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Controlling Collective Quasiparticle Dynamics Beyond Decoherence in Topological Interfaces

Fatemeh Davoodi

Published Jun 4, 2025• 1 citation
Publisher

Abstract

Abstract Long-lived coherent quasiparticles are a promising foundation for novel quantum technologies, where maintaining quantum coherence is crucial. Decoherence, driven by finite emitter lifetimes, remains a central challenge in quantum computing. Here, we control the dynamics of spatially separated quantum emitters via preserving their phase information by introducing a topological waveguide as a robust chiral reservoir. Incoherent quantum emitters randomly positioned near a perturbed honeycomb plasmonic interface and couple to the mutual topological interface mode. Using the S3 Stokes parameter, we trace far-field polarization patterns that reflect emitter coherence and spin–momentum locking. We show that even weakly coupled emitters exhibit coherent excitation and imprint phase on the emission. Time-domain dynamics reveal signatures of superradiance and subradiance that correlate with spatial interference in S3. These spatial-temporal features confirm that the observed polarization patterns arise from coherent quantum many-body dynamics, not classical interference. This challenges the conventional dichotomy between incoherent and coherent regimes, revealing that topological chiral photonic environments mediate long-range quantum correlations beyond standard waveguide QED.

DOI
10.21203/rs.3.rs-6796190/v1

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Abstract Long-lived coherent quasiparticles are a promising foundation for novel quantum technologies, where maintaining quantum coherence is crucial. Decoherence, driven by finite emitter lifetimes, remains a central challenge in quantum computing. Here, we control the dynamics of spatially separated quantum emitters via preserving their phase information by introducing a topological waveguide as a robust chiral reservoir. Incoherent quantum emitters randomly positioned near a perturbed honeycomb plasmonic interface and couple to the mutual topological interface mode. Using the S3 Stokes parameter, we trace far-field polarization patterns that reflect emitter coherence and spin–momentum locking. We show that even weakly coupled emitters exhibit coherent excitation and imprint phase on the emission. Time-domain dynamics reveal signatures of superradiance and subradiance that correlate with spatial interference in S3. These spatial-temporal features confirm that the observed polarization patterns arise from coherent quantum many-body dynamics, not classical interference. This challenges the conventional dichotomy between incoherent and coherent regimes, revealing that topological chiral photonic environments mediate long-range quantum correlations beyond standard waveguide QED.
When multiple quantum emitters couple to a common electromagnetic environment, interference in their collective radiative dynamics gives rise to superradiance and subradiance. In regimes where coherent interactions and collective dissipation compete, the microscopic many-body dynamics and quantum correlations among the emitters that underlie superradiance and subradiance are theoretically challenging and remain experimentally elusive, even though collective emission has been observed in many physical systems. Here, we realize a superconducting qubit array coupled to a common microwave waveguide that mediates collective dissipation, with simultaneous access to coherent interactions and microscopic measurements of many-body dynamics. Engineered qubit-waveguide couplings with tunable amplitude and phase enable control of collective interference and the resulting super- and subradiant states. Leveraging site-resolved control and readout, we directly observe the microscopic decay dynamics of multi-qubit states across different excitation manifolds and track the evolution of populations and tunable quantum correlations. We reveal collective decay in regimes beyond the ideal Dicke model, where strong qubit-qubit interactions stabilize superradiance and subradiance against local dephasing and reshape decay pathways through spatially and spectrally structured many-body eigenstates. Our results establish a flexible platform for exploring collective phenomena in many-body quantum optics and driven-dissipative approaches to robust quantum information processing.
Radiative coupling between quantum emitters leads to a range of spectacular emission phenomena. Dicke studied the foundations of collectively enhanced and suppressed decay, commonly referred to as super- and subradiance. Collective effects can further result in directionality of the emission, thus offering a complimentary implementation of chiral quantum optics. Waveguide quantum electrodynamics (QED) allows coupling between spatially separated emitters, enabling selective driving. In this work, we control the emission direction for a pair of quantum dots embedded in a bidirectional photonic crystal waveguide offering independent electrical tuning. Notably the emitters are 13 \micro m apart, which corresponds to 26 effective wavelengths, but are nevertheless radiatively coupled. The directionality arises from a dispersive dipole-dipole interaction, which shifts the energy of the collective states, so that the emitter pair effectively forms an artificial molecule. We show that the emission direction can be switched from left- to rightwards by manipulating the relative driving phase while collectively exciting the emitters. In addition, we observe directional photon statistics under continuous driving, with, for example, single photons detected on one output port, and photon pairs on the other. With pulsed excitation, both emitters are fully inverted and correlated photon pairs are observed in time-resolved intensity correlation measurements. This work demonstrates a novel implementation of chiral quantum optics using quantum dots coupled via a non-chiral waveguide, and reports key steps for scaling up as a multi-emitter waveguide QED platform.
Waveguide quantum electrodynamics (QED) studies the interaction between quantum emitters and guided photons in one dimension. When the waveguide hosts interacting photons, it becomes a platform to explore many-body quantum optics. However, the influence of photonic correlations on emitter dynamics remains poorly understood. In this work, we study the collective decay and coherent interactions of quantum emitters coupled to a one-dimensional Bose-Hubbard waveguide, an array of coupled photonic modes with repulsive on-site interactions that supports superfluid and Mott insulating phases. We show that photon-photon interactions alone can trigger a superradiant burst, independent of emitter spacing and transition frequency. In the off-resonant regime, emitters exhibit two distinct types of mediated interactions. Delocalized superfluid excitations yield persistent, long-range couplings, challenging the noninteracting paradigm, where long-range (dissipative) couplings occur in band, whereas short-range and coherent interactions occur in a bandgap. In the Mott limit, quasiparticles generate short-range interactions mediated by doublons and holons. Our work bridges many-body physics and waveguide QED, revealing how photonic many-body states shape emitter dynamics.
Nonlocal light-matter interactions with giant atoms in high-dimensional environments are not only fundamentally intriguing for testing quantum electrodynamics beyond the dipole approximation but also crucial for building high-dimensional quantum networks and engineering multipartite entangled states. Given the enigmatic and largely uncharted collective signatures exhibited by multiple giant atoms within two-dimensional optical baths, we delve into their nonperturbative collective dynamics within the single-excitation subspace, focusing on the case where they are coupled to a common two-dimensional photonic reservoir and employing a resolvent operator approach. We demonstrate that precisely engineered atomic arrangements lead to unconventional quantum dynamics, featuring non-Markovianity-induced beats and long-lived bound states in the continuum, thereby providing a versatile platform for implementing two-dimensional quantum memory. Phenomenologically, we observe the emergence of exotic photon emission patterns in both two- and three-dimensional (3D) baths. The emission directions are shown to be precisely controllable on demand through exact phase engineering of the coupling parameters, enabling a highly efficient chiral light-matter interface. Moreover, our generalization to a 3D bath reveals that coherent dipole-dipole interactions can survive despite the coupling to a continuum of modes, a finding that challenges conventional wisdom regarding decoherence.
Waveguide quantum electrodynamics (wQED) has become a central platform for studying collective light-matter interactions in low-dimensional photonic environments. While conventional wQED systems rely on uniform chirality or reciprocal emitter-waveguide coupling, we propose a structured wQED framework, where the coupling directionality of each emitter can be engineered locally to control excitation transport in an atom-nanophotonic interface. For different combinations of patterned coupling directionalities of the emitters, we identify four representative configurations that exhibit distinct dynamical behaviors: centering, wave-like, leap-frog, and dispersion excitations. Spectral analysis of the effective non-Hermitian Hamiltonian reveals that these dynamics originate from interferences among subradiant eigenmodes. Variance analysis further quantifies the spreading of excitation as functions of interatomic spacing and global chirality, showing tunable localization-delocalization transitions. Including nonguided losses, we find that the transport characteristics remain robust for realistic coupling efficiencies (beta >= 0.99). These results establish structured wQED as a practical route to manipulate excitation localization, coherence, and transport through programmable directionality patterns, paving the way for controllable subradiant transport and chiral quantum information routing.
Photon emission is the hallmark of light-matter interaction and the foundation of photonic quantum science, enabling advanced sources for quantum communication and computing. Although single-emitter radiation can be tailored by the photonic environment, the introduction of multiple emitters extends this picture. A fundamental challenge, however, is that the radiative dipole-dipole coupling rapidly decays with spatial separation, typically within a fraction of the optical wavelength. We realize distant dipole-dipole radiative coupling with pairs of solid-state optical quantum emitters embedded in a nanophotonic waveguide. We dynamically probe the collective response and identify both super- and subradiant emission as well as means to control the dynamics by proper excitation techniques. Our work constitutes a foundational step toward multiemitter applications for scalable quantum-information processing.