Single-photon scattering in waveguide-QED systems plays a pivotal role in quantum information processing and communication. We introduce a time-dependent variational approach employing a modified multiple Davydov Ansatz to simulate single-photon dynamics in one-dimensional waveguide-QED systems within the strong-coupling regime. The method is benchmarked across three configurations: a single qubit, two distant qubits, and a ladder-type qutrit coupled to the waveguide. For the single- and two-qubit cases, the variational results exhibit excellent agreement with those derived from a transformed rotating-wave approximation (TRWA). The accuracy of our approach is further verified by an analysis of the local-in-time error, which remains small even under strong coupling, indicating its potential superiority over TRWA in specific regimes. In addition, by contrasting our results with the rotating-wave approximation, we elucidate the significant influence of counter-rotating couplings on scattering dynamics. Our findings establish this variational method as a reliable and versatile tool for investigating single-photon scattering in diverse waveguide-QED systems, particularly in regimes where traditional approximations falter.
Single-photon scattering in waveguide-QED systems plays a pivotal role in quantum information processing and communication. We introduce a time-dependent variational approach employing a modified multiple Davydov Ansatz to simulate single-photon dynamics in one-dimensional waveguide-QED systems within the strong-coupling regime. The method is benchmarked across three configurations: a single qubit, two distant qubits, and a ladder-type qutrit coupled to the waveguide. For the single- and two-qubit cases, the variational results exhibit excellent agreement with those derived from a transformed rotating-wave approximation (TRWA). The accuracy of our approach is further verified by an analysis of the local-in-time error, which remains small even under strong coupling, indicating its potential superiority over TRWA in specific regimes. In addition, by contrasting our results with the rotating-wave approximation, we elucidate the significant influence of counter-rotating couplings on scattering dynamics. Our findings establish this variational method as a reliable and versatile tool for investigating single-photon scattering in diverse waveguide-QED systems, particularly in regimes where traditional approximations falter.
Abstract Recent experiments have pushed the studies on atom–photon interactions to the ultrastrong regime, which motivates the exploration of physics beyond the rotation wave approximation. Here we study the single-photon scattering on a system composed of a coupling cavity array with a two-level atom in the center cavity, which, by varying two outside coupling parameters, corresponds to a model from a supercavity (SC) QED to a waveguide QED with counter rotating wave (CRW) interaction. By applying a time-independent scattering theory based on the bound states in the scattering region, we find that the CRW interaction obviously changes the transmission valley even in the weak atom-cavity coupling regime; in particular, the CRW interaction leads to an inelastic scattering process and a Fano-type resonance, which is directly observed in the crossover from the SC-QED case to the waveguide QED case. Predictably, our findings provide the potential of manipulating the CRW effects in realistic systems and pave the way for the numerical study of very general QED systems.
Developed originally for the Holstein polaron, the Davydov D1 ansatz is an efficient, yet extremely accurate trial state for time-dependent variation of the spin-boson model [N. Wu, L. Duan, X. Li, and Y. Zhao, J. Chem. Phys. 138, 084111 (2013)]. In this work, the Dirac-Frenkel time-dependent variational procedure utilizing the Davydov D1 ansatz is implemented to study entanglement dynamics of two qubits under the influence of two independent baths. The Ohmic spectral density is used without the Born-Markov approximation or the rotating-wave approximation. In the strong coupling regime finite-time disentanglement is always found to exist, while at the intermediate coupling regime, the entanglement dynamics calculated by Davydov D1 ansatz displays oscillatory behavior in addition to entanglement disappearance and revival.
We present a quantum dynamical study of pulsed few-photon scattering from a single artificial atom, consisting of a two-level system (TLS) or qubit, in a waveguide QED system, directly comparing and contrasting two different quantum theoretical simulation methods: (i) an input-output scattering approach that uses frequency-dependent scattering matrices, and (ii) a matrix product states (MPS) approach, which uses quantum noise operators in time bins and a tensor network technique to solve the time-dependent waveguide function for the entire system. Beginning with pulsed excitation using one-photon and two-photon Fock state pulses, we first show how to compute time-dependent observables with the scattering matrix approach, in terms of frequency integrals that encode the pulse spectrum, including how to extract the population dynamics of the excited quantum emitter, as well as the linear and nonlinear contributions. We present solutions for both symmetric and chiral TLS coupling. We then show how to compute the qubit and field observables in a more direct way using MPS, and obtain the characteristic bird-like shape for the two-photon correlation function at two times, which has been observed in recent experiments. We compare and contrast both of these methods, for one and two-photon excitation pulses, and show excellent agreement. We also present a study of the linear and nonlinear contributions, which can easily be calculated using scattering theory, and show the important role of pulse duration. Finally, we demonstrate the clear advantages of MPS by easily going to higher N-photon excitations, and show selected example population dynamics of up to eight-photon Fock-state pulses, manifesting in clear nonlinear population oscillations during the pulse interaction, similar to classical Rabi oscillations, but with quantum input fields that have a vanishing electric field expectation value.
Strong coupling between light and matter has been demonstrated both in classical cavity quantum electrodynamics (QED) systems and in more recent circuit-QED experiments. This enables the generation of strong nonlinear photon-photon interactions at the single-photon level, which is of great interest for the observation of quantum nonlinear optical phenomena, the control of light quanta in quantum information protocols such as quantum networking, as well as the study of strongly correlated quantum many-body systems using light. Recently, strong coupling has also been realized in a variety of one-dimensional (1D) waveguide- QED experimental systems, which in turn makes them promising candidates for quantum information processing. Compared to cavity-QED systems, there are two new features in waveguide-QED: the existence of a continuum of states and the restricted 1D phase space, which together bring in new physical effects, such as the bound-state effects. This thesis consists of two parts: 1) understanding the fundamental interaction between local quantum objects, such as two-level systems and four-level systems, and photons confined in the waveguide; 2) exploring its implications in quantum information processing, in particular photonic quantum computation and quantum key distribution. First, we demonstrate that by coupling a two-level system (TLS) or three/fourlevel system to a 1D continuum, strongly-correlated photons can be generated inside the waveguide. Photon-photon bound states, which decay exponentially as a function of the relative coordinates of photons, appear in multiphoton scattering processes. As a result, photon bunching and antibunching can be observed in the photon-photon correlation function, and nonclassical light source can be generated on demand. In the case of an N-type four-level system, we show that the effective photon-photon interaction mediated by the four-level system, gives rise to a variety of nonlinear optical phenomena, including photon blockade, photon-induced tunneling, and creation of single-photon states and photon pairs with a high degree of spectral entanglement, all in the absence of a cavity. However, to enable greater quantum networking potential using waveguide- QED, it is important to study systems having more than just one TLS/qubit. We develop a numerical Green function method to study cooperative effects in a system of two qubits coupled to a 1D waveguide. Quantum beats emerge in photon-photon correlations, and persist to much longer time scales because of non-Markovian processes. In addition, this system can be used to generate a high-degree of long-distance entanglement when one of the two qubits is driven by an on-resonance laser, further paving the way toward waveguide-QED-based quantum networks. Furthermore, based on our study of light-matter interactions in waveguide- QED, we investigate its implications in quantum information processing. First, we study quantum key distribution using the sub-Possonian single photon source obtained by scattering a coherent state off a two-level system. The rate for key generation is found to be twice as large as for other sources. Second, we propose a new scheme for scalable quantum computation using flying qubits--propagating photons in a one-dimensional waveguide--interacting with matter qubits. Photonphoton interactions are mediated by the coupling to a three- or four-level system, based on which photon-photon -phase gates (Controlled-NOT) can be implemented for universal quantum computation. We show that high gate fidelity is possible given recent dramatic experimental progress in superconducting circuits and photonic-crystal waveguides. The proposed system can be an important building block for future on-chip quantum networks.
We employ the Dirac-Frenkel variational principle and the multiple Davydov ansatz to study time-dependent fluorescence spectra of a driven qubit in the weak to strong qubit-reservoir coupling regimes, where both the Rabi frequency and the spontaneous decay rate are comparable to the transition frequency of the qubit. Our method agrees well with the time-local master-equation approach in the weak coupling regime, and offers a flexible way to compute the spectra from the bosonic dynamics instead of two-time correlation functions. While the perturbative master equation breaks down in the strong coupling regime, our method actually becomes more accurate due to the use of bosonic coherent states under certain conditions. We show that the counter-rotating coupling between the qubit and the reservoir has considerable contributions to the photon number dynamics and the spectra under strong driving conditions even when the coupling is moderately weak. The time-dependent spectra are found to be generally asymmetric, a feature that is derived from photon number dynamics. In addition, it is shown that the spectral profiles can be dramatically different from the Mollow triplet due to strong dissipation and/or multiphoton processes associated with the strong driving. Our formalism provides a unique perspective to interpret time-dependent spectra.
We give an exposure to diagrammatic techniques in waveguide quantum electrodynamics (QED) systems. A particular emphasis is placed on the systems with delayed coherent quantum feedback. Specifically, we show that the N-photon scattering matrices in single-qubit waveguide QED systems, within the rotating wave approximation, admit for a parametrization in terms of ($N\ensuremath{-}1$)-photon effective vertex functions and provide a detailed derivation of a closed hierarchy of generalized Bethe-Salpeter equations satisfied by these vertex functions. The advantage of this method is that the above-mentioned integral equations hold independently of the number of radiation channels, their bandwidth, the dispersion of the modes they are supporting, and the structure of the radiation-qubit coupling interaction, thus enabling one to study multiphoton scattering problems beyond the Born-Markov approximation. Further, we generalize the diagrammatic techniques to the systems containing more than a single emitter by presenting an exact set of equations governing the generic two- and three-photon scattering operators. The above-described theoretical machinery is then showcased on the example of a three-photon scattering on a giant acoustic atom, recently studied experimentally [G. Andersson et al., Nat. Phys. 15, 1123 (2019)].