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Physical Review Letters

Deterministic Quantum State Generators and Stabilizers from Nonlinear Photonic Filter Cavities

Sean Chen, Nicholas Rivera, Jamison Sloan, Marin Soljacic A

Published May 28, 2025• 0 citations
Publisher

Abstract

Quantum states of light, particularly at optical frequencies, are considered necessary to realize a host of important quantum technologies and applications, spanning Heisenberg-limited metrology, continuous-variable quantum computing, and quantum communications. Nevertheless, a wide variety of important quantum light states are currently challenging to deterministically generate at optical frequencies. In part, this is due to a relatively small number of schemes that prepare target quantum states given nonlinear interactions. Here, we present an especially simple concept for deterministically generating and stabilizing important quantum states of light, using only third-order optical nonlinearities and engineered dissipation. We show how, by considering either a nonlinear cavity with frequency-dependent outcoupling or a chain of nonlinear waveguides, one can induce high loss for all but some desired light intensities. Specifically, we find that the stabilized intensities can correspond to an evenly spaced pattern of stablilized photon numbers. This is shown to produce important quantum states with coherent superpositions between various photon numbers. As examples of this phenomenon, we show cavities which can stabilize squeezed states, as well as produce "photon-number-comb" states. Moreover, in these types of filter cavities, Glauber coherent states will deterministically evolve into Schrodinger cat states of a desired order. We discuss potential realizations in quantum nonlinear optics. More broadly, we expect that combining the techniques introduced here with additional "phase-sensitive" nonlinearities (such as second-order nonlinearity) should enable passive stabilization and generation of a wider variety of states than shown here.

DOI
10.1103/physrevlett.134.213601

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Quantum states of light, particularly at optical frequencies, are considered necessary to realize a host of important quantum technologies and applications, spanning Heisenberg-limited metrology, continuous-variable quantum computing, and quantum communications. Nevertheless, a wide variety of important quantum light states are currently challenging to deterministically generate at optical frequencies. In part, this is due to a relatively small number of schemes that prepare target quantum states given nonlinear interactions. Here, we present an especially simple concept for deterministically generating and stabilizing important quantum states of light, using only third-order optical nonlinearities and engineered dissipation. We show how, by considering either a nonlinear cavity with frequency-dependent outcoupling or a chain of nonlinear waveguides, one can induce high loss for all but some desired light intensities. Specifically, we find that the stabilized intensities can correspond to an evenly spaced pattern of stablilized photon numbers. This is shown to produce important quantum states with coherent superpositions between various photon numbers. As examples of this phenomenon, we show cavities which can stabilize squeezed states, as well as produce "photon-number-comb" states. Moreover, in these types of filter cavities, Glauber coherent states will deterministically evolve into Schrodinger cat states of a desired order. We discuss potential realizations in quantum nonlinear optics. More broadly, we expect that combining the techniques introduced here with additional "phase-sensitive" nonlinearities (such as second-order nonlinearity) should enable passive stabilization and generation of a wider variety of states than shown here.
Quantum states of light, particularly at optical frequencies, are considered necessary to realize a host of important quantum technologies and applications, spanning Heisenberg-limited metrology, continuous-variable quantum computing, and quantum communications. Nevertheless, a wide variety of important quantum light states are currently challenging to deterministically generate at optical frequencies. In part, this is due to a relatively small number of schemes that prepare target quantum states given nonlinear interactions. Here, we present an especially simple concept for deterministically generating and stabilizing important quantum states of light, using only simple third-order optical nonlinearities and engineered dissipation. We show how by considering either a nonlinear cavity with frequency-dependent outcoupling, or a chain of nonlinear waveguides, one can "filter" out all but a periodic ladder of photon number components of a density matrix. As examples of this phenomenon, we show cavities which can stabilize squeezed states, as well as produce "photon-number-comb" states. Moreover, in these types of filter cavities, Glauber coherent states will deterministically evolve into Schrodinger cat states of a desired order. We discuss potential realizations in quantum nonlinear optics. More broadly, we expect that combining the techniques introduced here with additional "phase-sensitive" nonlinearities (such as second-order nonlinearity) should enable passive stabilization and generation of a wider variety of states than shown here.
Interactions between photons (nonlinearities) enable a powerful form of control over the state of light. This control has enabled technologies such as light sources at new wavelengths, ultra-short optical pulses, frequency-comb metrology systems, even quantum light sources. Common to a wide variety of nonlinear optical technologies is an equilibrium between an energy source, such as an external laser, and dissipation, such as radiation loss or absorption. In the vast majority of these systems, the coupling between the system and the outside world (which leads to loss) is well-described as ``Markovian,'' meaning that the outside world has no memory of its past state. In this work, we introduce a class of driven-dissipative systems in which a nonlinear cavity experiences non-Markovian coupling to the outside world. In the classical regime, we show that these non-Markovian cavities can have extremely low thresholds for nonlinear effects, as well as self-pulsing instabilities at THz rates, and rich phase diagrams with alternating regions of stability and instability. In the quantum regime, we show how these system, when implemented on state-of-the-art platforms, can enable generation of strongly squeezed cavity states with intensity fluctuations that can be more than 15 dB below the classical limit, in contrast to the Markovian driven-dissipative cavity, in which the limit is 3 dB. In the regime of few-photon nonlinearity, such non-Markovian cavities can enable a deterministic protocol to generate Fock states of high order, which are long-desired, but still elusive at optical frequencies. We expect that exploiting non-Markovian couplings in nonlinear optics should in the future lead to even richer possibilities than those discussed here for both classical and quantum light manipulations.
Interactions between photons (nonlinearities) enable a powerful form of control over the state of light. This control has enabled technologies such as light sources at new wavelengths, ultra-short optical pulses, frequency-comb metrology systems, even quantum light sources. Common to a wide variety of nonlinear optical technologies is an equilibrium between an energy source, such as an external laser, and dissipation, such as radiation loss or absorption. In the vast majority of these systems, the coupling between the system and the outside world (which leads to loss) is well described as “Markovian,” meaning that the outside world has no memory of its past state. In this work, we introduce a class of driven-dissipative systems in which a nonlinear cavity experiences non-Markovian coupling to the outside world. In the classical regime, we show that these non-Markovian cavities can have extremely low thresholds for nonlinear effects, as well as self-pulsing instabilities at THz rates, and rich phase diagrams with alternating regions of stability and instability. In the quantum regime, we show how these systems, when implemented on state-of-the-art platforms, can enable generation of strongly squeezed cavity states with intensity fluctuations that can be more than 15 dB below the classical limit, in contrast to the Markovian driven-dissipative cavity, in which the limit is 3 dB. In the regime of few-photon nonlinearity, such non-Markovian cavities can enable a deterministic protocol to generate Fock states of high order, which are long-desired, but still elusive at optical frequencies. We expect that exploiting non-Markovian couplings in nonlinear optics should in the future lead to even richer possibilities than those discussed here for both classical and quantum light manipulations.
Quantum states are important resources and their preparations are essential prerequisites to all quantum technologies. However, they are extremely fragile due to the inevitable dissipations. Here the all-optical generation of a deterministic squeezed Schr\"odinger-cat state based on dissipation is proposed. Our system is based on the Fredkin-type interaction between three optical modes, one of which is subject to coherent two-photon driving and the others are coherent driving. We show that an effective degenerate three-wave-mixing process can be engineered in our system, which can cause the simultaneous loss of two photons, resulting in the generation of a deterministic squeezed Schr\"odinger-cat state. More importantly, by controlling the driving fields in our system, the two-photon loss can be adjustable, which can accelerate the generation of squeezed Schr\"odinger-cat states. In addition, we exploit the squeezed Schr\"odinger-cat states to estimate the phase in the optical interferometer and show that the quantum Fisher information about the phase can reach the Heisenberg limit in the limit of a large photon number. Meanwhile, it can have an order of magnitude factor improvement over the Heisenberg limit in the low-photon-number regime, which is very valuable for fragile systems that cannot withstand large photon fluxes. This work proposes an all-optical scheme to deterministically prepare the squeezed Schr\"odinger-cat state with high speed and can also be generalized to other physical platforms.
While dissipation is widely considered to be harmful for quantum coherence, it can, when properly engineered, lead to the stabilization of nontrivial pure quantum states. We propose a scheme for continuous generation and stabilization of Schr\"odinger cat states in a cavity using dissipation engineering. We first generate nonclassical photon states with definite parity by means of a two-photon drive and dissipation, and then stabilize these transient states against single-photon decay. The single-photon stabilization is autonomous, and is implemented through a second engineered bath, which exploits the photon-number-dependent frequency splitting due to Kerr interactions in the strongly dispersive regime of circuit QED. Starting with the Hamiltonian of the baths plus cavity, we derive an effective model of only the cavity photon states along with analytic expressions for relevant physical quantities, such as the stabilization rate. The deterministic generation of such cat states is one of the key ingredients in performing universal quantum computation.