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APL Photonics

Spectral characterization of biphotons using quantum interferometric spectroscopy

Samuel Corona-Aquino, Zi-Qi Zeng, Tao Xie, Shi-Xin You, Chunling Ding, Yukun Song, Dongzhou Wang, Yun Meng, Kai Zou, Xiaolong Hu, Baihong Li, Alfred B. U’Ren, Roberto de J. León‐Montiel, Rui‐Bo Jin

Published Jun 1, 2025• 0 citations
Publisher

Abstract

The spectral distribution of photon pairs produced by spontaneous parametric downconversion (SPDC) is one of the most exploited degrees of freedom in multiphoton experiments. Consequently, the characterization of such correlations is, without a doubt, a task of utmost importance. Common methods for measuring the joint spectral intensity (JSI) of correlated photon pairs often exhibit several drawbacks, such as the requirement for a bright source to offset high losses or the need for two-dimensional measurements, which can lead to prolonged acquisition times. In this work, we experimentally demonstrate a technique that allows for the reconstruction of the JSI from a single interferometric measurement, thus reducing the dimensionality of the problem. The reconstructed JSIs show good agreement with those obtained directly through a fiber spectrometer, confirming the effectiveness of our approach. This technique significantly enhances the efficiency of JSI characterization, offering a resource-efficient method for quantum state characterization in SPDC-based experiments.

DOI
10.1063/5.0267337

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The spectral distribution of photon pairs produced by spontaneous parametric downconversion (SPDC) is one of the most exploited degrees of freedom in multiphoton experiments. Consequently, the characterization of such correlations is, without a doubt, a task of utmost importance. Common methods for measuring the joint spectral intensity (JSI) of correlated photon pairs often exhibit several drawbacks, such as the requirement for a bright source to offset high losses or the need for two-dimensional measurements, which can lead to prolonged acquisition times. In this work, we experimentally demonstrate a technique that allows for the reconstruction of the JSI from a single interferometric measurement, thus reducing the dimensionality of the problem. The reconstructed JSIs show good agreement with those obtained directly through a fiber spectrometer, confirming the effectiveness of our approach. This technique significantly enhances the efficiency of JSI characterization, offering a resource-efficient method for quantum state characterization in SPDC-based experiments.
The ability to determine the joint spectral properties of photon pairs produced by the processes of spontaneous parametric downconversion (SPDC) and spontaneous four-wave mixing (SFWM) is crucial for guaranteeing the usability of heralded single photons and polarization-entangled pairs for multi-photon protocols. In this paper, we compare six different techniques that yield either a characterization of the joint spectral intensity or of the closely related purity of heralded single photons. These six techniques include: (i) scanning monochromator measurements, (ii) a variant of Fourier transform spectroscopy designed to extract the desired information exploiting a resource-optimized technique, (iii) dispersive fibre spectroscopy, (iv) stimulated-emission-based measurement, (v) measurement of the second-order correlation function g(2) for one of the two photons, and (vi) two-source Hong–Ou–Mandel interferometry. We discuss the relative performance of these techniques for the specific cases of a SPDC source designed to be factorable and SFWM sources of varying purity, and compare the techniques’ relative advantages and disadvantages.
In spontaneous parametric down-conversion, the spectral correlations between the signal and the idler are expressed by the joint spectral amplitude (JSA) function. However, in the standard coincidence measurements, the phase information of the JSA is lost, and only the square of the absolute value of the JSA is recorded, thus preventing full characterization of the biphoton state. Here, we present an experimental technique to investigate the interference of biphoton joint spectral amplitudes, unlocking new avenues in quantum photonics research. Our method explores phase-dependent phenomena within entangled biphoton spectra. This is achieved by simultaneously pumping two structured nonlinear photonic crystals and observing their interference, which reveals previously inaccessible effects with direct intensity measurements. We demonstrate the versatility of our technique by analyzing two types of joint spectra: one exhibiting a two-lobe shape and the other a three-lobe shape. Additionally, we reconstruct the joint spectral amplitudes for both scenarios and observe good agreement with theoretical predictions. These results pave the way for developing advanced quantum communication and information processing technologies using biphoton spectra.
Joint spectral characterization of SPDC photon pairs near 2 μμμm in (Al)GaAs-on-insulator waveguides
Integrated photon-pair sources are a core component of chip-based quantum computing, communication, and metrology. Although such sources have been demonstrated at conventional telecom wavelengths, the 2 μμμm band remains comparatively less explored, despite offering advantages for free-space quantum communication, low-loss transmission in emerging fiber networks, and integration with silicon photonic platforms. In this paper, we demonstrate spontaneous parametric down-conversion (SPDC) in straight GaAs- and AlGaAs-on-insulator waveguides. This platform offers strong second-order nonlinearity and geometry-tunable dispersion, which are advantageous for efficient on-chip pair generation. Measurements of the joint spectral intensity and heralded second-order correlation function show broadband emission around 2 μμμm with strong spectral anti-correlations. To our knowledge, this is the first direct joint-spectral characterization of an integrated SPDC source in this wavelength regime.
Polarization-entangled photon pairs can be efficiently prepared into pure Bell states with a high fidelity via type-II spontaneous parametric down-conversion (SPDC) of narrow-band pump light. However, the use of femtosecond pump pulses to generate multiphoton states with precise timing often requires spectral filtering to maintain a high quality of polarization entanglement. This typically reduces the efficiency of photon pair collection. We experimentally map the polarization correlations of photon pairs from such a source over a range of down-converted wavelengths with a high spectral resolution and find strong polarization correlations everywhere. A spectrally dependent imbalance between contributions from the two possible decay paths of SPDC is identified as the reason for a reduction in entanglement quality observed with femtosecond pump pulses. Our spectral measurements allow us to predict the polarization correlations for arbitrary filter profiles when the frequency degree of freedom of the photon pairs is ignored.
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