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APL Photonics

High-dimensional frequency entanglement filter with anomalous Hong–Ou–Mandel interference

Chaojie Wang, Xutong Li, Yuning Zhang, Weifang Lu, Yuanyuan Chen, Lixiang Chen

Published Nov 1, 2025• 0 citations
Publisher

Abstract

Quantum entanglement is essential for various quantum information technologies that are beyond the possibilities of classical physics. However, it is susceptible to decoherence that may arise from noisy channels and environmental noise. While this deleterious problem has been explored by using filtering techniques, such as photon ancillas and Rydberg atom blockade, a concise yet efficient approach to entanglement retrieval is still a formidable challenge. Here, we present that nonunitary material provides an alternative tool to flexibly control the anomalous Hong–Ou–Mandel (HOM) interference and enables the selective entanglement filter with coherent perfect absorption of anti-symmetric quantum states. An elaborate Cr–SiN–Cr film is prepared as a nonunitary beam splitter such that its tunability over the effective photon–photon interaction in frequency modes can be readily explored in the experiment, which may introduce sophisticated nonunitary realization into integrated optical platforms. In addition, we confirm its ability for selective filtering of high-dimensional frequency entanglement by observing the output quantum state of the conventional HOM interference with a unitary beam splitter and the anomalous HOM interference with a nonunitary beam splitter. These results may offer new insights into investigating the quantum light–matter interaction and facilitating the use of two-photon interference for addressing central challenges in quantum technologies.

DOI
10.1063/5.0297494

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Quantum entanglement is essential for various quantum information technologies that are beyond the possibilities of classical physics. However, it is susceptible to decoherence that may arise from noisy channels and environmental noise. While this deleterious problem has been explored by using filtering techniques, such as photon ancillas and Rydberg atom blockade, a concise yet efficient approach to entanglement retrieval is still a formidable challenge. Here, we present that nonunitary material provides an alternative tool to flexibly control the anomalous Hong–Ou–Mandel (HOM) interference and enables the selective entanglement filter with coherent perfect absorption of anti-symmetric quantum states. An elaborate Cr–SiN–Cr film is prepared as a nonunitary beam splitter such that its tunability over the effective photon–photon interaction in frequency modes can be readily explored in the experiment, which may introduce sophisticated nonunitary realization into integrated optical platforms. In addition, we confirm its ability for selective filtering of high-dimensional frequency entanglement by observing the output quantum state of the conventional HOM interference with a unitary beam splitter and the anomalous HOM interference with a nonunitary beam splitter. These results may offer new insights into investigating the quantum light–matter interaction and facilitating the use of two-photon interference for addressing central challenges in quantum technologies.
Quantum beats, the fact that periodic oscillations arise from coherent superposition of frequency-distinguishable states, have enabled various quantum information technologies beyond the possibilities of classical physics. Although the conventional quantum beats are based on unitary optical elements, we present that nonunitary material provides an alternative degree-of-freedom to control the quantum interference and even enables the observation of anomalous quantum beating signals. An elaborate lossy film is used to explore its tunability over the effective photon–photon interaction in frequency modes, which may introduce sophisticated nonunitary realization into integrated optical platforms. In addition, we confirm its ability of harnessing the suppression and enhancement of single- and two-photon absorption by manipulating the symmetric property of frequency entanglement, and this would provide significant benefits in entanglement-assisted absorption spectroscopy. These results show an alternative method to investigate the quantum light–matter interaction, facilitating the use of two-photon interference for quantum light-based spectroscopy and microscopy.
Hong-Ou-Mandel interference is an intrinsic quantum phenomenon that goes beyond the possibilities of classical physics, and enables numerous applications in quantum information science. While the photon-photon interaction is fundamentally limited to the bosonic nature of photons and the restricted phase responses from commonly used unitary optical elements, we present that a nonunitary material provides an alternative degree of freedom to control the two-photon quantum interference, even revealing anomalous quantum interference paths that do not exist in a unitary configuration. An elaborate lossy multilayer graphene that can work as a nonunitary beam splitter is used to explore its tunability over the effective photon-photon interaction in spatial modes, and to verify the particle exchange statistics by its experimental implementation in quantum state filter. This scheme is further extended to observe four-dimensional quantum interference patterns on the lossless and lossy beam splitters, and thus show its applicability even in higher-dimensional Hilbert space.
Structured photons are a crucial resource in both classical and quantum technologies, particularly in spin–orbit hybrid photons, enabling various practical applications ranging from ultra-sensitive metrology techniques to quantum-enhanced information processing tasks. However, the two-photon interference of spin–orbit hybrid photons, which combines polarization modes and complex transverse spatial structures across the beam profile, remains unexplored. Here, we present an experimental observation of Hong–Ou–Mandel (HOM) interference of spin–orbit hybrid photons. The tunable q-plates that work as spin–orbit coupler devices are used to prepare various forms of spin–orbit hybrid entangled photons. By harnessing the match degree in the temporal domain, the coalescence and anti-coalescence effects resulting from the symmetric and anti-symmetric properties of the incident quantum states are observed. Moreover, we demonstrated the feasibility of quantum-enhanced photon polarization gears through HOM interference and theoretically analyze the noise-resilient advantages based on coherent HOM measurements. These results provide an alternative route toward quantum experiments with structured photons that allows for controlling their quantum interference in a compact, stable, and efficient way.
In the original formulation of the Hong–Ou–Mandel (HOM) experiment, when two otherwise indistinguishable photons are incident upon the two input ports of a balanced beam splitter, they coalesce, always leaving via the same output port. It is often interpreted that this interference arises due to the indistinguishability of the single photons at the beam splitter; the situation, however, is often more nuanced. Here, we demonstrate an analog of HOM interference between two photons of completely different color. To do so, we utilize a quantum frequency converter based on sum- and difference-frequency generation as an “active” beam splitter—coupling frequency-entangled red and telecom single photons with an octave-spanning energy difference of 282 THz. We achieve an uncorrected two-photon interference visibility beyond 90%. This work presents the first demonstration of HOM interference between two single photons of distinctly different color, deepening our understanding of what underlies quantum interference. It also suggests a novel approach to interfacing photonic qubits in heterogeneous quantum systems where frequency conversion and quantum interference are unified.
Two-photon interference effects arise because photons are indistinguishable particles. In the wellknown Hong-Ou-Mandel (HOM) effect, the transmission of two photons at a beam splitter interferes destructively with the reflection of both photons, requiring both photons to "bunch up" by leaving the beam splitter on the same side. Here, we show that the interference between locally propagating photons and photons exchanged by a mode swap can be implemented by post-selecting spatially separated photon outputs of a four-path interferometer. Even though the photons detected at spatially separated locations must have travelled along paths that never met up at the same beam splitter, the Hong-Ou-Mandel effect can be observed in correlations between the output ports that originate from the association of detection events with non-local output modes defined by the two single photon inputs. Local phase shifts can be used to map out non-classical correlations between the photons detected at different output locations, clarifying the role of linear optics in generating entanglement between spatially separated photons. Our work thus establishes a fundamental relation between multiphoton interference and entanglement, opening the door to new possibilities in optical quantum technologies.
Quantum interferometry provides a pivotal method for investigating complex photon-photon interaction, enabling various quantum information technologies that beyond the possibilities of classical physics. While such an effective interaction is mostly studied in N × N unitary transformation, m × n nonunitary transformation that relates to lossy multiport quantum interferometry requires a different approach. Here, we experimentally demonstrate a concise yet powerful tool to unravel fundamental features of multiport quantum interferometry with universal nonunitary transformations. To confirm their intriguing unitary and nonunitary properties, Hong-Ou-Mandel (HOM) interference is observed to reveal its nontrivial particle exchange phase, wherein the conventional HOM interference based on unitary transformation and the anomalous HOM interference based on nonunitary transformation can be readily harnessed. These results provide an alternative approach to investigate the quantum light-matter interaction, facilitating the use of complex multiport quantum interference for large-scale quantum information processing tasks such as quantum simulation and quantum computation.