High-dimensional quantum entanglement in photons offers significant advantages in quantum technologies, including enhanced information capacity and improved security in communication protocols [1]. However, when entangled photons propagate through complex media-such as turbulent atmospheres or multimode fibers-their spatial correlations degrade, limiting their practical utility [2]. While the effects of disorder near the nonlinear crystal generating entangled photons are well understood [3], the impact of disorder in the far field remains less explored. We have systematically investigated the impact of arbitrary phase distortions in the far field by decomposing the disorder into even- and odd-parity components [4]. Through theoretical analysis, we have demonstrated that only the even-parity component affects two-photon interference, while the odd-parity component leaves photon correlations unchanged, as shown in Fig. 1. To validate this prediction, we used a deformable mirror to introduce controlled phase distortions and experimentally confirm our findings. Additionally, numerical simulations showed that these results hold even for more complex disorders.
High-dimensional quantum entanglement in photons offers significant advantages in quantum technologies, including enhanced information capacity and improved security in communication protocols [1]. However, when entangled photons propagate through complex media-such as turbulent atmospheres or multimode fibers-their spatial correlations degrade, limiting their practical utility [2]. While the effects of disorder near the nonlinear crystal generating entangled photons are well understood [3], the impact of disorder in the far field remains less explored. We have systematically investigated the impact of arbitrary phase distortions in the far field by decomposing the disorder into even- and odd-parity components [4]. Through theoretical analysis, we have demonstrated that only the even-parity component affects two-photon interference, while the odd-parity component leaves photon correlations unchanged, as shown in Fig. 1. To validate this prediction, we used a deformable mirror to introduce controlled phase distortions and experimentally confirm our findings. Additionally, numerical simulations showed that these results hold even for more complex disorders.
High-dimensional quantum entanglement in photons offers notable technological advancements over traditional qubit-based systems, including increased information density and enhanced security. However, such high-dimensional states are vulnerable to disruption by complex disordered media, presenting significant challenges in practical applications. Spatially entangled photons are conventionally generated using a nonlinear crystal via spontaneous parametric downconversion. While the effect of disorder on spatially entangled photons in the near field of the crystal is well understood, the impact of disorder in the far field is more complex. In this work, we present a systematic study of the randomization of two-photon correlations caused by arbitrary phase distortions in the far field by breaking it down into odd and even parity components. First, we theoretically show that the two-photon field is only sensitive to the even-parity part of the phase distortion. In follow-up experiments, we employ a deformable mirror to implement random phase distortions, separating the contributions of odd and even parity phases using Zernike polynomials. The experimental results are in agreement with the theoretical predictions. Subsequently, we perform numerical simulations to show that these results extend to stronger degrees of disorder. Our key finding is that, since two-photon correlations are only affected by the even-parity component of phase modulations, the number of independent adaptive optics elements required for optimizing the correlation can be effectively halved, offering a significant practical advantage in managing disorder in quantum systems.
Wavefront shaping enables control of classical light through scattering media. Extending these techniques to spatially entangled photons promises new quantum applications, but their fundamental limits, especially when both photons scatter, remain unclear. Here, we theoretically and numerically investigate the enhancement of two-photon correlations through thick scattering media. We analyze configurations where a spatial light modulator shapes one or both photons, either before or after the medium, and show that the optimal enhancement differs fundamentally from classical expectations. For a system with N modes, we show that shaping one photon yields the classical enhancement η≈(π/4)N, while shaping both photons before the medium reduces it to η≈(π/4)2N. However, in some symmetric detection schemes, when both photons are measured at the same mode, perfect correlations are restored with η≈N, resembling digital optical phase conjugation. Conversely, shaping both photons after the medium leads to a complex, NP-hard-like optimization problem, yet achieves superior enhancements, up to η≈4.6N. These results reveal unique quantum effects in complex media and identify strategies for quantum imaging and communication through scattering environments.
Wavefront shaping enables control of classical light through scattering media. Extending these techniques to spatially entangled photons promises new quantum applications, but their fundamental limits, especially when both photons scatter, remain unclear. Here, we theoretically and numerically investigate the enhancement of two-photon correlations in two specific output modes through thick scattering media. We analyze three configurations: shaping one photon after the medium, shaping both photons before the medium, and shaping both photons after the medium. We show that each configuration yields fundamentally different enhancements compared to classical expectations. For a system with N modes, we show that shaping one photon yields the classical enhancement η ≈ (π/4)N, while shaping both photons before the medium reduces it to η ≈ (π/4)2N. However, in some symmetric detection schemes, when both photons are measured at the same mode, perfect correlations are restored with η ≈ N, resembling digital optical phase conjugation. Conversely, shaping both photons after the medium leads to a complex, NP-hard-like optimization problem, yet achieves superior enhancements, up to η ≈ 4.6N. These results reveal unique quantum effects in complex media and identify strategies for quantum imaging and communication through scattering environments.
High-dimensional entanglement in the form of transverse spatial correlation between a pair of photons generated via spontaneous parametric downconversion is not only a valuable resource in many academic and real-life applications but also provides access to several intriguing quantum phenomena. One such non-intuitive phenomenon is phase entanglement, in which the biphoton state is correlated in the complex phase of its wavefunction. This state, which emerges during the propagation of the biphoton wavefunction, exhibits neither position nor momentum correlation, yet retains full entanglement. In this work, we experimentally explore this state in two distinct ways. The first is by tracking the vanishing spatial photon number correlation over propagation distances lying in [0,∞), folded into a finite range using single-lens imaging. These observations show excellent agreement with our theoretical predictions based on the Double Gaussian (DG) approximation of the biphoton state. The second approach involves performing a two-photon interference experiment using a double slit and this state, which reveals the correlated phase front. We show, both theoretically and experimentally, that the observed two-photon interference structure is markedly different from that produced by position-correlated photons, as confirmed by computing the joint probability distribution of photons (JPD) and related metrics. Such interference using phase-entangled light has not been attempted before and opens avenues for advanced experiments and applications in the field of spatial entanglement.
Understanding the complex interactions of the quantum light with different media provides valuable insights into potential applications in quantum tomography, microscopy, circuit and network design, and imaging. This thesis investigates quantum light interaction with two types of media: I. Random media entailing multiple scattering (Chapters 2-5), and II. Structured media, specifically designed to control quantum interferences (Chapters 6 and 7). In the first part of the thesis, and through solving the Lippmann-Schwinger equation for collections of small scatterers, a first principle scalar model for multiple scattering in finite-sized random media is developed. This efficient numerical model serves as the basis for investigating the coherent backscattering, a manifestation of weak localization in random media, for several bounded random media and various illuminations. Through employing mode expansion, next, the developed model is adapted to a general class of quantum-optical studies and quantum correlations are successfully derived and analyzed in scattering from finite disordered structures as well as systems of few scatterers. In multiple scattering of two-photon states in weak localization regime, the emergence of coherent two-photon backscattering is presented for the first time in coincidence detection, and it is demonstrated that quantum correlations can be used as a probe of entanglement dimensionality. Multiple scattering of two-photon states results in granular patterns known as speckle patterns. The statistical properties of single- and two-photon speckle patterns in scattering of different states are numerically calculated and the speckle visibilities and relevant parameters are derived. Specifically, the deviation of the probability density functions from negative exponential distributions, traditionally recognized as Rayleigh statistics in classical scattering, is identified, and shown to significantly depend on the presence of entanglement. Lastly, a different numerical implementation (based on COMSOL Multiphysics package) is used to consolidate our findings by incorporating the polarization effects. Coherent backscattering and coherent two-photon backscattering are observed for co-polarized fields in scattering from synthesized disordered media. It is demonstrated that depending on the particle exchange symmetry in polarization entangled excitation, the photons can exhibit statistical tendency to bunch together in the same mode, appear in separate modes (antibunching), or show a mixed response after multiple scattering. These bosonic-, fermionic-, and anyonic-like behaviors are studied in connection with coherent backscattering phenomenon, and it is demonstrated that the degree of enhancement in backscattering depends on the exchange symmetries. The simplicity and effectiveness of the implemented scattering analysis and the significance of the consequent conclusions suggest our approach as a promising platform for ‘numerical experiments’ without the limitations of analytical or semi-analytical models, and a practical tool prior to experiments. In the second part of the thesis, the random media operating as multimode platforms are replaced with engineered surfaces, i.e., metasurfaces, to realize targeted quantum interferences. First, a design roadmap for general lossy, asymmetric, and unbalanced coupling networks is presented, allowing to achieve maximum programmability in two-photon interferences. Next, two switchable metasurface-based coupling networks are designed to control nonclassical two-photon interferences via thermally driven crystallographic phase transitions. Numerical simulations confirm smooth transition between coalescence and anti-coalescence, aiming to address the current need in quantum optics for free-space compact devices creating tunable quantum interferences and acting as fast modulators for the second order quantum correlations. Our proposed compact and rapidly controllable devices pave the way towards new quantum applications as well as improving the current free-space quantum systems.
Spatial entanglement is a key resource in quantum technologies, enabling applications in quantum communication, imaging, and computation. However, propagation through complex media distorts spatial correlation, posing a challenge for practical implementations. We introduce a symmetrized genetic algorithm (sGA) for adaptive wavefront correction of spatially entangled photons, leveraging the insight that only the even-parity component of wavefront distortions affects two-photon correlation. By enforcing symmetry constraints, sGA reduces the optimization parameter space by half, leading to faster convergence and improved enhancement within a finite number of generations compared to standard genetic algorithms. In addition, we establish the dependence of enhancement on the signal-to-noise ratio of the feedback signal, which is controlled by detector integration time. This technique enables correction of entanglement degradation, enhancing quantum imaging, secure quantum communication, and quantum sensing in complex environments.