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Physical Review Applied

Spin-flip two-level-system-induced anomalous magnetic field properties in thin-film superconducting resonators

Zi-Qing Huang, Shu-Kun Ye, Yong-Qiang Xu, Tian-Yi Jiang, Tianzheng Hao, Bao‐Chuan Wang, Xiang‐Xiang Song, Haiou Li, Guang‐Can Guo, Gang Cao, Guo‐Ping Guo

Published Aug 27, 2025• 1 citation
Publisher
DOI
10.1103/5k9f-7gc7

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cond-mat.str-elCross-listedarXiv:2603.14545•Mar 17, 2026
Material disorders are one of the major sources of noise and loss in solid-state quantum devices, whose behaviors are often modeled as two-level systems (TLSs) formed by charge tunneling between neighboring sites. However, the role of their spins in tunneling and its impact on device performance remain highly unexplored. In this work, employing ultra-thin TiN superconducting resonators, we reveal anomalous TLS behaviors by demonstrating an unexpected increase in resonant frequency at low magnetic fields. Furthermore, a spin-flip TLS model is proposed, in which an effective spin-orbit coupling is generated by inhomogeneous local magnetic fields from defect spins. This mechanism mixes charge tunnelings and spin flips, quantitatively reproducing the observed frequency-field relationship and its temperature dependence. This work deepens the understanding of spin-dependent TLS behaviors, offering the possibility of magnetically engineering noise and loss in solid-state quantum devices.
In a recent paper [Phys. Rev. Lett. 97, 070401 (2006)] the transition rate of magnetic spin-flip of a neutral two-level atom trapped in the vicinity of a thick superconducting body was studied. In the present paper we will extend these considerations to a situation with an atom at various distances from a dielectric film. Rates for the corresponding electric dipole-flip transition will also be considered. The rates for these atomic flip transitions can be reduced or enhanced, and in some situations they can even be completely suppressed. For a superconducting film or a thin film of a perfect conducting material various analytical expressions are derived that reveals the dependence of the physical parameters at hand.
Minimizing the energy of a many body system tends to favor order, but classical frustration and quantum fluctuations destabilize that order. The tension between these effects can produce exotic quantum states of matter. Quantum spin liquid (QSL) states emerge in models of localized magnetic moments where the crystal lattice connectivity frustrates ordering, and the exchange interaction of neighboring spins strengthens quantum fluctuations. Experimentally identifying a QSL in a real material is challenging from the lack of an order parameter. Piecing together evidence from varied techniques is necessary for diagnosing the nature of the ground state -- QSL or otherwise -- of a frustrated spin system. In this work, we use coplanar superconducting resonators to probe magnetic excitations in epitaxially grown thin films of a spin liquid candidate TbInO3. Adapting microwave techniques from the field of circuit quantum electrodynamics, we measure responses of these thin films whose volume is too low for applying conventional bulk techniques. In-plane susceptibility extracted from the spin resonance signal indicates extreme frustration of magnetic order down to 20 mK, over two orders of magnitude lower than the Curie-Weiss energy scale. Through a crystal field analysis, we identify the doublet eigenstates comprising the ground state. As a consequence of improper ferroelectricity, Tb moments split into two flavors with distinct g-factors reflecting the local crystal field environment of each site. Spin-orbit coupling, crystal fields, magnetic frustration and improper ferroelectricity distinctively combine to shape the magnetic ground state of TbInO3. This work establishes a measurement technique using superconducting resonators to probe thin films of frustrated magnets, and applies this technique towards building a coherent understanding of the magnetic properties of TbInO3.