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Discovery of a Turbulent Correlated Liquid in a Non-Local Driven-Dissipative Quantum Fluid

Weysi, Martin

Published Nov 10, 2025• 0 citations
Publisher

Abstract

The definitive non-equilibrium ground state of the driven-dissipative quantum fluid, previously identified as a turbulent correlated liquid, is hereby revealed to be the terminal phase of an intrinsic, deterministic decay cascade. High-fidelity spinor Gross-Pitaevskii simulations prove that the system’s true initial state is a metastable soliton. This state inevitably decays via a newly discovered, transient ”hyper-ordered” intermediate lattice phase before fracturing into the final turbulent liquid attractor. This three-stage mechanistic pathway (Soliton → Hyper-Ordered Lattice → Turbulence) is shown to be a universal and fundamental property of the non-local spinor dynamics, supplanting previous phenomenological descriptions with a rigorous, mechanistic proof.

DOI
10.5281/zenodo.17571129

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Strongly correlated quantum fluids and effective thermalization in non-Markovian driven-dissipative photonic systems

José Lebreuillly

Collective quantum phenomena are fascinating, as they repeatedly challenge our comprehension of nature and its underlying mechanisms. The qualification ``quantum'' can be attributed to a generic many-body system whenever the interference effects related to the underlying wave nature of its elementary constituents can not be neglected anymore, and a naive classical description in terms of interacting billiard balls fails to catch its most essential features. This interference phenomenon called ``quantum degeneracy'' which occurs at weak temperatures, leads to spectacular collective behaviours such as the celebrated Bose-Einstein Condensation (BEC) phase transition, where a macroscopic fraction of a bosonic system of particles collapses below a critical temperature T_c on a single-particle state. 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Yet, over the last two decades a broad community has started investigating the possibility of stabilizing interacting quantum phases in novel nonlinear quantum optics architectures, where interacting photons have replaced their atomic and electronic counterpart. Thanks to their high level of controllability and flexibility, and the possibility of reaching the quantum degeneracy regime at exceptionally high temperatures, these platforms appear as extremely promising candidates for the ``quantum simulation'' of the most exotic many-body quantum problems: while the precursors experiments in semiconductor exciton-polariton already allow to reach the Bose-Einstein Condensation and superfluid regimes, novel platforms such as superconducting circuits, coupled cavity arrays or photons coupled to Rydberg EIT (Electromagnetically induced Transparency) atoms have entered the so-called `photon blockade' where photons behave as impenetrable particles, and open a encouraging pathway toward the future generation of strongly correlated phases with light. \nA specificity of quantum optics devices is their intrinsic ``non-equilibrium'' nature: the interplay between the practically unavoidable radiative and non-radiative losses and the external drive needed to replenish the photon gas leads the many-body system toward a steady-state presenting important non-thermal features. 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While being able to quantum simulate those emblematic strongly correlated quantum phases in this novel experimental context would strongly benefit to the quantum optics community, gaining such a kind of flexibility would also contribute to fill an important bridge between the equilibrium and the non-equilibrium statistical physics of open quantum systems, allowing to access in a controlled manner a whole new phenomenology at the interface between the two theories. \nIn this thesis I address those questions, which I reformulate in the following manner: \n \n-What are the conditions for the emergence of analogue equilibrium properties in open quantum systems in contact with a non-thermal environment ? \n \n-In particular, is it possible to stabilize strongly correlated quantum phases with a perfectly defined particle number in driven-dissipative photonic platforms, in spite of environment-induced losses and heating effects ? \n \nThe structure of the thesis is the following. \n \n \n[Chapter 1.] We give an overview of the physics of many-body photonic systems. As a first step we address the weakly interacting regime in the physical context of exciton-polaritons: after describing the microscopic aspects of typical experiments, we move to the discussion of non-equilibrium Bose-Einstein Condensation and the various mechanisms related to the emergence of thermal signatures at steady-state. The second part of this Chapter is dedicated to strongly interacting fluids. After drawing a quick overview of several experimental platforms presenting a good potential for the study of such physics in a near future, we discuss the relative performance of several schemes proposed in order to replenish the photonic population \n \n[Chapter 2.] We investigate the potential of a non-Markovian pump scheme with a narrow bandpass (Lorentzian shaped) emission spectrum for the generation of strongly correlated states of light in a Bose-Hubbard lattice. Our proposal can be implemented by mean of embedded inverted two-level emitters with a strong incoherent pumping toward the excited state. Our study confirms in a single cavity the possibility of stabilizing photonic Fock states in a single configuration, and strongly localized n=1 Mott-Insulator states in a lattice with n=1 density. We show that a relatively moderate hopping is responsible for a depletion of the Mott-state, which then moves toward a delocalized state reminiscent of the superfluid regime. Finally, we proceed to a mean-field analysis of the phase diagram, and unveil a Mott-to-Superfluid transition characterized by a spontaneous breaking of the U(1) symmetry and incommensurate density. The results of this Chapter are based on the following publications: \n- J. Lebreuilly, M. Wouters and I. Carusotto, ``Towards strongly correlated photons in arrays of dissipative nonlinear cavities under a frequency-dependent incoherent pumping'', C. R. Phys., 17(8), 836, 2016. \n- A. Biella, F. Storme, J. Lebreuilly, D. Rossini, R. Fazio, I. Carusotto and C. Ciuti, ``Phase diagram of incoherently driven strongly correlated photonic lattice'', Phys. Rev. A, 96, 023839, 2017. \n \n[Chapter 3.] In view of improving the performance of the scheme introduced in last chapter, and reproducing in particular the equilibrium zero temperature phenomenology in driven-dissipative photonic lattices, we develop a fully novel scheme based on the use of non-Markovian reservoirs with tailored broadband spectra which allows to mimick the effect of tunable chemical potential. Our proposal can be implemented by mean of a small number of emitters and absorbers and is accessible to current technologies. \n \nWe first analyse the case of a frequency-dependent emission with a square spectrum and confirm the possibility of stabilizing Mott insulator states with arbitrary integer density. Unlike the previous proposal the Mott state is robust against both losses and tunneling. A sharp transition toward a delocalized superfluid-like state can be induced by strong values of the tunneling or a change in the effective chemical potential. While an overall good agreement is found with the T=0 predictions, our analysis highlights small deviations from the equilibrium case in some parts of the parameters space, which are characterized by a non-vanishing entropy and the kinetic generation of doublon excitations. We finally consider an improved scheme involving additional frequency-dependent losses, and show in that case that the Hamiltonian ground-state is fully recovered for any choice of parameters. Our proposal, whose functionality relies on generic energy relaxation mechanisms and is not restricted to the Bose-Hubbard model, appears as a promising quantum simulator of zero temperature physics in photonic devices. The results of this Chapter are based on the following publication: \n- J. Lebreuilly, A. Biella, F. Storme, D. Rossini, R. Fazio, C. Ciuti and I. Carusotto, ``Stabilizing strongly correlated photon fluids with non-Markovian reservoirs'', Phys. Rev. A 96, 033828 (2017). \n \n[Chapter 4.] We adopt a broader perspective, and analyse the conditions for the emergence of analogous thermal properties in driven-dissipative quantum systems. We show that the impact of an equilibrated environment can be mimicked by several non-Markovian and non-equilibrated reservoirs. Chapter 2 already f

•Dec 7, 2017•2 citations
The definitive non-equilibrium ground state of the driven-dissipative quantum fluid, previously identified as a turbulent correlated liquid, is hereby revealed to be the terminal phase of an intrinsic, deterministic decay cascade. High-fidelity spinor Gross-Pitaevskii simulations prove that the system’s true initial state is a metastable soliton. This state inevitably decays via a newly discovered, transient ”hyper-ordered” intermediate lattice phase before fracturing into the final turbulent liquid attractor. This three-stage mechanistic pathway (Soliton → Hyper-Ordered Lattice → Turbulence) is shown to be a universal and fundamental property of the non-local spinor dynamics, supplanting previous phenomenological descriptions with a rigorous, mechanistic proof.
We numerically investigate the nonlinear dynamics of a two-dimensional exciton-polariton quantum fluid coherently driven by two counter-propagating laser beams. Using an exciton-photon coupled driven-dissipative Gross-Pitaevskii framework, we identify four distinct regimes-linear, solitonic, turbulent, and superfluid-emerging from the interplay between pump strength, laser detuning, and injected momentum, which together control the balance between kinetic and interaction energies in the quantum fluid. The different regimes are characterized through real-space and momentum-space observables, as well as through the temporal first-order coherence function. We show that turbulence occupies a well-defined and extended region of parameter space, marked by spontaneous vortex nucleation, and a pronounced reduction of temporal coherence, providing a clear signature of nonstationary dynamics. By constructing quantitative phase diagrams, we delineate the transitions between the various regimes and identify multiple pathways connecting solitonic, turbulent, and superfluid behaviors. Finally, we demonstrate that the turbulent regime persists over experimentally realistic parameter ranges compatible with state-of-the-art GaAs-based micro-cavity platforms, establishing counter-propagating polariton flows as a robust and versatile setting for the study of driven-dissipative quantum turbulence in two dimensions.
Investigating the initial conditions that lead many-body quantum systems to an out-of-equilibrium state is fundamental for understanding their thermalization dynamics. In this work we observe the relaxation for two regimes of excitation that can drive the turbulent Bose-Einstein condensate into two distinct final states, and are defined by the amount of energy injected into the system. The subcritical regime is characterized by a lower injection of energy, which can lead to an inverse particle cascade and, consequently, to the BEC mode repopulation during the relaxation process. The supercritical regime is marked by a higher energy injection, that may lead to the BEC dissolution and a final thermal state. In both cases we observe relaxation stages that exhibit the same key features: a direct cascade, a non-thermal fixed point with the same exponents, a prethermalization region and, finally, the thermalization of the system. In the final thermalization stage, universal scaling is observed for both regimes, even though their final states are completely different. By analyzing the coherence length of our turbulent cloud, we clearly visualize the recovery and the loss of the coherence for the subcritical and supercritical regimes after relaxation. These results indicate that the evolution of turbulence occurs independent of its initial conditions and of the final state achieved.
We review turbulence in ultracold quantum gases, using the scalar contact-interaction Bose-Einstein condensate as the reference system for quantized circulation, compressibility, vortices, sound, and cascades. We focus on the quantitative diagnostics that connect helium and classical phenomenology to microscopic wave-function dynamics: incompressible and compressible kinetic-energy spectra, wave-occupation spectra, spectral fluxes, vortex-resolved correlations, and velocity statistics. These diagnostics distinguish equilibrium vortex organization, decaying turbulent relaxation, forced cascade dynamics, and weak-wave turbulence, and show why power laws alone are insufficient evidence for a cascade. We survey experiments on two-dimensional Onsager clustering, three-dimensional vortex-line turbulence, box-trap wave cascades, engineered dissipation, and turbulent equations of state. We close by briefly placing the contact-interaction scalar superfluid system in a broader landscape of nonlocal, multicomponent, fermionic, and driven-dissipative quantum fluids, where turbulence concepts can be tested for universality.
The dynamics of nonequilibrium closed quantum systems and their route to thermalization are of fundamental interest to several fields, from cosmology to particle physics. However, a comprehensive description of nonequilibrium phenomena still presents a significant challenge. In this work, we report the observation of distinct stages during the relaxation of the decaying turbulence in trapped Bose-Einstein condensates. Our findings show a direct particle cascade from low to high momenta, a consequence of the energy injection in the system, exhibiting a characteristic universal scaling. This stage is followed by an inverse particle cascade responsible for repopulating the previously depleted condensate. Both cascades can be explained through self-similar solutions provided by wave turbulence theory. These findings provide important insights into the relaxation stages of out-of-equilibrium quantum many-body systems.
We investigate the emergence and evolution of turbulence in Bose-Einstein condensates driven far from equilibrium through a controlled energy injection. By applying a timeperiodic modulation for a fixed duration, we trigger nonequilibrium dynamics that lead to the formation of a turbulent state characterized by a complex distribution of excitations and density fluctuations. Our study focuses on the post-excitation relaxation process, where we observe a transient broadening of the momentum distribution: a signature of a direct energy cascade followed by an inverse particle cascade due to the nonlinear intra-scales energy transfer. Through systematic analysis based on the nonthermal fixed points and weak wave turbulence theories, we identify universal scaling laws governing the repopulation dynamics of the condensate. These findings advance our understanding of turbulent relaxation pathways in superfluids while enhancing the understanding of driven-dissipative quantum systems.
Collective quantum phenomena are fascinating, as they repeatedly challenge our comprehension of nature and its underlying mechanisms. The qualification ``quantum'' can be attributed to a generic many-body system whenever the interference effects related to the underlying wave nature of its elementary constituents can not be neglected anymore, and a naive classical description in terms of interacting billiard balls fails to catch its most essential features. This interference phenomenon called ``quantum degeneracy'' which occurs at weak temperatures, leads to spectacular collective behaviours such as the celebrated Bose-Einstein Condensation (BEC) phase transition, where a macroscopic fraction of a bosonic system of particles collapses below a critical temperature T_c on a single-particle state. Quantum coherence, when combined with inter-particle interactions, gives rise to highly non-classical frictionless hydrodynamic behaviours such as superfluidity (SF) and superconductivity (SC). \nEven more exotic quantum phases emerge in presence of important interactions as matter reaches a ``strongly correlated regime'' dominated by quantum fluctuations, where each particle is able to affect significantly the surrounding fluid: characteristic examples are the so-called Mott-Insulator (MI) quantum phase where particles are localized on a lattice due to a strong interaction-induced blockade, along with the Tonks-Girardeau (TG) gas where impenetrable bosons in one-dimension acquire effective fermionic statistics up to a unitary transformation, and the Fractional Quantum Hall (FQH) effect which occurs in presence of a gauge field, and features a special type of elementary excitation possessing a fractional charge and obeying to fractional statistics called `anyon'. \nThese quantum many-body effects were explored in a first place in systems well isolated from the external environment such as ultra-cold atomic gases or electrons in solid-state systems, within a physical context well described by ``equilibrium statistical mechanics''. Yet, over the last two decades a broad community has started investigating the possibility of stabilizing interacting quantum phases in novel nonlinear quantum optics architectures, where interacting photons have replaced their atomic and electronic counterpart. Thanks to their high level of controllability and flexibility, and the possibility of reaching the quantum degeneracy regime at exceptionally high temperatures, these platforms appear as extremely promising candidates for the ``quantum simulation'' of the most exotic many-body quantum problems: while the precursors experiments in semiconductor exciton-polariton already allow to reach the Bose-Einstein Condensation and superfluid regimes, novel platforms such as superconducting circuits, coupled cavity arrays or photons coupled to Rydberg EIT (Electromagnetically induced Transparency) atoms have entered the so-called `photon blockade' where photons behave as impenetrable particles, and open a encouraging pathway toward the future generation of strongly correlated phases with light. \nA specificity of quantum optics devices is their intrinsic ``non-equilibrium'' nature: the interplay between the practically unavoidable radiative and non-radiative losses and the external drive needed to replenish the photon gas leads the many-body system toward a steady-state presenting important non-thermal features. One one hand, an overwhelmingly large quantity of novel quantum phenomena is expected in the non-equilibrium framework, as breaking the thermal equilibrium condition releases severe constraints on the state of a quantum system and on the nature of its surrounding environment. On the other hand, we do not benefit yet of an understanding of non-equilibrium statistical mechanics comparable with its well-established equilibrium counterpart, which relies on strong historical foundations. Understanding how to tame (and possibly exploit) non-equilibrium effects in order to stabilize interesting quantum phases in a controlled manner often reveals a hard challenge. \nIn that prospect, an important conceptual issue in the non-equilibrium physics of strongly interacting photons regards the possibility of stabilizing ``incompressible quantum phases'' such as the Mott-Insulator or Fractional Quantum Hall states, and more generally to stabilize the ground-state of a given particle-number conserving Hamiltonian, in a physical context where dissipative losses can not be neglected. While being able to quantum simulate those emblematic strongly correlated quantum phases in this novel experimental context would strongly benefit to the quantum optics community, gaining such a kind of flexibility would also contribute to fill an important bridge between the equilibrium and the non-equilibrium statistical physics of open quantum systems, allowing to access in a controlled manner a whole new phenomenology at the interface between the two theories. \nIn this thesis I address those questions, which I reformulate in the following manner: \n \n-What are the conditions for the emergence of analogue equilibrium properties in open quantum systems in contact with a non-thermal environment ? \n \n-In particular, is it possible to stabilize strongly correlated quantum phases with a perfectly defined particle number in driven-dissipative photonic platforms, in spite of environment-induced losses and heating effects ? \n \nThe structure of the thesis is the following. \n \n \n[Chapter 1.] We give an overview of the physics of many-body photonic systems. As a first step we address the weakly interacting regime in the physical context of exciton-polaritons: after describing the microscopic aspects of typical experiments, we move to the discussion of non-equilibrium Bose-Einstein Condensation and the various mechanisms related to the emergence of thermal signatures at steady-state. The second part of this Chapter is dedicated to strongly interacting fluids. After drawing a quick overview of several experimental platforms presenting a good potential for the study of such physics in a near future, we discuss the relative performance of several schemes proposed in order to replenish the photonic population \n \n[Chapter 2.] We investigate the potential of a non-Markovian pump scheme with a narrow bandpass (Lorentzian shaped) emission spectrum for the generation of strongly correlated states of light in a Bose-Hubbard lattice. Our proposal can be implemented by mean of embedded inverted two-level emitters with a strong incoherent pumping toward the excited state. Our study confirms in a single cavity the possibility of stabilizing photonic Fock states in a single configuration, and strongly localized n=1 Mott-Insulator states in a lattice with n=1 density. We show that a relatively moderate hopping is responsible for a depletion of the Mott-state, which then moves toward a delocalized state reminiscent of the superfluid regime. Finally, we proceed to a mean-field analysis of the phase diagram, and unveil a Mott-to-Superfluid transition characterized by a spontaneous breaking of the U(1) symmetry and incommensurate density. The results of this Chapter are based on the following publications: \n- J. Lebreuilly, M. Wouters and I. Carusotto, ``Towards strongly correlated photons in arrays of dissipative nonlinear cavities under a frequency-dependent incoherent pumping'', C. R. Phys., 17(8), 836, 2016. \n- A. Biella, F. Storme, J. Lebreuilly, D. Rossini, R. Fazio, I. Carusotto and C. Ciuti, ``Phase diagram of incoherently driven strongly correlated photonic lattice'', Phys. Rev. A, 96, 023839, 2017. \n \n[Chapter 3.] In view of improving the performance of the scheme introduced in last chapter, and reproducing in particular the equilibrium zero temperature phenomenology in driven-dissipative photonic lattices, we develop a fully novel scheme based on the use of non-Markovian reservoirs with tailored broadband spectra which allows to mimick the effect of tunable chemical potential. Our proposal can be implemented by mean of a small number of emitters and absorbers and is accessible to current technologies. \n \nWe first analyse the case of a frequency-dependent emission with a square spectrum and confirm the possibility of stabilizing Mott insulator states with arbitrary integer density. Unlike the previous proposal the Mott state is robust against both losses and tunneling. A sharp transition toward a delocalized superfluid-like state can be induced by strong values of the tunneling or a change in the effective chemical potential. While an overall good agreement is found with the T=0 predictions, our analysis highlights small deviations from the equilibrium case in some parts of the parameters space, which are characterized by a non-vanishing entropy and the kinetic generation of doublon excitations. We finally consider an improved scheme involving additional frequency-dependent losses, and show in that case that the Hamiltonian ground-state is fully recovered for any choice of parameters. Our proposal, whose functionality relies on generic energy relaxation mechanisms and is not restricted to the Bose-Hubbard model, appears as a promising quantum simulator of zero temperature physics in photonic devices. The results of this Chapter are based on the following publication: \n- J. Lebreuilly, A. Biella, F. Storme, D. Rossini, R. Fazio, C. Ciuti and I. Carusotto, ``Stabilizing strongly correlated photon fluids with non-Markovian reservoirs'', Phys. Rev. A 96, 033828 (2017). \n \n[Chapter 4.] We adopt a broader perspective, and analyse the conditions for the emergence of analogous thermal properties in driven-dissipative quantum systems. We show that the impact of an equilibrated environment can be mimicked by several non-Markovian and non-equilibrated reservoirs. Chapter 2 already f