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Journal of Physics B Atomic Molecular and Optical Physics

Effects of counter-rotating couplings in bichromatically driven three-level V-type systems

Yiying Yan, Zhiguo Lü, Hang Zheng

Published Aug 13, 2025• 1 citation
Publisher

Abstract

Abstract We study the resonance and dynamics of a three-level V-type system strongly driven by a quasiperiodic bichromatic field by making use of a unitary-transformation (UT) method. The UT is used to construct a periodic effective Hamiltonian which incorporates the effects of counter-rotating couplings and takes a physically transparent form, and the Floquet theory is used to calculate transition probabilities. By comparing the UT results with those from the rotating-wave approximation (RWA) and generalized Floquet theory, we illustrate that the UT method captures not only accurate resonance structures but also dynamics of the driven V system in a strong-driving regime where the RWA breaks down. We show that there are two dynamical features, namely, peak-dip structures and beat behaviors, which are ascribed to a time-dependent coupling between the two upper levels due to the counter-rotating terms and cannot be described by a RWA Hamiltonian. Moreover, we show that the effective Hamiltonian can be used to calculate higher-order Bloch–Siegert shifts, which is another feature caused by the counter-rotating terms. Present work offers insights into the role of counter-rotating couplings in a bichromatically driven three-level system.

DOI
10.1088/1361-6455/adfb16

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Abstract We study the resonance and dynamics of a three-level V-type system strongly driven by a quasiperiodic bichromatic field by making use of a unitary-transformation (UT) method. The UT is used to construct a periodic effective Hamiltonian which incorporates the effects of counter-rotating couplings and takes a physically transparent form, and the Floquet theory is used to calculate transition probabilities. By comparing the UT results with those from the rotating-wave approximation (RWA) and generalized Floquet theory, we illustrate that the UT method captures not only accurate resonance structures but also dynamics of the driven V system in a strong-driving regime where the RWA breaks down. We show that there are two dynamical features, namely, peak-dip structures and beat behaviors, which are ascribed to a time-dependent coupling between the two upper levels due to the counter-rotating terms and cannot be described by a RWA Hamiltonian. Moreover, we show that the effective Hamiltonian can be used to calculate higher-order Bloch–Siegert shifts, which is another feature caused by the counter-rotating terms. Present work offers insights into the role of counter-rotating couplings in a bichromatically driven three-level system.
Abstract The resonance and dynamics of a qubit exposed to a strong aperiodic bichromatic field are studied by using a periodic counter‐rotating hybridized rotating wave (CHRW) Hamiltonian, which is derived from the original Hamiltonian with the unitary transformations under a reasonable approximation and enables the application of the Floquet theory. It is found that the consistency between the CHRW results and numerically exact generalized‐Floquet‐theory (GFT) results in the valid regime of the former while the widely used rotating‐wave approximation breaks down. It is illustrated that the resonance exhibits band structure and the Bloch–Siegert shifts induced by the counter‐rotating couplings of the bichromatic field become notable at the multiphoton resonance band. In addition, the CHRW method is found to have a great advantage of efficiency over the GFT approach particularly in the low beat‐frequency case where the latter converges very slowly. The present CHRW method provides a highly efficient way to calculate the resonance frequency incorporating the Bloch–Siegert shift and provides insights into the effects of the counter‐rotating couplings of the bichromatic field in the strong‐driving regimes.
We theoretically study the dynamics and resonance shift of the Rabi model with frequency modulation, i.e., the Rabi model driven additionally by a slow longitudinal field, by using the counterrotating-hybridized rotating-wave (CHRW) method, aiming to illustrate the effects of the counterrotating (CR) terms of the transverse field. The CHRW method is based on a unitary transformation and reduces the aperiodic Hamiltonian to an effective periodic Hamiltonian that can be efficiently treated by Floquet theory. The validity of the effective Hamiltonian and widely used rotating-wave approximation (RWA) Hamiltonian is carefully examined compared to the numerically exact results over a wide parameter range. It is found that the effective Hamiltonian gives a correct description, while the RWA breaks down in the strong driving regime. Interestingly, we show that under certain conditions the longitudinal field can be used to modify resonance widths such that resonance widths can be comparable to the magnitude of the Bloch-Siegert (BS) shift, which in turn makes the CR-induced BS shift significant and leads to the complete breakdown of the RWA even in a moderately strong driving regime (in which the RWA holds for the Rabi model without frequency modulation). In addition, by using the effective Hamiltonian, we can efficiently access resonance positions for the bichromatically driven qubit and study how the resonance shifts due to the combined effects of the CR terms and frequency modulation. For a weak longitudinal field, we show that resonance positions can be analytically calculated from the effective Rabi frequency for the effective Hamiltonian, which are in excellent agreement with the numerically exact results.
We study the fluorescence spectrum of a strongly driven two-level system (TLS) with modulated transition frequency, which is a bichromatically driven TLS and has multiple resonance frequencies. We are aiming to provide a reliable description of the fluorescence in a regime that is difficult to tackle with perturbation theory and the rotating-wave approximation (RWA), and illustrate the spectral features of the fluorescence under off- and multiphoton-resonance conditions. To go beyond the RWA, we use a semianalytical counter-rotating-hybridized rotating-wave method that combines a unitary transformation and Floquet theory to calculate the two-mode Floquet states and quasienergies for the bichromatically driven TLS. We then solve the master equation accounting for the spontaneous decay in the bases of the two-mode Floquet states, and derive a physically transparent fluorescence spectrum. In comparison with the numerically exact spectrum from the generalized Floquet-Liouville approach, the present spectrum is found to be applicable in a wide range of the parameters where the RWA and the secular approximation may break down. We find that the counter-rotating (CR) terms of the transverse field omitted in the RWA have non-negligible contributions to the spectrum under certain conditions. Particularly, at the multiphoton resonance the width of which is comparable with the Bloch-Siegert shift, the RWA and non-RWA spectra markedly differ from each other because of the CR-induced shift. We also analyze the symmetry of the spectrum in terms of the transition matrix elements between the two-mode Floquet states. We show that the strict symmetry of the spectrum cannot be expected without the RWA but the almost symmetric spectrum can be obtained at the single-photon resonance that takes the Bloch-Siegert shift into account if the driving is moderately strong and at the multiphoton resonance with a sufficiently weak transverse field.
We investigate the dynamics of a driven two-level system (classical Rabi model) using the counter-rotating-hybridized rotating-wave method (CHRW), which is a simple method based on a unitary transformation with a parameter $\ensuremath{\xi}$. This approach is beyond the traditional rotating-wave approximation (Rabi-RWA) and more importantly, remains the RWA form with a renormalized tunneling strength and a modified driving strength. The reformulated rotating-wave method not only possesses the same mathematical simplicity as the Rabi-RWA but also allows us to explore the effects of counter-rotating (CR) components. We focus on the properties of off-resonance cases for which the Rabi-RWA method breaks down. After comparing the results of different RWA schemes and those of the numerically exact method in a wide range of parameter regime, we show that the CHRW method gives the accurate driven dynamics which is in good agreement with the numerical method. Moreover, the other RWA methods appear as various limiting cases of the CHRW method. The CHRW method reveals the effects of the CR terms clearly by means of coherent destruction of tunneling and Bloch-Siegert shift. Our main results are as follows: (i) the dynamics of the coherent destruction of tunneling is explicitly given and its dependence on $\ensuremath{\Delta}$ is clarified, which is quantitatively in good agreement with the exact results; (ii) the CR modulated Rabi frequency and the Bloch-Siegert shift are analytically calculated, which is the same as the exact results up to fourth order; (iii) the validity of parameter regions of different RWA methods are given and the comparison of dynamics of these methods are shown. Since the CHRW approach is mathematically simple as well as tractable and physically clear, it may be extended to some complicated problems where it is difficult to do a numerical study.
Floquet theory combined with the generalized Van Vleck nearly degenerate perturbation theory has been widely employed for studying various two-level systems that are driven by external fields via time-dependent longitudinal (i.e., diagonal) couplings. However, three-level systems strongly driven by time-dependent transverse (i.e., off-diagonal) couplings have rarely been investigated, due to the breakdown of the traditional rotating wave approximation. Meanwhile, the conventional perturbation theory is not directly applicable, since a small parameter for the perturbed part is no longer apparent. Here we develop a double-unitary-transformation approach to deal with periodically modulated and strongly driven systems, where the time-dependent Hamiltonian has large off-diagonal elements. The first unitary transformation converts strong off-diagonal elements to diagonal ones, and the second enables us to harness the generalized Van Vleck perturbation theory to deal with the transformed Floquet matrix and also allows us to reduce the infinite-dimensional Floquet Hamiltonian to a finite effective one. For a strongly modulated three-level system, with the combination of the Floquet theory and the transformed generalized Van Vleck perturbation theory, we obtain analytical results of the system, which agree well with exact numerical solutions. This method offers a useful tool to analytically study multilevel systems with strong transverse couplings.
We investigate the bias-modulated dynamics of a strongly driven two-level system using the counterrotating-hybridized rotating-wave (CHRW) method. This CHRW method treats the driving field and the bias on equal footing by a unitary transformation with two parameters $\ensuremath{\xi}$ and $\ensuremath{\zeta}$, and is nonperturbative in driving strength, tunneling amplitude, or bias. In addition, this CHRW method is beyond the traditional rotating-wave approximation (Rabi-RWA) and yet by properly choosing the two parameters $\ensuremath{\xi}$ and $\ensuremath{\zeta}$, the transformed Hamiltonian takes the RWA form with a renormalized energy splitting and a renormalized driving strength. The reformulated CHRW method possesses the same mathematical simplicity as the Rabi-RWA approach and thus allows us to calculate analytically the dynamics and explore explicitly the effect of the bias. We show that the CHRW method gives the accurate driven dynamics for a wide range of parameters as compared to the numerically exact results. When energy scales of the driving are comparable to the intrinsic energy scale of the two-level systems, the counterrotating interactions and static bias profoundly influence the generalized Rabi frequency. In this regime, where ordinary perturbation approaches fail, the CHRW works very well and efficiently. We also demonstrate the dynamics of the system in the strong-driving and off-resonance cases for which the Rabi-RWA method breaks down but the CHRW method remains valid. We obtain analytical expressions for the generalized Rabi frequency and bias-modulated Bloch-Siegert shift as functions of the bias, tunneling, and driving field parameters. The CHRW approach is a mathematically simple and physically clear method. It can be applied to treat some complicated problems for which a numerical study is difficult to perform.