Quantum Dynamics in Simple Nonlinear Optical Systems

Daniel F. Walls, Gerard J Milburn

Daniel F. Walls, Gerard J Milburn

Chang‐Sheng Hu, Li-Tuo Shen, Zhen‐Biao Yang +3 more

Cavity optomechanical systems involving an optical parametric amplifier (OPA) can exhibit rich classical and quantum dynamical behaviors. By simply modulating the frequency of the laser pumping the OPA, we find two interesting parameter regimes, with one of them enabling us to study quantum-classical correspondence in system dynamics, while there exist no classical counterparts of the quantum features for the other. For the detuning of the laser pumping around the mechanical frequency, as the parametric gain of OPA increases to a critical value, the classical dynamics of the optical or mechanical modes can experience a transition from the regular periodic oscillation to a period-doubling motion, in which case the light-mechanical entanglement can be well studied by the logarithmic negativity and can manifest the dynamical transition the classical nonlinear dynamics. In addition, the optomechanical entanglement shows a second-order transition characteristic at the critical parametric gain. For the laser detuning being about twice the mechanical frequency, the kind of normal mode splitting comes up in the laser detuning dependence of optomechanical entanglement, which is induced by the squeezing of the optical and mechanical hybrid modes and finds no classical correspondence. The OPA-assisted optomechanical systems therefore offer a simple way to study and exploit quantum manifestations of classical nonlinear dynamics.

Matteo Bruschi, Federico Gallina, Barbara Fresch

Multidimensional optical spectroscopies are powerful techniques to investigate energy transfer pathways in natural and artificial systems. Because of the high information content of the spectra, numerical simulations of the optical response are of primary importance to assist the interpretation of spectral features. However, the increasing complexity of the investigated systems and their quantum dynamics call for the development of novel simulation strategies. In this work, we consider using digital quantum computers. By combining quantum dynamical simulation and nonlinear response theory, we present a quantum algorithm for computing the optical response of molecular systems. The quantum advantage stems from the efficient quantum simulation of the dynamics governed by the molecular Hamiltonian, and it is demonstrated by explicitly considering exciton-vibrational coupling. The protocol is tested on a near-term quantum device, providing the digital quantum simulation of the linear and nonlinear response of simple molecular models.

Yannick Dumeige, Patrice Féron

A simple model is used to simulate the dynamic properties of coupled nonlinear microcavities. The model has been checked using a nonlinear finite difference time domain code. We show that two coupled nonlinear cavities with a Kerr nonlinearity can have multistable or self pulsing behaviors. Finally, an application as a positive pulse all-optical memory is proposed.