crystals is rapidly expanding across quantum technology and fundamental physics applications with trapped ions. We present a deterministic and efficient technique to produce such crystals, utilizing the segmented structure of a linear Paul trap. By precisely tailoring the trapping potentials, we can split, move, and discard parts of an ion chain. This process is automated in a sequence that converts a larger ion sample into the desired configuration. A critical component of our approach is the accurate identification of crystal constituents. This is achieved by matching the measured positions of fluorescing ions against theoretical expectations for larger crystals, thus facilitating the detection of nonfluorescing ions and enabling accurate ion counting. We demonstrate that our method reliably produces two-ion crystals within minutes. These results represent a significant advance in the production of two-species ion crystals with applications ranging from quantum logic spectroscopy and optical clocks to quantum computing and simulations with trapped ions.

DOI
10.15488/20134

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The demand for efficient preparation methods for dual-species ion crystals is rapidly expanding across quantum technology and fundamental physics applications with trapped ions. We present a deterministic and efficient technique to produce such crystals, utilizing the segmented structure of a linear Paul trap. By precisely tailoring the trapping potentials, we can split, move, and discard parts of an ion chain. This process is automated in a sequence that converts a larger ion sample into the desired configuration. A critical component of our approach is the accurate identification of crystal constituents. This is achieved by matching the measured positions of fluorescing ions against theoretical expectations for larger crystals, thus facilitating the detection of nonfluorescing ions and enabling accurate ion counting. We demonstrate that our method reliably produces two-ion crystals within minutes. These results represent a significant advance in the production of two-species ion crystals with applications ranging from quantum logic spectroscopy and optical clocks to quantum computing and simulations with trapped ions.
The demand for efficient preparation methods for dual-species ion crystals is rapidly expanding across quantum technology and fundamental physics applications with trapped ions. We present a deterministic and efficient technique to produce such crystals, utilizing the segmented structure of a linear Paul trap. By precisely tailoring the trapping potentials, we can split, move, and discard parts of an ion chain. This process is automated in a sequence that converts a larger ion sample into the desired configuration. A critical component of our approach is the accurate identification of crystal constituents. This is achieved by matching the measured positions of fluorescing ions against theoretical expectations for larger crystals, thus facilitating the detection of nonfluorescing ions and enabling accurate ion counting. We demonstrate that our method reliably produces two-ion crystals within minutes. These results represent a significant advance in the production of two-species ion crystals with applications ranging from quantum logic spectroscopy and optical clocks to quantum computing and simulations with trapped ions. Published by the American Physical Society 2024
The demand for efficient preparation methods for dual-species ion crystals is rapidly expanding across quantum technology and fundamental physics applications with trapped ions. We present a deterministic and efficient technique to produce such crystals, utilizing the segmented structure of a linear Paul trap. By precisely tailoring the trapping potentials, we can split, move, and discard parts of an ion chain. This process is automated in a sequence that converts a larger ion sample into the desired configuration. A critical component of our approach is the accurate identification of crystal constituents. This is achieved by matching the measured positions of fluorescing ions against theoretical expectations for larger crystals, thus facilitating the detection of non-fluorescing ions and enabling accurate ion counting. We demonstrate that our method reliably produces two-ion crystals within minutes. These results represent a significant advance in the production of two-species ion crystals with applications ranging from quantum logic spectroscopy and optical clocks to quantum computing and simulation with trapped ions.
In the endeavour to scale up the number of qubits in an ion-based quantum computer several groups have started to develop miniaturized ion traps for extended spatial control and manipulation of the ions. Shuttling and separation of ion strings have been the foremost issues in linear-trap arrangements and some prototypes of junctions have been demonstrated for the extension of ion motion to two dimensions (2D). While junctions require complex trap structures, small extensions to the 1D motion can be accomplished in simple linear trap arrangements. Here, control of the extended field in a planar, linear chip trap is used to shuttle ions in 2D. With this approach, the order of ions in a string is deterministically reversed. Optimized potentials are theoretically derived and simulations show that the reordering can be carried out adiabatically. The control over individual ion positions in a linear trap presents a new tool for ion-trap quantum computing. The method is also expected to work with mixed crystals of different ion species and as such could have applications for sympathetic cooling of an ion string.
The outstanding degree of control over trapped ions in Paul traps gives rise to the development of novel quantum manipulation techniques. Optical transitions can be used for precise manipulation of internal and external states. This way, non-classical states can be created which are a key component of quantum algorithms based on quantum logic operations. This powerful optical toolbox enabled the trapped ion system to assume leadership in the field of quantum computation. This thesis addresses two major challenges in the field of micro ion trap quantum optics. The temperature dependence of the heating rate from the ion trap surface is analysed in a novel cryogenic micro ion trap. Furthermore segmented traps allow state manipulations by time dependent electrical potentials, generated by the control voltages. These electrical fields provide a fast and reliable control handle to the ions external degrees of freedom. Quantum computation in Paul trap arrays is based on a combination of ion crystal transport, splitting and merging operations, while laser driven quantum state manipulations are mainly carried out on small ion crystals. Within this thesis a basic building block was realised by performing transport operations with a single ground-state cooled ion. As a highlight of experimental achievements, shuttling in the non-adiabatic regime, on the timescale of the motional period was demonstrated with low residual energy transfer. For his endeavour a specialised low noise arbitrary function generator was designed and manufactured during this thesis. Arbitrary voltage ramps at a sampling rate of up to 2.5 MS/s on up to 12 channels allow the study of a novel excitation method by directly manipulating the ion using electrical forces. Accurate numerical simulations in combination with the fast high resolution voltage supply allow deterministic quantum manipulations via momentum kicks. I report the first experimental demonstration of displaced number states with trapped ions.
Modern experiments with cold molecular ions have reached a high degree of complexity requiring frequent sample preparation, state initialization, and protocol execution while demanding precise control over multiple devices and laser sources. To maintain a high experimental duty cycle and robust measurement conditions, automation becomes essential. We present a fully automated control system for the preparation of trapped state-selected molecular ions and subsequent quantum logic-based experiments. Adaptive feedback routines based on real-time image analysis introduce and identify single molecular ions in atomic-ion Coulomb crystals. By appropriate manipulation of the trapping potentials, excess atomic ions are released from the trap to produce dual-species two-ion strings, specifically Ca+-N2+. After mass and state identification of the molecular ion, nanosecond-level synchronization of laser pulses employing the Sinara/ARTIQ framework and real-time data analysis enable quantum-logic-spectroscopic measurements. The present automated control system enables robust, unsupervised operation over extended periods resulting in an increase in the number of experimentation cycles by about a factor of ten compared to manual operation and a factor of about eight in loaded molecules in typical practical situations. The modular, distributed design of the system provides a scalable blueprint for similar molecular-ion experiments.
We theoretically investigate the process of splitting two-ion crystals in segmented Paul traps, i.e. the structural transition from two ions confined in a common well to ions confined in separate wells. The precise control of this process by application of suitable voltage ramps to the trap segments is non-trivial, as the harmonic confinement transiently vanishes during the process. This makes the ions strongly susceptible to background electric field noise, and to static offset fields in the direction of the trap axis. We analyze the reasons why large energy transfers can occur, which are impulsive acceleration, the presence of residual background fields and enhanced anomalous heating. For the impulsive acceleration, we identify the diabatic and adiabatic regimes, which are characterized by different scaling behavior of the energy transfer with respect to time. We propose a suitable control scheme based on experimentally accessible parameters. Simulations are used to verify both the high sensitivity of the splitting result and the performance of our control scheme. Finally, we analyze the impact of trap geometry parameters on the crystal splitting process.