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Quantum ground-state cooling of two librational modes of a nanorotor

Stephan Troyer, Florian Fechtel, Hummer, Lorenz, Rudolph, Henning, Benjamin A. Stickler, Uroš Delić, Markus Arndt

Published Sep 16, 2025• 0 citations
Publisher

Abstract

Controlling the motion of nanoscale objects at the quantum limit promises new tests of quantum mechanics and advanced sensors. Rotational motion is of particular interest, as it follows nonlinear dynamics in a compact, closed configuration space, giving rise to a plethora of phenomena and applications beyond the possibilities of free or trapped linear motion. A prerequisite for such experiments is the capability to trap nanorotors and initialize them in a quantum ground state of libration. Here, we demonstrate the reliable, repetitive laser-induced loading of silica nanodimers and trimers into an optical tweezer. Coherent scattering in a high-finesse cavity allows us to cool two different librational modes to the quantum ground state with occupation numbers as low as nβ = 0.54 ± 0.32 and nα = 0.21 ± 0.03. By simultaneously cooling both degrees of freedom (nβ = 0.73 ± 0.22, nα = 1.02 ± 0.08) we align nanorotors to a space-fixed axis with precision better than 20 μrad, close to the zero-point amplitude of librations.

DOI
10.34726/11340

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Controlling the motion of nanoscale objects at the quantum limit promises new tests of quantum mechanics and advanced sensors. Rotational motion is of particular interest, as it follows nonlinear dynamics in a compact, closed configuration space, giving rise to a plethora of phenomena and applications beyond the possibilities of free or trapped linear motion. A prerequisite for such experiments is the capability to trap nanorotors and initialize them in a quantum ground state of libration. Here, we demonstrate the reliable, repetitive laser-induced loading of silica nanodimers and trimers into an optical tweezer. Coherent scattering in a high-finesse cavity allows us to cool two different librational modes to the quantum ground state with occupation numbers as low as nβ = 0.54 ± 0.32 and nα = 0.21 ± 0.03. By simultaneously cooling both degrees of freedom (nβ = 0.73 ± 0.22, nα = 1.02 ± 0.08) we align nanorotors to a space-fixed axis with precision better than 20 μrad, close to the zero-point amplitude of librations.
Abstract Controlling the motion of nanoscale objects at the quantum limit promises opportunities to test fundamental quantum physics and advances in quantum sensing. Rotational motion is of particular interest, as its nonlinear dynamics in a compact, closed configuration space provides access to phenomena such as rotational interferometry, tunnelling between angular configurations and quantum-enhanced torque sensing. A key requirement for such experiments is the capability to trap nanorotors and cool their orientation close to the two-dimensional librational quantum ground state. When rotational motion is confined in a harmonic potential, it becomes librational. Here we demonstrate that coherent scattering into a high-finesse cavity enables the ground-state cooling of two orthogonal librational modes of an optically levitated SiO 2 nanoparticle. Using a laser-induced desorption loading technique, we trap and cool several dimers and trimers of silica nanospheres to their respective ground states, all within a single day. The simultaneous cooling of both librational degrees of freedom allows us to align an individual nanorotor with respect to a space-fixed axis with an angular precision better than 20 µrad—close to the quantum-mechanical zero-point fluctuations.
Ground-state cooling is a prerequisite for exploring macroscopic quantum effects in mechanical motion of massive objects. Here we construct a polarization-angle-controllable coupled cavity-levitated-nanoparticle system in which two nanoparticles trapped by individual tweezers are coupled to a single-mode field in a cavity. We also study the simultaneous ground-state cooling of six mechanical displacement modes of the two levitated nanoparticles through the coherent scattering mechanism. By deriving the Hamiltonian of the system and performing the linearization, we obtain a linearized seven-mode Hamiltonian, which can exhibit the coupling structure and cooling mechanism. We confirm the physical condition for the appearance of dark modes, which will suppress the simultaneous ground-state cooling of these mechanical modes. We also find that, by properly tuning the polarization angle θθθ between the cavity field and the optical tweezer fields, the coupling channels can be controlled on demand and simultaneous ground-state cooling of these six motional modes of the two nanoparticles can be realized. Our work paves the way for generation and manipulation of collective macroscopic quantum effects in multiple levitated nanoparticles.
State purity is a key resource for experimental tests of quantum mechanics with massive objects. Cavity cooling of a levitated nanoparticle via coherent scattering stands out as a strategy to prepare highly pure states of its roto-translational motion. In several cases, though, the performance of cooling by coherent scattering is limited by the classical fluctuations of the laser field. Here we present a quantum theory of coherent-scattering experiments which includes the effect of the laser amplitude and phase noise. We derive a master equation for the noise-averaged particle's dynamics, valid for both center-of-mass and rotational degrees of freedom, and quantify the cooling performance for different levels of noise in state-of-the-art experiments. We compute approximate analytical expressions for the laser-noise-induced heating rates and excess phonon number in both regimes of weak and strong optomechanical coupling. Moreover, our model can be applied to laser noise processes with generic power spectral densities and finite correlation times. This work offers a toolbox to quantify and optimize the state purity in coherent-scattering experiments, and opens new avenues towards the preparation of quantum states with levitated systems.
Laser cooling is fundamental to quantum computing and metrology using atomic systems. Precise control often requires cooling atoms' motional degrees of freedom to the quantum ground state, imposing operation time and architectural limitations particularly in large-scale systems. Here we demonstrate how the integrated optical control of interest for scaling trapped-ion systems additionally enables laser cooling that bypasses limitations of conventional schemes. Leveraging multi-channel integrated delivery of ultraviolet to infrared wavelengths for calcium ion control including in passively phase-stable ultraviolet standing waves (SWs), we experimentally verify a long-standing prediction by Cirac et al., realizing Doppler cooling to below the conventional Doppler limit at a SW node. We also present the first realization of ground-state cooling via electromagnetically induced transparency (EIT) using a ``probe" beam delivered as a SW with atoms positioned at a node, predicted to enable multi-mode sub-recoil-limit laser cooling. We demonstrate cooling of motional modes spanning an approximately 5 MHz bandwidth from the Doppler temperature to near the ground state within 150~\textmu s, reaching nˉ≈0.05\bar n \approx 0.05nˉ≈0.05 phonon number occupancies for the target mode. Direct evaluation against the comparable running-wave (RW) scheme shows the SW implementation's simultaneous advantage in cooling rate, motional mode bandwidth, and final phonon number, as previously theoretically predicted. Our work leverages capabilities enabled by integrated optical delivery to demonstrate fast cooling of multiple modes to the quantum ground state, and more broadly how scalable approaches to optical control can enable enhancements in fundamental atomic functionalities.
This manuscript is a Matters Arising prepared for Nature Physics in response to Troyer et al. (2026), "Quantum ground-state cooling of two librational modes of a nanorotor" (doi.org/10.1038/s41567-026-03219-1). It proposes that the experimental demonstration of orientational alignment as a quantizable, ground-state-achievable property in a mesoscale rotor carries underexplored implications for theoretical coherence models in biological and complex adaptive systems. The argument identifies open problems made newly tractable by the Troyer et al. result and outlines implications for biometric coherence measurement instrumentation. No original experimental data are presented. This is a theoretical contribution by an independent researcher working within the Applied Quantum Psychology framework.
A nanoparticle trapped and cooled Cooling massive particles to the quantum ground state allows fundamental tests of quantum mechanics to be made; it would provide an experimental probe of the boundary between the classical and quantum worlds. Delić et al. laser-cooled an optically trapped solid-state object (a ∼150-nanometer-diameter silic a nanoparticle) into its quantum ground state of motion starting from room temperature. Because the object is levitated using optical forces, the experimental configuration can be switched to free fall, thereby providing a test bed for several macroscopic quantum experiments. Science , this issue p. 892