Theory of Time-Dependent Spectral Observations in Qed and Quantum Optics

R. Loudon

Kamran Akbari, Franco Nori, Stephen Hughes

Strong periodic driving of cavity-quantum electrodynamics (QED) in the ultrastrong-coupling regime creates nonequilibrium states whose dissipation is governed by Floquet quasienergies rather than undriven dressed resonances. However, modeling such a regime is a significant theoretical challenge, including a number of subtle problems such as the need to ensure gauge invariance for truncated matter-cavity systems with time-dependent driving. To fill this theoretical gap, we introduce a nonsecular Floquet generalized master equation framework for strongly driven open cavity-QED systems, formulated in the dressed basis of the quantum Rabi model and applicable to structured reservoirs without rotating-wave approximations. Our theory can thus model Floquet-driven dynamics in open ultrastrong-coupling cavity-QED, and demonstrates a wide range of quantum state control. Using strong optical pumping and parametric mechanical modulation, we compute long-time populations, fluorescence spectra, and the Floquet-Liouville eigenspectra, resolving observable resonances into hybridized quasienergy channels and decay rates. By systematically comparing with conventional time-independent dressed-basis generalized master equations, we show that static approaches only reproduce steady-state populations in restricted excitation regimes, and fail for frequency-resolved observables and break down under appropriate Floquet engineering, surprisingly, even for spectrally flat baths. Structured environments, such as Lorentzian-Ohmic reservoirs, further amplify these discrepancies through sideband-selective decay. Our results demonstrate that dissipation in driven ultrastrong cavity-QED is intrinsically quasienergy resolved and we establish Floquet-dissipative theory as an accurate and powerful framework for predicting spectra, controlling decay pathways, and engineering nonequilibrium quantum states and reservoirs.

Christina J. Hood, Michael Chapman, T. W. Lynn +1 more

The combination of cold atoms and large coherent coupling enables investigations in a new regime in cavity QED with single-atom trajectories monitored in real time with high signal-to-noise ratio. The underlying ``vacuum-Rabi'' splitting is clearly reflected in the frequency dependence of atomic transit signals recorded atom by atom, with evidence for mechanical light forces for intracavity photon number $<1$. The nonlinear optical response of one atom in a cavity is observed to be in accord with the one-atom quantum theory but at variance with semiclassical predictions.

Richard H. Picard, C. R. Willis

Ravinder Rupchand Puri

Dylan J. Young, Eric Yilun Song, Anjun Chu +6 more

We use an ensemble of laser-cooled strontium atoms in a high-finesse cavity to cleanly emulate the technique of rf spectroscopy employed in studies of BEC-BCS physics in fermionic superfluids of degenerate cold gases. Here, we leverage the multilevel internal structure of the atoms to study the physics of Cooper pair breaking in this system. In doing so, we observe and distinguish the properties of two distinct many-body gaps, the BCS pairing gap and the spectral gap, using nondestructive readout techniques. The latter is found to depend on the populations of the internal atomic states, reflecting the chemical potential dependence predicted in fermionic superfluids. This work opens the path for more fully exploiting the rich internal structure of atoms in cavity QED emulators to study both analogous systems and also more exotic states yet to be realized.