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Proceedings of the National Academy of Sciences

Experimental determination of tripartite quantum discord

Vaishali Gulati, Shaileyee Bhowmick, Tim Byrnes, Chandrashekar Radhakrishnan, Kavita Dorai

Published Jul 2, 2025• 3 citations

Abstract

Quantum discord is a measure of nonclassical correlations in quantum systems. While the bipartite version of quantum discord is experimentally well-studied, the multipartite version has never been convincingly measured. In this study, we experimentally investigate tripartite quantum discord using an NMR quantum information processor. Building on a theoretical framework for conditional projective measurements and quantum conditional mutual information, we quantify the tripartite quantum discord and its contributions in different three-qubit states such as the Greenberger-Horne-Zeilinger (GHZ) and Werner (W) states as well as classical mixtures of biseparable Bell states, and classical mixtures of product states. The experiments employed full quantum state tomography and temporal averaging to prepare mixed states, achieving fidelities exceeding 95%. Our results confirm that quantum discord persists even in the absence of entanglement, highlighting its utility as a broader indicator of quantum correlations. Furthermore, we validate the nonconvexity of discord, confirming that classical mixtures of zero-discord states can exhibit nonzero discord. This experimentally confirms that quantum discord does not fit into the framework of resource theory. This work establishes a robust methodology for measuring quantum discord, illuminating the structure and distribution of quantum correlations in multipartite systems.

DOI: 10.1073/pnas.2507467122

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Quantum discord is a measure of nonclassical correlations in quantum systems. While the bipartite version of quantum discord is experimentally well-studied, the multipartite version has never been convincingly measured. In this study, we experimentally investigate tripartite quantum discord using an NMR quantum information processor. Building on a theoretical framework for conditional projective measurements and quantum conditional mutual information, we quantify the tripartite quantum discord and its contributions in different three-qubit states such as the Greenberger-Horne-Zeilinger (GHZ) and Werner (W) states as well as classical mixtures of biseparable Bell states, and classical mixtures of product states. The experiments employed full quantum state tomography and temporal averaging to prepare mixed states, achieving fidelities exceeding 95%. Our results confirm that quantum discord persists even in the absence of entanglement, highlighting its utility as a broader indicator of quantum correlations. Furthermore, we validate the nonconvexity of discord, confirming that classical mixtures of zero-discord states can exhibit nonzero discord. This experimentally confirms that quantum discord does not fit into the framework of resource theory. This work establishes a robust methodology for measuring quantum discord, illuminating the structure and distribution of quantum correlations in multipartite systems.

A new measure based on the tripartite information diagram is proposed for identifying quantum discord in tripartite systems. The proposed measure generalizes the mutual information underlying discord from bipartite to tripartite systems, and utilizes both one-particle and two-particle projective measurements to reveal the characteristics of the tripartite quantum discord. The feasibility of the proposed measure is demonstrated by evaluating the tripartite quantum discord for systems with states close to Greenberger–Horne–Zeilinger, W, and biseparable states. In addition, the connections between tripartite quantum discord and two other quantum correlations—namely genuine tripartite entanglement and genuine tripartite Einstein–Podolsky–Rosen steering—are briefly discussed. The present study considers the case of quantum discord in tripartite systems. However, the proposed framework can be readily extended to general N-partite systems.

A generalization of quantum discord to multipartite systems is proposed. A key feature of our formulation is its consistency with the conventional definition of discord in bipartite systems. It is by construction zero only for systems with classically correlated subsystems and is a non-negative quantity, giving a measure of the total nonclassical correlations in the multipartite system with respect to a fixed measurement ordering. For the tripartite case, we show that the discord can be decomposed into contributions resulting from changes induced by nonclassical correlation breaking measurements in the conditional mutual information and tripartite mutual information. The former gives a measure of the bipartite nonclassical correlations and is a non-negative quantity, while the latter is related to the monogamy of the nonclassical correlations.

We propose a global measure for quantum correlations in multipartite systems, which is obtained by suitably recasting the quantum discord in terms of relative entropy and local von Neumann measurements. The measure is symmetric with respect to subsystem exchange and is shown to be nonnegative for an arbitrary state. As an illustration, we consider tripartite correlations in the Werner-GHZ (Greenberger-Horne-Zeilinger) state and multipartite correlations at quantum criticality. In particular, in contrast with the pairwise quantum discord, we show that the global quantum discord is able to characterize the infinite-order quantum phase transition in the Ashkin-Teller spin chain.

Abstract Quantum discord is a measure of non-classical correlations, which are excess correlations inherent in quantum states that cannot be accessed by classical measurements. For multipartite states, the classically accessible correlations can be defined by the mutual information of the multipartite measurement outcomes. In general the quantum discord of an arbitrary quantum state involves an optimisation of over the classical measurements which is hard to compute. In this paper, we examine the quantum discord in the experimentally relevant case when the quantum states are Gaussian and the measurements are restricted to Gaussian measurements. We perform the optimisation over the measurements to find the Gaussian discord of the bipartite EPR state and tripartite GHZ state in the presence of different types of noise: uncorrelated noise, multiplicative noise and correlated noise. We find that by adding uncorrelated noise and multiplicative noise, the quantum discord always decreases. However, correlated noise can either increase or decrease the quantum discord. We also find that for low noise, the measurements that maximise the classically accessible correlations are single quadrature measurements. As the noise increases, a dual quadrature measurement becomes optimal.

Quantum discord represents a correlation beyond classicality that could be useful for many quantum information tasks, and therefore is viewed as a valuable quantum resource. Theoretically, whether a bipartite quantum state has a non-zero amount of quantum discord or not can be determined once its density matrix is given. Experimentally, however, it is not easy to perform a reliable tomography on the state, especially when considering the imperfection of devices and the high dimensionality of system. Here, inspired by the so-called dimension witness, we propose a new approach using uncharacterized measurements to witness quantum discord of an unknown bipartite state within arbitrary dimension system. Furthermore,

2 \times 2

measurements are sufficient for any bipartite state of arbitrarily large dimension. For any two-qubit state, we show that the maximum of witness happens when one performs mutually orthogonal basis measurement on each qubit. Our method exhibits high robustness against device imperfections, such as error tolerance, indicating its experimental feasibility.

A comparison is made between normal discord, super quantum discord, and entanglement for the tripartite Greenberger-Horne-Zeilinger (GHZ)-type squeezed states. For this aim, we start by studying the behavior of quantum discord for tripartite GHZ-type squeezed states. Also, we verify the monotonicity of the super quantum discord according to weaker quantum measurements. This was done by manipulating the amount of quantum information lost during the disruption of our quantum system and by controlling the measurement strength. Furthermore, we calculate the entanglement for our system.