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Acta Physica Polonica A

Classical Control of Quantized Fields: Cavity Qed and the Photon Pistol

Joseph H. Eberly, C. K. Law

Published Jan 1, 1998• 11 citations
Publisher

Abstract

By using the double-lambda configuration of energy levels and three classical fields, an atom or ion in a high-Q resonant cavity can be manipulated to create a single-mode quantum state in the cavity that is an arbitrary combination of Fock states for that mode.The same principles of operation can be applied to a cavity with much lower Q in order to produce a "photon pistol", a device that "shoots" one and only one photon when a trigger is pulled, and emits no photons at other times.

DOI
10.12693/aphyspola.93.55

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It was first realized by Purcell (1) that the spontaneous emission rate of a quantum system can be enhanced or suppressed by placing it in a resonant radiofrequency cavity. Spontaneous emission as it was first theoretically described by Einstein (2) is not a pure property of matter. It is described by matter coupled to quantized radiation field modes, which can be manipulated in an artificial structure such as a cavity. Cavity quantum electrodynamics (QED) is used to describe such effects that intimately depend on the fact that light is made of photons. Cavity QED has been extensively studied in atoms and the experimental proof was awarded with the Nobel Prize in 2012 (3). It has been applied to cooling of single atoms and for the detection of single atoms and creating and studying states with few photons and few atoms (4). In more recent developments these ideas have been extended to manipulate electronic states (5) and vibrations in molecules (6, 7). In PNAS, Flick et al. (8) introduce recent theoretical developments for the application of cavity QED to molecules and suggest possible novel applications to photochemistry. These include nonadiabatic dynamics of molecules in cavities, the modification of molecular properties, and the integration of QED with density functional theory. A quantized electromagnetic field mode can be described as a harmonic oscillator whose coordinate is the electric field displacement (Fig. 1 A ). The zero point energy translates into a nonvanishing field intensity ⟨ e 2 ⟩ in the ground state | 0 ⟩ (vacuum fluctuations). The electric vacuum field increases for a small cavity volume e c = ℏ ω c V ϵ 0 , [1] Fig. 1. ( A ) Illustration of the standing wave cavity mode and the resulting field quantization (Fock states). ( B ) Combined matter-field states (dressed states, | ± , n ⟩ … [↵][1]1To whom correspondence should be addressed. Email: smukamel{at}uci.edu. [1]: #xref-corresp-1-1

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Focus section on Cavity QED

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A single two-level emitter coupled to a single mode of an electromagnetic resonator constitutes the most fundamental instance of light--matter interaction. Realizations of this type of system are investigated in the field of cavity quantum electrodynamics (cavity QED). Particularly important are schemes in which the coupling is strong enough to exceed the spontaneous emission rate as well as cavity damping. In this case, the coherent exchange of excitation between source and photon is the dominating process, providing the unique possibility to deterministically control the quantum evolution of the system. Great progress has recently been accomplished, technologically as well as conceptually, and the focus section in this issue of Journal of Optics B: Quantum and Semiclassical Optics features five articles highlighting important recent developments in the field. 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The authors discuss how detunings between the subsystems affect the quantum feedback, an issue particularly relevant for ensembles of atoms with a spread in detuning. Perfect quantum feedback in this case requires the use of additional parameters to control the system. The majority of optical cavity QED experiments performed so far have used as a medium atoms traversing the cavity on random trajectories, such as, for example, thermal atomic beams. In this case, the observation of quantum effects is degraded in two ways. The Doppler effect and the finite transit time lead to line broadening, while the spatial structure of the cavity mode results in atoms in different locations experiencing different coupling with the photonic field. J E Reiner et al (pages 135--142) investigate the impact of these effects on quantum fluctuations in their cavity QED system. In order to overcome line broadening, they have developed a continuous cold atomic beam, extracted from a magneto-optical trap. An even better control of broadening effects and fluctuating coupling strength is provided by trapping the atoms inside the cavity and cooling them to temperatures at which their position spread is smaller than the optical wavelength. Much recent activity has been devoted to developing such an ultimate cavity QED system. A Vukics et al (pages 143--153) present a theoretical proposal for dynamically trapping and cooling atoms inside a cavity. By driving the atoms with a standing wave injected from the side of the cavity and by weakly exciting the cavity field itself, they predict three-dimensional trapping of the atom for periods around 1 second, an extremely long time on the typical scale of cavity QED dynamics. The essential component of their scheme is the interference between the two driving fields, determining the temperature of the particle and the stable trapping positions. 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In this short communication, a new type of two-channel cavity QED model is derived. Two-channel models are important for they often lead to quantum interference phenomena. The previous models relied on the use of two or more modes of the quantized electromagnetic field, partially because of energy and parity restrictions. As it is shown in this work, such restrictions may be overcome with the use of properly chosen configurations of atomic levels and the aplication of classical external fields. Competing one- and two-photon processes involving one single mode may be obtained.

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It has been recently shown [1] that, under suitable conditions, the interaction between a three-level atom and the quantized field of a bimodal microcavity may be effectively reduced to the two-photon coupling between a single two-level atom and the electromagnetic field in the resonator. The corresponding Hamiltonian model is characterized by intensity-dependent Stark shifts due to the presence of an intermediate off-resonance atomic level. Assume the cavity field prepared at in an arbitrary state and let an initially excited atom cross the cavity with an appropriately selected velocity. It is possible to show that, exploiting a single conditional measurement of the atomic state immediately after the atom leaves the resonator, the bimodal field is projected into a new state characterized by the same photon number distribution present at More in detail, the experimental scheme we propose makes it possible manipulating only the phases of the initial probability amplitudes of finding a well defined population in the cavity. We prove that the state into which the cavity collapses after a successful atomic measurement is unitarily related to the initial field state and the explicit form of the accomplishing operator is constructed. We wish to remark that, beside its inherent theoretical interest, this simple experimental scheme might also be of relevance in the socalled field of quantum communication [2], where implementing unitary modifications of a quantum state signal represents an issue of topical and central importance. More in general, our proposal provides a systematic procedure for controlling selected properties of a quantum state. We in fact demonstrate that our experimental scheme may be reliably exploited to generate orthogonal states to a prefixed one or to control the squeezing direction.

Kluwer Academic Publishers eBooks•Mar 5, 2006•0 citations
By using the double-lambda configuration of energy levels and three classical fields, an atom or ion in a high-Q resonant cavity can be manipulated to create a single-mode quantum state in the cavity that is an arbitrary combination of Fock states for that mode.The same principles of operation can be applied to a cavity with much lower Q in order to produce a "photon pistol", a device that "shoots" one and only one photon when a trigger is pulled, and emits no photons at other times.
Summary form only given. In quantum information processing, a qubit is realised as a superposition of atomic or ionic eigenstates, or as a superposition of the states of a photon. A coupling between these different types of qubits is necessary to perform quantum operations or quantum transmissions, e.g. in a quantum network where single atoms or ions are entangled with individual photons. To generate such an entanglement in a controlled way, a triggered source for single photons, a photon pistol, will be needed. Our scheme will lead to the emission of one photon into a single, predetermined mode of the radiation field in response to a trigger event. This photon is emitted from an atom strongly coupled to a high-finesse optical cavity, and the trigger is a classical light pulse. The device combines cavity-QED with an adiabatic transfer technique. We consider a single lambda-type three-level atom being placed inside an empty cavity.
A single two-level atom can be used to prepare an arbitrary photon number state (Fock state) in a high Q cavity . The atom undergoes a controlled succession of interactions with two cavity modes. One of them contains a coherent field. The atom transfers photons one by one from this field to the initially empty second mode. The scheme can be extended to prepare a quantum superposition of the vacuum with a Fock state, a highly non-classical situation. We discuss the feasibility of the experiment with our present Rydberg-atom cavity QED set-up.
It was first realized by Purcell (1) that the spontaneous emission rate of a quantum system can be enhanced or suppressed by placing it in a resonant radiofrequency cavity. Spontaneous emission as it was first theoretically described by Einstein (2) is not a pure property of matter. It is described by matter coupled to quantized radiation field modes, which can be manipulated in an artificial structure such as a cavity. Cavity quantum electrodynamics (QED) is used to describe such effects that intimately depend on the fact that light is made of photons. Cavity QED has been extensively studied in atoms and the experimental proof was awarded with the Nobel Prize in 2012 (3). It has been applied to cooling of single atoms and for the detection of single atoms and creating and studying states with few photons and few atoms (4). In more recent developments these ideas have been extended to manipulate electronic states (5) and vibrations in molecules (6, 7). In PNAS, Flick et al. (8) introduce recent theoretical developments for the application of cavity QED to molecules and suggest possible novel applications to photochemistry. These include nonadiabatic dynamics of molecules in cavities, the modification of molecular properties, and the integration of QED with density functional theory. A quantized electromagnetic field mode can be described as a harmonic oscillator whose coordinate is the electric field displacement (Fig. 1 A ). The zero point energy translates into a nonvanishing field intensity ⟨ e 2 ⟩ in the ground state | 0 ⟩ (vacuum fluctuations). The electric vacuum field increases for a small cavity volume e c = ℏ ω c V ϵ 0 , [1] Fig. 1. ( A ) Illustration of the standing wave cavity mode and the resulting field quantization (Fock states). ( B ) Combined matter-field states (dressed states, | ± , n ⟩ … [↵][1]1To whom correspondence should be addressed. Email: smukamel{at}uci.edu. [1]: #xref-corresp-1-1
A single two-level emitter coupled to a single mode of an electromagnetic resonator constitutes the most fundamental instance of light--matter interaction. Realizations of this type of system are investigated in the field of cavity quantum electrodynamics (cavity QED). Particularly important are schemes in which the coupling is strong enough to exceed the spontaneous emission rate as well as cavity damping. In this case, the coherent exchange of excitation between source and photon is the dominating process, providing the unique possibility to deterministically control the quantum evolution of the system. Great progress has recently been accomplished, technologically as well as conceptually, and the focus section in this issue of Journal of Optics B: Quantum and Semiclassical Optics features five articles highlighting important recent developments in the field. Strong coupling between single atoms and the electromagnetic cavity field have been achieved in two distinct regimes, the optical and the microwave region. The latter is represented by the micromaser, a high-Q microwave cavity pumped by a beam of highly excited Rydberg atoms. It has proved to be an almost ideal system for the generation of non-classical field states. A constraint in these experiments is the fact that the field inside the cavity can only be examined indirectly, by analysing the occupation of atoms leaving the cavity. While only two atomic states were previously identified for this purpose, V A Reshetov shows in his article (pages 119--126) that more information on the field may be extracted by taking advantage of the Zeeman substructure of the atomic levels. In the optical domain of cavity QED, by contrast, the state of the resonator field may be probed directly by measuring the light leaking from the cavity using photodetectors. In order to minimize damping, high-quality cavities must be employed. In most optical experiments these are Fabry--Perot resonators with ultra-high reflectivity mirrors, with losses as low as a few parts per million being state of the art. At the same time, the coupling of atoms and photons is enhanced by reducing the length of the cavity, so that strong coupling conditions are reached. A very attractive application of this type of cavity QED setup is the possibility of exerting control over the quantum dynamics of the system. An impressive example is the implementation of quantum feedback, reported in the paper by W P Smith and L A Orozco (pages 127--134). Using information gained from detecting a single photon escaping from the cavity, active feedback is applied to halt the dynamical evolution of the system. This is the first time active feedback has been used to modify the quantum evolution of a system at the single-photon level. The authors discuss how detunings between the subsystems affect the quantum feedback, an issue particularly relevant for ensembles of atoms with a spread in detuning. Perfect quantum feedback in this case requires the use of additional parameters to control the system. The majority of optical cavity QED experiments performed so far have used as a medium atoms traversing the cavity on random trajectories, such as, for example, thermal atomic beams. In this case, the observation of quantum effects is degraded in two ways. The Doppler effect and the finite transit time lead to line broadening, while the spatial structure of the cavity mode results in atoms in different locations experiencing different coupling with the photonic field. J E Reiner et al (pages 135--142) investigate the impact of these effects on quantum fluctuations in their cavity QED system. In order to overcome line broadening, they have developed a continuous cold atomic beam, extracted from a magneto-optical trap. An even better control of broadening effects and fluctuating coupling strength is provided by trapping the atoms inside the cavity and cooling them to temperatures at which their position spread is smaller than the optical wavelength. Much recent activity has been devoted to developing such an ultimate cavity QED system. A Vukics et al (pages 143--153) present a theoretical proposal for dynamically trapping and cooling atoms inside a cavity. By driving the atoms with a standing wave injected from the side of the cavity and by weakly exciting the cavity field itself, they predict three-dimensional trapping of the atom for periods around 1 second, an extremely long time on the typical scale of cavity QED dynamics. The essential component of their scheme is the interference between the two driving fields, determining the temperature of the particle and the stable trapping positions. In the quest for better confinement of radiation, lately, an appealing alternative to the Fabry--Perot cavity has been investigated -- the optical microsphere resonator. A sphere with a diameter of a few tens of microns, it supports so-called whispering gallery modes near its circumference, for which quality factors up to 10 10 have been measured. In order to exploit the correspondingly low field damping rates for cavity QED, a method must be found to couple atomic or solid state emitters to these modes. S Göotzinger et al (pages 154--158) report the coupling of single nanocrystals on the surface of a microsphere through the evanescent field of the mode. Selective excitation of a single nano-emitter was accomplished with a scanning confocal microscope. The system is a promising candidate for cavity QED with single-quantum emitters. The ability to fully control the quantum dynamics of atoms and light is beginning to spawn early applications. The most notable example is quantum information processing. This requires the coherent manipulation of single-quantum systems, which is ideally provided by cavity QED interaction in the strong-coupling limit. The development of practical devices will be among the principal future tasks for research in the field. This will include physical systems, which have not been covered in this issue, such as semiconductors, quantum dots as emitters, or photonic crystals as resonator structures. Cavity QED is therefore guaranteed to remain a vigorous field in the years to come.
In this short communication, a new type of two-channel cavity QED model is derived. Two-channel models are important for they often lead to quantum interference phenomena. The previous models relied on the use of two or more modes of the quantized electromagnetic field, partially because of energy and parity restrictions. As it is shown in this work, such restrictions may be overcome with the use of properly chosen configurations of atomic levels and the aplication of classical external fields. Competing one- and two-photon processes involving one single mode may be obtained.
It has been recently shown [1] that, under suitable conditions, the interaction between a three-level atom and the quantized field of a bimodal microcavity may be effectively reduced to the two-photon coupling between a single two-level atom and the electromagnetic field in the resonator. The corresponding Hamiltonian model is characterized by intensity-dependent Stark shifts due to the presence of an intermediate off-resonance atomic level. Assume the cavity field prepared at in an arbitrary state and let an initially excited atom cross the cavity with an appropriately selected velocity. It is possible to show that, exploiting a single conditional measurement of the atomic state immediately after the atom leaves the resonator, the bimodal field is projected into a new state characterized by the same photon number distribution present at More in detail, the experimental scheme we propose makes it possible manipulating only the phases of the initial probability amplitudes of finding a well defined population in the cavity. We prove that the state into which the cavity collapses after a successful atomic measurement is unitarily related to the initial field state and the explicit form of the accomplishing operator is constructed. We wish to remark that, beside its inherent theoretical interest, this simple experimental scheme might also be of relevance in the socalled field of quantum communication [2], where implementing unitary modifications of a quantum state signal represents an issue of topical and central importance. More in general, our proposal provides a systematic procedure for controlling selected properties of a quantum state. We in fact demonstrate that our experimental scheme may be reliably exploited to generate orthogonal states to a prefixed one or to control the squeezing direction.