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Quantum Correlations in Molecular Cavity Optomechanics

Philippe Djorwé, Kongkui Berinyuy Emale, D. R. K. Massembele, Reem Altuijri, Mohamed Rabea Eid, Abdel‐Haleem Abdel‐Aty, S. G. Nana Engo

Published Jan 1, 2025• 0 citations
Publisher
DOI
10.2139/ssrn.5343091

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Multipartite quantum entanglement in PT\mathcal{PT}PT-symmetric molecular optomechanics: Nonreciprocal enhancement and thermal resilience to \SI{500}{\kelvin}
We present a theoretical framework for a PT\mathcal{PT}PT-symmetric double-cavity molecular optomechanical system demonstrating nonreciprocal enhancement of multipartite quantum entanglement at elevated temperatures. All bipartite entanglement channels (EacE_{ac}Eac​, EaB1E_{aB_1}EaB1​​, EcB2E_{cB_2}EcB2​​, EB1B2E_{B_1B_2}EB1​B2​​) simultaneously maximize at optimal nonreciprocal asymmetry J1/J2≈5J_1/J_2 \approx 5J1​/J2​≈5, with entanglement persisting to $T \sim \SIrange{400}{500}{\kelvin}$ (material-limited ceiling) two orders of magnitude beyond conventional optomechanical systems. This thermal resilience and balanced enhancement across all channels arise from synergistic combination of ultra-high-frequency molecular vibrations ($ω_m/2π= \SI{30}{\tera\hertz}$), collective N\sqrt{N}N​ coupling enhancement with $N=\num{e6}$ molecules, and directional nonreciprocal coupling shielding entanglement-generating interactions from backaction noise. Unlike optical parametric amplifier schemes where vibration-vibration enhancement suppresses optical-vibration correlations, our PT\mathcal{PT}PT-symmetric architecture circumvents this fundamental trade-off, validated through rigorous stability analysis via Routh-Hurwitz criterion.