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Spin liquid phase in the Hubbard model: Luttinger-Ward analysis ofthe slave-rotor formalism

Mehdi Kargarian, Xia-Ming Zheng

Published Jan 1, 2025• 0 citations
Publisher
DOI
10.2139/ssrn.5933379

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Motivated by recent experiments on the triangular lattice Mott-Hubbard system $\ensuremath{\kappa}\text{\ensuremath{-}}{(\mathrm{BEDT}\text{\ensuremath{-}}\mathrm{TTF})}_{2}{\mathrm{Cu}}_{2}{(\mathrm{C}\mathrm{N})}_{3}$, we develop a general formalism to investigate quantum spin liquid insulators adjacent to the Mott transition in Hubbard models. This formalism, dubbed the SU(2) slave-rotor formulation, is an extension of the SU(2) gauge theory of the Heisenberg model to the case of the Hubbard model. Furthermore, we propose the honeycomb lattice Hubbard model (at half filling) as a candidate for a spin liquid ground state near the Mott transition; this is an appealing possibility, as this model can be studied via quantum Monte Carlo simulation without a sign problem. The pseudospin symmetry of Hubbard models on bipartite lattices turns out to play a crucial role in our analysis, and we develop our formalism primarily for the case of a bipartite lattice. We also sketch its development for a general Hubbard model. We develop a mean-field theory to describe spin liquids and some competing states, and apply it to the honeycomb lattice. On the insulating side of the Mott transition, we find an SU(2) algebraic spin liquid (ASL), described by gapless S=1∕2S=1∕2S=1∕2 Dirac fermions (spinons) coupled to a fluctuating SU(2) gauge field. This result contrasts with that obtained via a U(1) slave-rotor approach, which instead found a U(1) ASL. That formulation does not respect the pseudospin symmetry, and is therefore not correct on the honeycomb lattice. We construct a low-energy effective theory describing the ASL phase, the conducting semimetal phase and the Mott transition between them. This physics can be detected in numerical simulations via the simultaneous presence of substantial antiferromagnetic and valence-bond solid correlations. In the SU(2) ASL, these observables have slowly decaying fluctuations in space and time, described by power laws with the same critical exponent. We recover the results of the U(1) slave-rotor formulation in the presence of a strong breaking of pseudospin symmetry. Our analysis suggests that both a third-neighbor electron hopping, and/or pseudospin-breaking terms such as a nearest-neighbor density interaction, may help to stabilize a spin liquid phase.
We study an optical Raman square lattice with U(1)\mathrm{U}(1)U(1) synthetic gauge flux to show a chiral spin liquid (CSL) phase for cold atoms based on slave-rotor and spinon mean-field theories, respectively. An effective U(1) gauge flux generated by Raman potentials plays a major role in realizing the CSL phase. By using slave-rotor techniques we find the CSL phase at a strong on-site Fermi Hubbard interacting regime. For large value of Hubbard interaction, we derive an effective spin model including up to the four spin interactions. By spinon mean-field analysis it is shown that the CSL phase is stabilized in the case of strong magnetic frustration. Two mean-field approximation methods give consistent phase diagrams and provide qualitative numerical evidence of the CSL phase.
We study the repulsive Hubbard model on an anisotropic honeycomb lattice within a mean-field and a slave-rotor treatment. In addition to the known semi-metallic and band-insulating phases, obtained for very weak interactions, and the anti-ferromagnetic phase at large couplings, various insulating spin-liquid phases develop at intermediate couplings. Whereas some of these spin liquids have gapless spinon excitations, a gapped one occupies a large region of the phase diagram and becomes the predominant phase for large hopping anisotropies. This phase can be understood in terms of weakly coupled strongly dimerized states.