Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Optica

Visualizing strongly focused 3D light fields in an atomic vapor

Sphinx J. Svensson, Clare R. Higgins, Danielle Pizzey, Ifan G. Hughes, Sonja Franke‐Arnold

Published Aug 29, 2025• 5 citations
Publisher

Abstract

Structured light, when strongly focused, generates highly confined vectorial electromagnetic field distributions, which may feature a polarization component along the optical axis. Manipulating and detecting such 3D light fields is challenging, as conventional optical elements and detectors do not interact with the axial polarization component. Vector light can, however, be mapped onto atomic polarizations, making electric dipole transitions an ideal candidate to sense such 3D light configurations. Working in the hyperfine Paschen–Back regime, where the electric dipole transitions are spectrally resolved, we demonstrate direct evidence of the axial polarization component of strongly focused radial light. We investigate the influence of various input polarization states, including radial, azimuthal, and higher-order optical vortices, on atomic absorption profiles. Our results confirm a clear mapping between the 3D vector light and the atomic transition strength. This work provides insights into vectorial light–matter interaction and opens avenues for quantum sensing applications.

DOI
10.1364/optica.568785

Related papers

Visualizing strongly focused 3D light fields in an atomic vapor

Sphinx J. Svensson, Clare R. Higgins, Danielle Pizzey +2 more

Structured light, when strongly focused, generates highly confined vectorial electromagnetic field distributions which may feature a polarization component along the optical axis. Manipulating and detecting such 3D light fields is challenging, as conventional optical elements and detectors do not interact with the axial polarization component. Vector light can, however, be mapped onto atomic polarizations, making electric dipole transitions an ideal candidate to sense such 3D light configurations. Working in the hyperfine Paschen-Back regime, where the electric dipole transitions are spectrally resolved, we demonstrate direct evidence of the axial polarization component of strongly focused radial light. We investigate the influence of various input polarization states, including radial, azimuthal, and higher-order optical vortices, on atomic absorption profiles. Our results confirm a clear mapping between the 3D vector light and the atomic transition strength. This work provides new insights into vectorial light-matter interaction, and opens avenues for novel quantum sensing applications.

arXiv:2506.01680•Jun 2, 2025•0 citations

Transformation of vector modes by the Faraday effect in strong magnetic fields

Sphinx J. Svensson, Craig J. A. Millar, Danielle Pizzey +2 more

Large Faraday rotations can be generated by circular birefringence of atomic samples in an axial magnetic field in the vicinity of atomic resonance lines. More generally, magneto-optical effects in atomic samples include circular dichroism in addition to birefringence, resulting in a modification of the ellipticity as well as the polarization alignment. Usually such effects are investigated for homogeneous linear polarizations, but the mechanisms apply also to polarization structures such as vector vortices. We investigate the effect of optical activity of a rubidium vapor in the hyperfine Paschen–Back regime along the D2 line, for the example of azimuthally polarized input light. We show that for low atomic densities, circular birefringence dominates over dichroism, and azimuthal polarization is rotated toward radial polarization. The rotation angle increases with increasing optical densities. At high vapor temperatures, dichroism becomes more and more relevant, leading to intricate variations of both alignment and ellipticity. Our results shine new light on the interplay between different magneto-optic effects at strong magnetic fields. Their highly sensitive response to detuning may find applications in spectroscopy and quantum sensing.

arXiv:2607.15088•Journal of the Optical Society of America B•Sep 4, 2026•0 citations

Unambiguous vector magnetometry with structured light in atomic vapor

Seeram Ramakrishna, S. Fritzsche

Absorption profiles of vector light upon interaction with atomic vapor carries distinct signatures of an external magnetic field vector. However, this signature becomes ambiguous for antiparallel magnetic field vectors of equal magnitude, which makes their absorption profiles visually indistinguishable. To resolve this ambiguity, we present a theoretical analysis of the interaction of vector light with optically polarized atoms immersed in reference and test magnetic fields. Furthermore, we demonstrate the complete characterization of the arbitrarily oriented test magnetic field via a Fourier analysis of the absorption profile. This analysis reveals a one-to-one correspondence between the magnetic field properties and the profile's contrast and rotational angle. Our findings open an avenue to design an optical vector atomic magnetometer based on structured light fields.

arXiv:2601.22998•Physical Review A•Mar 4, 2026•1 citation

Trapped atoms in spatially-structured vector light fields

Maurizio Verde, Christian Tomás Schmiegelow, Ulrich Poschinger +1 more

Spatially-structured laser beams, eventually carrying orbital angular momentum, affect electronic transitions of atoms and their motional states in a complex way. We present a general framework, based on the spherical tensor decomposition of the interaction Hamiltonian, for computing atomic transition matrix elements for light fields of arbitrary spatial mode and polarization structures. We study both the bare electronic matrix elements, corresponding to transitions with no coupling to the atomic center-of-mass motion, as well as the matrix elements describing the coupling to the quantized atomic motion in the resolved side-band regime. We calculate the spatial dependence of electronic and motional matrix elements for tightly focused Hermite-Gaussian, Laguerre-Gaussian and for radially and azimuthally polarized beams. We show that near the diffraction limit, all these beams exhibit longitudinal fields and field gradients, which strongly affect the selection rules and could be used to tailor the light-matter interaction. The presented framework is useful for describing trapped atoms or ions in spatially-structured light fields and therefore for designing new protocols and setups in quantum optics, -sensing and -information processing. We provide open code to reproduce our results or to evaluate interaction matrix elements for different transition types, beam structures and interaction geometries.

arXiv:2306.17571•Scientific Reports•Dec 2, 2023•21 citations

Nonlinear Quantum Optics With Structured Light: Tightly Trapped Atoms in the 3D Focus of Vectorial Waves

R. Gutiérrez-Jáuregui, Rocío Jáuregui

Atomic gases tightly trapped near the focus of an electromagnetic wave interact with photons that exhibit a complex structure, displaying strong gradients of field amplitude and local polarization that can lead to topological phase singularities. We illustrate the consequences of this structure on a paradigmatic nonlinear optical process: three-wave mixing. The process begins by proper selection of the pump field, whose spatial structure is tailored to present huge gradients of the EM field that enhance atomic excitations through forbidden transitions. Atoms can then be depopulated via two electric dipole decays in a cascade configuration, thus providing the three necessary waves. The properties of the down-converted photons are conditioned to those of the pump field through phase matching conditions. It is emphasized that the expression of the photons must incorporate both the structure of the vectorial EM modes and the spatial configuration of the atomic trap. Due to the three-dimensional focusing, the slowly varying envelope approximation becomes inadequate when describing the scattered EM field. We discuss an alternative using a Green function formalism valid for any configuration of the field that also allows to identify the phase matching conditions. Spherical vectorial waves exemplify most concepts here discussed, including the possibility of observing nonlinear quantum phenomena at the single photon level.

Frontiers in Physics•Jun 16, 2022•3 citations

Visualization of magnetic fields with cylindrical vector beams in a warm atomic vapor

Shuwei Qiu, Jinwen Wang, Francesco Castellucci +6 more

We propose and demonstrate an experimental implementation for the observation of magnetic fields from spatial features of absorption profiles in a warm atomic vapor. A radially polarized vector beam that traverses atomic vapor will generate an absorption pattern with a petal-like structure by the mediation of a transverse magnetic field (TMF). The spatial absorption pattern rotates when the azimuthal angle of the TMF is changed, while its contrast decreases when the longitudinal component of the magnetic field increases. By analyzing the intensity distribution of the transmitted pattern, we can determine the magnetic field strength. Our work provides a framework for investigating 3D magnetic field distributions based on atoms.

arXiv:2109.14405•Photonics Research•Sep 29, 2021•36 citations
Structured light, when strongly focused, generates highly confined vectorial electromagnetic field distributions, which may feature a polarization component along the optical axis. Manipulating and detecting such 3D light fields is challenging, as conventional optical elements and detectors do not interact with the axial polarization component. Vector light can, however, be mapped onto atomic polarizations, making electric dipole transitions an ideal candidate to sense such 3D light configurations. Working in the hyperfine Paschen–Back regime, where the electric dipole transitions are spectrally resolved, we demonstrate direct evidence of the axial polarization component of strongly focused radial light. We investigate the influence of various input polarization states, including radial, azimuthal, and higher-order optical vortices, on atomic absorption profiles. Our results confirm a clear mapping between the 3D vector light and the atomic transition strength. This work provides insights into vectorial light–matter interaction and opens avenues for quantum sensing applications.
Structured light, when strongly focused, generates highly confined vectorial electromagnetic field distributions which may feature a polarization component along the optical axis. Manipulating and detecting such 3D light fields is challenging, as conventional optical elements and detectors do not interact with the axial polarization component. Vector light can, however, be mapped onto atomic polarizations, making electric dipole transitions an ideal candidate to sense such 3D light configurations. Working in the hyperfine Paschen-Back regime, where the electric dipole transitions are spectrally resolved, we demonstrate direct evidence of the axial polarization component of strongly focused radial light. We investigate the influence of various input polarization states, including radial, azimuthal, and higher-order optical vortices, on atomic absorption profiles. Our results confirm a clear mapping between the 3D vector light and the atomic transition strength. This work provides new insights into vectorial light-matter interaction, and opens avenues for novel quantum sensing applications.
Large Faraday rotations can be generated by circular birefringence of atomic samples in an axial magnetic field in the vicinity of atomic resonance lines. More generally, magneto-optical effects in atomic samples include circular dichroism in addition to birefringence, resulting in a modification of the ellipticity as well as the polarization alignment. Usually such effects are investigated for homogeneous linear polarizations, but the mechanisms apply also to polarization structures such as vector vortices. We investigate the effect of optical activity of a rubidium vapor in the hyperfine Paschen–Back regime along the D2 line, for the example of azimuthally polarized input light. We show that for low atomic densities, circular birefringence dominates over dichroism, and azimuthal polarization is rotated toward radial polarization. The rotation angle increases with increasing optical densities. At high vapor temperatures, dichroism becomes more and more relevant, leading to intricate variations of both alignment and ellipticity. Our results shine new light on the interplay between different magneto-optic effects at strong magnetic fields. Their highly sensitive response to detuning may find applications in spectroscopy and quantum sensing.
Absorption profiles of vector light upon interaction with atomic vapor carries distinct signatures of an external magnetic field vector. However, this signature becomes ambiguous for antiparallel magnetic field vectors of equal magnitude, which makes their absorption profiles visually indistinguishable. To resolve this ambiguity, we present a theoretical analysis of the interaction of vector light with optically polarized atoms immersed in reference and test magnetic fields. Furthermore, we demonstrate the complete characterization of the arbitrarily oriented test magnetic field via a Fourier analysis of the absorption profile. This analysis reveals a one-to-one correspondence between the magnetic field properties and the profile's contrast and rotational angle. Our findings open an avenue to design an optical vector atomic magnetometer based on structured light fields.
Spatially-structured laser beams, eventually carrying orbital angular momentum, affect electronic transitions of atoms and their motional states in a complex way. We present a general framework, based on the spherical tensor decomposition of the interaction Hamiltonian, for computing atomic transition matrix elements for light fields of arbitrary spatial mode and polarization structures. We study both the bare electronic matrix elements, corresponding to transitions with no coupling to the atomic center-of-mass motion, as well as the matrix elements describing the coupling to the quantized atomic motion in the resolved side-band regime. We calculate the spatial dependence of electronic and motional matrix elements for tightly focused Hermite-Gaussian, Laguerre-Gaussian and for radially and azimuthally polarized beams. We show that near the diffraction limit, all these beams exhibit longitudinal fields and field gradients, which strongly affect the selection rules and could be used to tailor the light-matter interaction. The presented framework is useful for describing trapped atoms or ions in spatially-structured light fields and therefore for designing new protocols and setups in quantum optics, -sensing and -information processing. We provide open code to reproduce our results or to evaluate interaction matrix elements for different transition types, beam structures and interaction geometries.
Atomic gases tightly trapped near the focus of an electromagnetic wave interact with photons that exhibit a complex structure, displaying strong gradients of field amplitude and local polarization that can lead to topological phase singularities. We illustrate the consequences of this structure on a paradigmatic nonlinear optical process: three-wave mixing. The process begins by proper selection of the pump field, whose spatial structure is tailored to present huge gradients of the EM field that enhance atomic excitations through forbidden transitions. Atoms can then be depopulated via two electric dipole decays in a cascade configuration, thus providing the three necessary waves. The properties of the down-converted photons are conditioned to those of the pump field through phase matching conditions. It is emphasized that the expression of the photons must incorporate both the structure of the vectorial EM modes and the spatial configuration of the atomic trap. Due to the three-dimensional focusing, the slowly varying envelope approximation becomes inadequate when describing the scattered EM field. We discuss an alternative using a Green function formalism valid for any configuration of the field that also allows to identify the phase matching conditions. Spherical vectorial waves exemplify most concepts here discussed, including the possibility of observing nonlinear quantum phenomena at the single photon level.
We propose and demonstrate an experimental implementation for the observation of magnetic fields from spatial features of absorption profiles in a warm atomic vapor. A radially polarized vector beam that traverses atomic vapor will generate an absorption pattern with a petal-like structure by the mediation of a transverse magnetic field (TMF). The spatial absorption pattern rotates when the azimuthal angle of the TMF is changed, while its contrast decreases when the longitudinal component of the magnetic field increases. By analyzing the intensity distribution of the transmitted pattern, we can determine the magnetic field strength. Our work provides a framework for investigating 3D magnetic field distributions based on atoms.