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Correlated Quantum Matter Beyond Band Theory: A Continuum-Interaction Formalism for Strongly Coupled Electrons

Ndenga, Barack

Published Nov 26, 2025• 0 citations
Publisher

Abstract

This publication introduces the Extended Interaction Continuum (EIC) framework, providing a unified non-perturbative approach to strongly correlated electron systems. The framework captures Fermi liquid, strange-metal, and Mott insulating phases in 1D, 2D, and 3D systems. It provides falsifiable predictions for ARPES, STM/STS, and transport experiments. Numerical benchmarks and theoretical derivations validate the approach. Experimental collaboration is proposed to fully test the model.

DOI
10.5281/zenodo.17727010

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Journal of Advanced Interdisciplinary Studies•Jul 4, 2026•0 citations
This publication introduces the Extended Interaction Continuum (EIC) framework, providing a unified non-perturbative approach to strongly correlated electron systems. The framework captures Fermi liquid, strange-metal, and Mott insulating phases in 1D, 2D, and 3D systems. It provides falsifiable predictions for ARPES, STM/STS, and transport experiments. Numerical benchmarks and theoretical derivations validate the approach. Experimental collaboration is proposed to fully test the model.
The failure of conventional band theory to describe strongly correlated materials—high-Tc superconductors, Mott insulators, and strange metals—reveals a fundamental incompleteness in our current understanding of electron–electron interactions. In this work, I propose a unified continuum-interaction formalism that treats electronic behavior not as a perturbation around independent quasiparticles, but as an emergent quantum collective governed by non-local correlations. Using an extended Hubbard–Landau functional, a correlation-driven spectral reconstruction model, and a tensor-network-inspired coarse-graining operator, I derive a framework capable of capturing insulating, metallic, and incoherent regimes within a single mathematical structure. This approach suggests that the breakdown of band theory is not an anomaly but an inevitable manifestation of collective entanglement. I discuss analytical consequences, numerical implications, limitations, and future research directions toward a full predictive theory of correlated quantum matter.
In framework of eigen-functional bosonization method, we introduce an imaginary phase field to uniquely represent electron correlation, and demonstrate that the Landau Fermi liquid theory and the Tomonaga-Luttinger liquid theory can be unified. It is very clear in this framework that the Tomonaga-Luttinger liquid behavior of one-dimensional interacting electron gases originates from their Fermi structure, and the non-Landau-Fermi liquid behavior of 2D interacting electron gases is induced by the long-range electron interaction, while 3D interacting electron gases generally show the Landau Fermi liquid behavior. Typeset using REVTEX 1 Since the discovery of high Tc cuprate superconductors [1], the strongly correlated electron systems has been extensively studied theoretically [2–10]. Now a common consensus is reached that the low energy physics properties of cuprate superconductors, such as anomalous normal state behavior and high superconducting transition temperature, are determined
In framework of eigen-functional bosonization method, we introduce an imaginary phase field to uniquely represent electron correlation, and demonstrate that the Landau Fermi liquid theory and the Tomonaga-Luttinger liquid theory can be unified. It is very clear in this framework that the Tomonaga-Luttinger liquid behavior of one-dimensional interacting electron gases originates from their Fermi structure, and the non-Landau-Fermi liquid behavior of 2D interacting electron gases is induced by the long-range electron interaction, while 3D interacting electron gases generally show the Landau Fermi liquid behavior.
This dissertation is a study of various aspects of metals with strong interactions between electrons, with a particular emphasis on the problem of charge transport through them. We consider the physics of clean or weakly-disordered metals near some quantum critical points, and highlight novel transport regimes that could be relevant to experiments. We then develop a variety of exactly-solvable lattice models of strongly interacting non-Fermi liquid metals using novel non-perturbative techniques based on the Sachdev-Ye-Kitaev models, and relate their physics to that of the ubiquitous “strange metal” normal state of most correlated-electron superconductors, providing controlled theoretical insight into the possible mechanisms behind it. Finally, we use ideas from the field of quantum chaos to study mathematical quantities that can provide evidence for the existence of quasiparticles (or the lack thereof) in quantum many-body systems, in the context of metals with correlated electrons.
Experiments on strongly correlated quasi-two-dimensional electronic materials---for example, the high-temperature cuprate superconductors and the putative quantum spin liquids kappa-(BEDT-TTF)2Cu2(CN)3 and EtMe3Sb[Pd(dmit)2]2---routinely reveal highly mysterious quantum behavior which cannot be explained in terms of weakly interacting degrees of freedom. Theoretical progress thus requires the introduction of completely new concepts and machinery beyond the traditional framework of the band theory of solids and its interacting counterpart, Landau's Fermi liquid theory. In full two dimensions, controlled and reliable analytical approaches to such problems are severely lacking, as are numerical simulations of even the simplest of model Hamiltonians due to the infamous fermionic sign problem.Here, we attempt to circumvent some of these difficulties by studying analogous problems in quasi-one dimension. In this lower dimensional setting, theoretical and numerical tractability are on much stronger footing due to the methods of bosonization and the density matrix renormalization group, respectively. Using these techniques, we attack two problems: (1) the Mott transition between a Fermi liquid metal and a quantum spin liquid as potentially directly relevant to the organic compounds kappa-(BEDT-TTF)2Cu2(CN)3 and EtMe3Sb[Pd(dmit)2]2 and (2) non-Fermi liquid metals as strongly motivated by the strange metal phase observed in the cuprates. In both cases, we are able to realize highly exotic quantum phases as ground states of reasonable microscopic models. This lends strong credence to respective underlying slave-particle descriptions of the low-energy physics, which are inherently strongly interacting and also unconventional in comparison to weakly interacting alternatives.Finally, working in two dimensions directly, we propose a new slave-particle theory which explains in a universal way many of the intriguing experimental results of the triangular lattice organic spin liquid candidates kappa-(BEDT-TTF)2Cu2(CN)3 and EtMe3Sb[Pd(dmit)2]2. With use of large-scale variational Monte Carlo calculations, we show that this new state has very competitive trial energy in an effective spin model thought to describe the essential features of the real materials.
Abstract: The metal–insulator transition (MIT) constitutes one of the most profound and persistent problems in condensed matter physics, sitting at the intersection of electronic structure theory, many-body physics, and emergent quantum phenomena. Conventional band theory, which successfully classifies materials as metals or insulators according to the filling of their electronic bands, fails dramatically when confronted with a class of compounds transition metal oxides chief among them that ought to be metallic by band-counting arguments yet are robustly insulating in the laboratory. The resolution of this paradox required abandoning the independent-electron picture entirely and recognizing that strong Coulomb repulsion between electrons can, by itself, drive localization. This insight, formalized by Mott and later distilled into the Hubbard model, established correlation-driven insulation as a phenomenon distinct from band insulation. The present paper offers a theoretical exploration of the MIT problem, tracing its conceptual development from the Mott criterion through the Hubbard Hamiltonian, the Brinkman–Rice scenario of quasiparticle mass divergence, and the watershed development of dynamical mean-field theory (DMFT), which rendered the Mott transition quantitatively tractable for the first time. We argue that the competition between the electronic bandwidth and the on-site interaction encoded in the ratio U/W provides the unifying organizing principle for the field. Building toward the modern frontier, we examine how the Mott transition connects to quantum phase transitions and quantum criticality, where zero-temperature instabilities governed by quantum rather than thermal fluctuations produce non-Fermi-liquid behavior and anomalous scaling. Case studies of vanadium oxides, rare-earth nickelates, and doped cuprates illustrate the diversity and subtlety of real correlated materials. We conclude that the MIT remains a central and unresolved problem whose continued study is increasingly entangled with the development of quantum materials and quantum technologies. Keywords: Metal–Insulator Transition; Mott Insulator; Strongly Correlated Electrons; Hubbard Model; DMFT; Quantum Criticality; Quantum Materials; Condensed Matter Physics