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Measurements of Atomic Beam Velocities with Phase Choppers and Precision Measurements of Alkali Atomic Polarizabilities

Ivan Hromada

Published Jan 1, 2014• 0 citations
OpenAlex

Abstract

Atom interferometers, in which de Broglie waves are coherently split and recombined to make interference fringes, now serve as precision measurement tools for several quantities in physics. Examples include measurements of Newton's constant, the fine structure constant, van der Waals potentials, and atomic polarizabilities. To make next-generation measurements of static electric dipole atomic polarizabilities with an atom beam interferometer, I worked on new methods to precisely measure the velocity distribution for atom beams. I will explain how I developed and used phase choppers to measure lithium, sodium, potassium, and cesium atomic beam velocities with 0.07% accuracy. I also present new measurements of polarizability for these atoms. I classify systematic errors into two broad categories: (1) fractional errors that are similar for all different types of atoms in our experiments, and (2), errors that scale with de Broglie wavelength or inverse atomic momentum in our experiments. This distinction is important for estimating the uncertainty in our measurements of ratios of atomic polarizabilities, e.g., αCs / αNₐ = 2.488(12).

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Atomic polarizability plays an essential role in topics ranging from van der Waals interactions, state lifetimes, and indices of refraction, to next generation atomic clocks and atomic parity non-conservation experiments. Polarizability measurements, such as the ones described in this thesis, provide valuable input to these subjects and serve as benchmark tests for sophisticated atomic structure calculations. We measured the static polarizability of potassium and rubidium with record precision and 0.5% uncertainty using a Mach-Zehnder atom interferometer with an electric-field gradient. To support future precision measurements of polarizability, we developed a new atom beam velocity measurement technique called phase choppers. Using phase choppers, we demonstrated measurements of mean atom beam velocity with an uncertainty of 0.1%. We also developed a new way to probe atomic structure: a measurement of a zero-crossing of the dynamic polarizability of potassium, known as a magic-zero wavelength. We measured the first magic-zero wavelength of potassium with 1.5 pm uncertainty and established a new benchmark measurement for the ratio of the D1 and D2 line strengths. Finally, we propose the use of a resonant photoionization detector for measurements of strontium polarizability, and the use of contrast interferometry for measurements of alkali dimer tensor polarizabilities.

•Jan 1, 2013•4 citations

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I used a Mach-Zehnder atom interferometer to measure the static electric-dipole polarizabilities of K, Rb, and Cs atoms with 0.11\% uncertainty. Static polarizability measurements serve as benchmark tests for 𝑎𝑏 𝑖𝑛𝑖𝑡𝑖𝑜 atomic structure calculations. Calculating atomic properties such as polarizabilities, van der Waals coefficients, state lifetimes, or oscillator strengths involves accurately calculating the valence electrons' electric-dipole transition matrix elements. Additionally, testing Cs atomic structure calculations helps interpret the results of parity non-conservation experiments, which in turn places constraints on beyond-the-standard-model physics. I discuss improvements to our experiment that allowed us to measure static polarizabilities with 0.11% uncertainty, and we present our results in the context of recent 𝑎𝑏 𝑖𝑛𝑖𝑡𝑖𝑜 and semi-empirical static polarizabilities and recent, high-precision measurements of excited state lifetimes and van der Waals C₆ coefficients. I also used our interferometer to develop a new technique for inertial sensing. High precision, portable, atom-interferometer gyroscopes and accelerometers are desirable for self-contained inertial navigation and in the future may be used for tests of General Relativity and searches for gravitational waves using satellite-mounted inertial sensors. Satellite-mounted atom interferometers are challenging to build because of size, weight, power, and reliability constraints. Atom interferometers that use nanogratings to diffract atoms are attractive for satellite-mounted inertial sensing applications because nanogratings weigh approximately nothing and require no power. We developed a new 𝑖𝑛 𝑠𝑖𝑡𝑢 measurement technique using our nanograting atom interferometer, and we used it to measure inertial forces for the benefit of our static polarizability measurements. I also review how to calculate the sensitivity of a nanograting atom interferometer, and I employed these calculations in order to design a portable, nanograting atom interferometer inertial sensor.

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Atom beam velocity measurements using phase choppers

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We describe a new method to measure atom beam velocity in an atom interferometer using phase choppers. Phase choppers are analogous to mechanical chopping discs, but rather than being transmitted or blocked by mechanical choppers, an atom receives different differential phase shifts (e.g. zero or π radians) from phase choppers. Phase choppers yield 0.1% uncertainty measurements of beam velocity in our interferometer with 20 min of data and enable new measurements of polarizability with unprecedented precision.

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Barbara Goss Levi

Thanks to the wave nature of matter, it's possible to build the atomic analog of an optical interferometer, although it's extremely difficult, because the de Broglie wavelengths of atoms are typically 10 000 times shorter than those of light. The feat was accomplished four years ago by a number of groups, each with a different scheme for splitting and recombining the matter waves. (See PHYSICS TODAY, July 1991, page 17.) We are now starting to see the fulfillment of the hopes raised by those first atom interferometers as researchers hone their interferometers to yield ever more precise values of fundamental constants or explore fundamental aspects of quantum mechanics such as Berry's phase. For example, Steven Chu and his colleagues at Stanford University have measured the ratio h/m of Planck's constant to the mass of a cesium atom with a precision of one part in 107, although the systematic errors are at the level of 1 part in 106. An experiment to improve the absolute accuracy of the h/m measurement to a few parts in 109 is underway. This ratio is one factor in the determination of the finestructure constant.

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Analysis of polarizability measurements made with atom interferometry

Maxwell D. Gregoire, Nathan J. Brooks, Raisa Trubko +1 more

We present revised measurements of the static electric dipole polarizabilities of K, Rb, and Cs based on atom interferometer experiments presented in [Phys. Rev. A 2015, 92, 052513] but now re-analyzed with new calibrations for the magnitude and geometry of the applied electric field gradient. The resulting polarizability values did not change, but the uncertainties were significantly reduced. Then we interpret several measurements of alkali metal atomic polarizabilities in terms of atomic oscillator strengths $f_{ik}$, Einstein coefficients $A_{ik}$, state lifetimes $τ_{k}$, transition dipole matrix elements $D_{ik}$, line strengths $S_{ik}$, and van der Waals $C_6$ coefficients. Finally, we combine atom interferometer measurements of polarizabilities with independent measurements of lifetimes and $C_6$ values in order to quantify the residual contribution to polarizability due to all atomic transitions other than the principal $ns$-$np_J$ transitions for alkali metal atoms.

arXiv:1606.01963•Jun 6, 2016•0 citations
Atom interferometers, in which de Broglie waves are coherently split and recombined to make interference fringes, now serve as precision measurement tools for several quantities in physics. Examples include measurements of Newton's constant, the fine structure constant, van der Waals potentials, and atomic polarizabilities. To make next-generation measurements of static electric dipole atomic polarizabilities with an atom beam interferometer, I worked on new methods to precisely measure the velocity distribution for atom beams. I will explain how I developed and used phase choppers to measure lithium, sodium, potassium, and cesium atomic beam velocities with 0.07% accuracy. I also present new measurements of polarizability for these atoms. I classify systematic errors into two broad categories: (1) fractional errors that are similar for all different types of atoms in our experiments, and (2), errors that scale with de Broglie wavelength or inverse atomic momentum in our experiments. This distinction is important for estimating the uncertainty in our measurements of ratios of atomic polarizabilities, e.g., αCs / αNₐ = 2.488(12).
Atomic polarizability plays an essential role in topics ranging from van der Waals interactions, state lifetimes, and indices of refraction, to next generation atomic clocks and atomic parity non-conservation experiments. Polarizability measurements, such as the ones described in this thesis, provide valuable input to these subjects and serve as benchmark tests for sophisticated atomic structure calculations. We measured the static polarizability of potassium and rubidium with record precision and 0.5% uncertainty using a Mach-Zehnder atom interferometer with an electric-field gradient. To support future precision measurements of polarizability, we developed a new atom beam velocity measurement technique called phase choppers. Using phase choppers, we demonstrated measurements of mean atom beam velocity with an uncertainty of 0.1%. We also developed a new way to probe atomic structure: a measurement of a zero-crossing of the dynamic polarizability of potassium, known as a magic-zero wavelength. We measured the first magic-zero wavelength of potassium with 1.5 pm uncertainty and established a new benchmark measurement for the ratio of the D1 and D2 line strengths. Finally, we propose the use of a resonant photoionization detector for measurements of strontium polarizability, and the use of contrast interferometry for measurements of alkali dimer tensor polarizabilities.
I used a Mach-Zehnder atom interferometer to measure the static electric-dipole polarizabilities of K, Rb, and Cs atoms with 0.11\% uncertainty. Static polarizability measurements serve as benchmark tests for 𝑎𝑏 𝑖𝑛𝑖𝑡𝑖𝑜 atomic structure calculations. Calculating atomic properties such as polarizabilities, van der Waals coefficients, state lifetimes, or oscillator strengths involves accurately calculating the valence electrons' electric-dipole transition matrix elements. Additionally, testing Cs atomic structure calculations helps interpret the results of parity non-conservation experiments, which in turn places constraints on beyond-the-standard-model physics. I discuss improvements to our experiment that allowed us to measure static polarizabilities with 0.11% uncertainty, and we present our results in the context of recent 𝑎𝑏 𝑖𝑛𝑖𝑡𝑖𝑜 and semi-empirical static polarizabilities and recent, high-precision measurements of excited state lifetimes and van der Waals C₆ coefficients. I also used our interferometer to develop a new technique for inertial sensing. High precision, portable, atom-interferometer gyroscopes and accelerometers are desirable for self-contained inertial navigation and in the future may be used for tests of General Relativity and searches for gravitational waves using satellite-mounted inertial sensors. Satellite-mounted atom interferometers are challenging to build because of size, weight, power, and reliability constraints. Atom interferometers that use nanogratings to diffract atoms are attractive for satellite-mounted inertial sensing applications because nanogratings weigh approximately nothing and require no power. We developed a new 𝑖𝑛 𝑠𝑖𝑡𝑢 measurement technique using our nanograting atom interferometer, and we used it to measure inertial forces for the benefit of our static polarizability measurements. I also review how to calculate the sensitivity of a nanograting atom interferometer, and I employed these calculations in order to design a portable, nanograting atom interferometer inertial sensor.
We describe a new method to measure atom beam velocity in an atom interferometer using phase choppers. Phase choppers are analogous to mechanical chopping discs, but rather than being transmitted or blocked by mechanical choppers, an atom receives different differential phase shifts (e.g. zero or π radians) from phase choppers. Phase choppers yield 0.1% uncertainty measurements of beam velocity in our interferometer with 20 min of data and enable new measurements of polarizability with unprecedented precision.
We have built an atom interferometer and, by applying an electric field on one of the two interfering beams, we have measured the static electric polarizability of lithium $\ensuremath{\alpha}=(24.33\ifmmode\pm\else\textpm\fi{}0.16)\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}30}\phantom{\rule{0.3em}{0ex}}{\mathrm{m}}^{3}$ with a 0.66% uncertainty. Our experiment is similar to an experiment done on sodium in 1995 by Pritchard and co-workers, with several improvements: the electric field can be calculated analytically and the interference signals have a large intensity and a high visibility, resulting in accurate phase measurements. This experiment illustrates the extreme sensitivity of atom interferometry: when the atom enters the electric field, its velocity increases and the fractional change, equal to $4\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}9}$ for our largest field, is measured with a ${10}^{\ensuremath{-}3}$ accuracy.
Thanks to the wave nature of matter, it's possible to build the atomic analog of an optical interferometer, although it's extremely difficult, because the de Broglie wavelengths of atoms are typically 10 000 times shorter than those of light. The feat was accomplished four years ago by a number of groups, each with a different scheme for splitting and recombining the matter waves. (See PHYSICS TODAY, July 1991, page 17.) We are now starting to see the fulfillment of the hopes raised by those first atom interferometers as researchers hone their interferometers to yield ever more precise values of fundamental constants or explore fundamental aspects of quantum mechanics such as Berry's phase. For example, Steven Chu and his colleagues at Stanford University have measured the ratio h/m of Planck's constant to the mass of a cesium atom with a precision of one part in 107, although the systematic errors are at the level of 1 part in 106. An experiment to improve the absolute accuracy of the h/m measurement to a few parts in 109 is underway. This ratio is one factor in the determination of the finestructure constant.
We present revised measurements of the static electric dipole polarizabilities of K, Rb, and Cs based on atom interferometer experiments presented in [Phys. Rev. A 2015, 92, 052513] but now re-analyzed with new calibrations for the magnitude and geometry of the applied electric field gradient. The resulting polarizability values did not change, but the uncertainties were significantly reduced. Then we interpret several measurements of alkali metal atomic polarizabilities in terms of atomic oscillator strengths fikf_{ik}fik​, Einstein coefficients AikA_{ik}Aik​, state lifetimes τkτ_{k}τk​, transition dipole matrix elements DikD_{ik}Dik​, line strengths SikS_{ik}Sik​, and van der Waals C6C_6C6​ coefficients. Finally, we combine atom interferometer measurements of polarizabilities with independent measurements of lifetimes and C6C_6C6​ values in order to quantify the residual contribution to polarizability due to all atomic transitions other than the principal nsnsns-npJnp_JnpJ​ transitions for alkali metal atoms.