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Physical Review A

Saturation of the Cramér-Rao bound for atomic resonance frequency measurements with a phased array of hyperbolic secant pulses

Tharon Holdsworth, Jacob Adamczyk, G. S. Agarwal

Published Aug 26, 2025• 1 citation
Publisher

Abstract

Precise estimation of the atomic resonance frequency is fundamental for the characterization and control of quantum systems. The resonance experiment is a standard method for this measurement, wherein the drive field frequency is swept to invert the system population. We analyze the classical and quantum Fisher information for the resonance experiment driven by hyperbolic-secant-shaped $\ensuremath{\pi}$ pulses, setting a fundamental limit on the precision obtainable using the resonance method. We show that measurements using sequences of pulses with alternating phases nearly saturate the quantum Cram\'er-Rao bound, improving the precision of atomic resonance frequency measurements.

DOI
10.1103/2y17-j6fv

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Precise estimation of the atomic resonance frequency is fundamental for the characterization and control of quantum systems. The resonance experiment is a standard method for this measurement, wherein the drive field frequency is swept to invert the system population. We analyze the classical and quantum Fisher information for the resonance experiment driven by hyperbolic-secant-shaped \ensuremathπ\ensuremath{\pi}\ensuremathπ pulses, setting a fundamental limit on the precision obtainable using the resonance method. We show that measurements using sequences of pulses with alternating phases nearly saturate the quantum Cram'er-Rao bound, improving the precision of atomic resonance frequency measurements.
The quantum Cramer-Rao bound sets a fundamental limit on the accuracy of unbiased parameter estimation in quantum systems, relating the uncertainty in determining a parameter to the inverse of the quantum Fisher information. We experimentally demonstrate near saturation of the quantum Cramer-Rao bound in the phase estimation of a solid-state spin system, provided by a nitrogen-vacancy center in diamond. This is achieved by comparing the experimental uncertainty in phase estimation with an independent measurement of the related quantum Fisher information. The latter is finely extracted from coherent dynamical responses of the system under weak parametric modulations, without performing any quantum-state tomography. Our method offers a versatile and powerful tool to explore the fundamental role of the quantum Fisher information in quantum technologies.
Abstract The quantum Cramér–Rao bound sets a fundamental limit on the accuracy of unbiased parameter estimation in quantum systems, relating the uncertainty in determining a parameter to the inverse of the quantum Fisher information. We experimentally demonstrate near saturation of the quantum Cramér–Rao bound in the phase estimation of a solid-state spin system, provided by a nitrogen-vacancy center in diamond. This is achieved by comparing the experimental uncertainty in phase estimation with an independent measurement of the related quantum Fisher information. The latter is independently extracted from coherent dynamical responses of the system under weak parametric modulations, without performing any quantum-state tomography. While optimal parameter estimation has already been observed for quantum devices involving a limited number of degrees of freedom, our method offers a versatile and powerful experimental tool to explore the Cramér–Rao bound and the quantum Fisher information in systems of higher complexity, as relevant for quantum technologies.
Precision measurements with quantum systems rely on our ability to trace the differences between experimental signals to variations in unknown physical parameters. In this Letter we derive the Fisher information and the ensuing Cramér-Rao sensitivity limit for parameter estimation by continuous measurements on an open quantum system. We illustrate our theory by its application to resonance fluorescence from a laser-driven two-state atom; we show that photon counting and homodyne detection records yield different sensitivity to the atomic parameters, while none of them exceed our general result.
The field of quantum metrology seeks to apply quantum techniques and/or resources to classical sensing approaches with the goal of enhancing the precision in the estimation of a parameter beyond what can be achieved with classical resources. Theoretically, the fundamental minimum uncertainty in the estimation of a parameter for a given probing state is bounded by the quantum Cramér-Rao bound. From a practical perspective, it is necessary to find physical measurements that can saturate this fundamental limit and to show experimentally that it is possible to perform measurements with the required precision to do so. Here we perform experiments that saturate the quantum Cramér-Rao bound for transmission estimation over a wide range of transmissions when probing the system under study with a continuous wave bright two-mode squeezed state. To properly take into account the imperfections in the generation of the quantum state, we extend our previous theoretical results to incorporate the measured properties of the generated quantum state. For our largest transmission level of 84%, we show a 62% reduction over the optimal classical protocol in the variance in transmission estimation when probing with a bright two-mode squeezed state with -8 dB of intensity-difference squeezing. Given that transmission estimation is an integral part of many sensing protocols, such as plasmonic sensing, spectroscopy, calibration of the quantum efficiency of detectors, etc., the results presented promise to have a significant impact on a number of applications in various fields of research.
Abstract Quantum metrology aims at delivering new quantum-mechanical improvement to technologies of parameter estimations with precision bounded by the quantum Cramér-Rao bound. The currently used quantum Cramér-Rao bound was established with measurements of observables restricted to be Hermitian. This constrains the bound and limits the precision of parameter estimation. In this paper, we lift the constraint and derive a previously unknown quantum Cramér-Rao bound. We find that the new bound can reach arbitrary small value with mixed states and it breaks the Heisenberg limit in some cases. We construct a setup to measure non-Hermitian operators and discuss the saturation of the present bound. Two examples—the phase estimation with Greenberger-Horne-Zeilinger states of trapped ions and the adiabatic quantum parameter estimation with the nuclear magnetic resonance—are employed to demonstrate the theory. The present study might open a new research direction—non-Hermitian quantum metrology.
The quantum Fisher information constrains the achievable precision in parameter estimation via the quantum Cramér-Rao bound, which has attracted much attention in Hermitian systems since the 60s of the last century. However, less attention has been paid to non-Hermitian systems. In this Letter, working with different logarithmic operators, we derive two previously unknown expressions for quantum Fisher information, and two Cramér-Rao bounds lower than the well-known one are found for non-Hermitian systems. These lower bounds are due to the merit of non-Hermitian observable and it can be understood as a result of extended regimes of optimization. Two experimentally feasible examples are presented to illustrate the theory, saturation of these bounds and estimation precisions beyond the Heisenberg limit are predicted and discussed. A setup to measure non-Hermitian observable is also proposed.