The integration of elementary quantum objects (atoms, molecules, and quantum dots) with solid-state nanostructures lies at the forefront of nano-optics, nanophotonics, and quantum information science. However, the advancement of this field is hindered by the lack of a rigorous and feasible theoretical framework for describing atom-nanostructure interactions, which are inherently complex and multiparametric. In this work, we develop a theory of light transmission through a zero-mode waveguide (ZMW) containing a single atom. It is shown that the presence of a single atom inside the ZMW can lead to either a significant enhancement or suppression of light transmission, depending on the detuning of the excitation field frequency from the atomic resonance. This extraordinary transmission and blocking effect can be employed for studying the spatiotemporal dynamics of atoms in complex nanoscopic environments, probing quantum optical phenomena, and developing novel nano-optical devices.
The integration of elementary quantum objects (atoms, molecules, and quantum dots) with solid-state nanostructures lies at the forefront of nano-optics, nanophotonics, and quantum information science. However, the advancement of this field is hindered by the lack of a rigorous and feasible theoretical framework for describing atom-nanostructure interactions, which are inherently complex and multiparametric. In this work, we develop a theory of light transmission through a zero-mode waveguide (ZMW) containing a single atom. It is shown that the presence of a single atom inside the ZMW can lead to either a significant enhancement or suppression of light transmission, depending on the detuning of the excitation field frequency from the atomic resonance. This extraordinary transmission and blocking effect can be employed for studying the spatiotemporal dynamics of atoms in complex nanoscopic environments, probing quantum optical phenomena, and developing novel nano-optical devices.
In this work, we develop a theory of light transmission through a Zero-Mode Waveguide (ZMW) containing a single atom. It is shown that the presence of a single atom inside the ZMW can lead to either a significant enhancement or suppression of light transmission, depending on the detuning of the excitation field frequency from the atomic resonance. This extraordinary transmission and blocking effect can be employed for studying the spatiotemporal dynamics of atoms in complex nanoscopic environments, probing quantum optical phenomena, and developing novel nano-optical devices.
An exciting frontier in quantum information science is the integration of otherwise "simple" quantum elements into complex quantum networks. The laboratory realization of even small quantum networks enables the exploration of physical systems that have not heretofore existed in the natural world. Within this context, there is active research to achieve nanoscale quantum optical circuits, for which atoms are trapped near nano-scopic dielectric structures and "wired" together by photons propagating through the circuit elements. Single atoms and atomic ensembles endow quantum functionality for otherwise linear optical circuits and thereby enable the capability of building quantum networks component by component. Toward these goals, we have experimentally investigated three different systems, from conventional to rather exotic systems : free-space atomic ensembles, optical nano fibers, and photonics crystal waveguides. First, we demonstrate measurement-induced quadripartite entanglement among four quantum memories. Next, following the landmark realization of a nanofiber trap, we demonstrate the implementation of a state-insensitive, compensated nanofiber trap. Finally, we reach more exotic systems based on photonics crystal devices. Beyond conventional topologies of resonators and waveguides, new opportunities emerge from the powerful capabilities of dispersion and modal engineering in photonic crystal waveguides. We have implemented an integrated optical circuit with a photonics crystal waveguide capable of both trapping and interfacing atoms with guided photons, and have observed the collective effect, superradiance, mediated by the guided photons. These advances provide an important capability for engineered light-matter interactions, enabling explorations of novel quantum transport and quantum many-body phenomena.
Abstract Complete control of light-matter interactions at a single quantum level is critical for quantum science applications such as precision measurement and information processing. Nanophotonic devices, developed with recent advancements in nanofabrication techniques, can be used to tailor the interactions between single photons and atoms. One example of such a nanophotonic device is the optical nanofibre, which provides an excellent platform due to the strongly confined transverse light fields, long interaction length, low loss, and diverse optical modes. This facilitates a strong interaction between atoms and guided light, revealing chiral atom-light processes and the prospect of waveguide quantum electrodynamics. This paper highlights recent advances, experimental techniques, and future perspectives of the optical nanofibre-atom hybrid quantum platform.
We propose and demonstrate a general mechanism for nanoscale lensing based on the phase gradient imposed by a single nanostructure scattering light in its near-field. We verify this effect using an optical waveguide on a substrate, with single atoms serving as quantum probes that sample the near-field intensity through their fluorescence. This quantum probing technique provides a unique, non-destructive approach to characterizing focused optical fields and reveals a 4-fold enhancement in single atom detection efficiency. This work establishes on-chip nanostructures as a multi-functional quantum optics platform that can efficiently route photons, localize fields, and enhance atom-photon coupling, offering new opportunities for trapping and manipulating single atoms and realizing hybrid nanophotonic-atomic systems for quantum applications.
Techniques to controllably interface atoms with quantum optical fields form the basis for many applications in quantum information science. For example, photons are convenient to relay information over large quantum networks, while atoms naturally are physical systems that can process and store this information. Thus far, the available techniques to efficiently couple single photons with atomic media fall into one of the following, mostly independent, categories: i) cavity quantum electrodynamics (QED), where atomic interactions with light are enhanced via a high-finesse cavity, ii) coherent coupling with atomic ensembles exhibiting large optical depths, and iii) the use of fields tightly focused to dimensions smaller than or approaching the scattering cross-section of a single atom. Although remarkable achievements have been made with all of these approaches, a robust, scalable technique remains elusive. Recently, several groups have successfully demonstrated that cold atoms can be trapped near and interfaced with nanophotonic systems, such as hollow-core photonic crystal fibers [1] and tapered nanofibers [2–4]. The traps are well-characterized [2, 3, 5], and the nearly diffraction-limited transverse confinement of optical fields enables ∼ 10% coupling efficiency of a single atom to the fiber [2, 3]. This has already led to remarkable observations of strong light-matter interactions using relatively few atoms and low powers [1]. It has also been proposed that such techniques can be extended to highly configurable photonic crystal waveguides [6]. Together, these efforts raise the intriguing possibility for future nanophotonic systems with tremendous figures of merit, wherein atom-light interactions can be tailored nearly at will. Here, we discuss recent efforts to develop novel techniques to realize strong, controllable atom-photon and photon-photon interactions, which take full advantage of the parameter space afforded by nanophotonic interfaces and are not based upon the extension of existing techniques. As a specific example, we discuss a protocol to achieve “all-atomic” cavity QED [7], as briefly described below. First, we show that although the single-atom coupling to guided modes of a nanophotonic waveguide might be relatively weak, there exist collective modes of a trapped atomic ensemble whose coupling to light is enhanced by the square root of the atom number, √ NA. While collective effects are generally well-known, special consequences emerge in the nanofiber system when the atoms are trapped in a lattice. In particular, collective effects cause such a lattice to act as a near-perfect mirror for an incident field close to resonance. In analogy to cavity QED, we then demonstrate that two sets of atomic mirrors can form an effective cavity, which can greatly enhance the coupling of a single, specially chosen “impurity” atom (or a few impurity atoms) positioned inside. We introduce a novel quantum spin model to describe the atom-light coupling, which allows one to exactly map the atom-nanofiber interface onto the simple and elegant Jaynes-Cummings model of cavity QED [8]. A unique feature of our atomic mirrors compared to conventional cavities is that they have long relaxation times and are highly dispersive. Remarkably, even with very low mirror finesse (F ∼ 10 2 ), this property allows one to attain the “strong coupling” regime of cavity QED, where vacuum Rabi oscillations [9–12] occur between an excited impurity atom and a single “photon” stored in the cavity (or more precisely, in the atomic mirrors). Furthermore, as quantum mechanical objects, these atom mirrors can be used to store quantum information and transfer this information into propagating waveguide modes. These various features can be combined to realize all of the building blocks for scalable quantum information processing.
Atoms coupled to nanophotonic interfaces represent an exciting frontier for the investigation of quantum light-matter interactions. While most work has considered the interaction between statically positioned atoms and light, here we demonstrate that a wealth of phenomena can arise from the self-consistent interaction between atomic internal states, optical scattering, and atomic forces. We consider in detail the case of atoms coupled to a one-dimensional nanophotonic waveguide and show that this interplay gives rise to the self-organization of atomic positions along the waveguide, which can be probed through distinct characteristics in the reflection and transmission spectra.