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ACS Photonics

Automated Modal Analysis of Entanglement with Bipartite Self-Configuring Optics

Charles Roques‐Carmes, Aviv Karnieli, David A. B. Miller, Shanhui Fan

Published May 28, 2025• 5 citations
Publisher

Abstract

Entanglement is a unique feature of quantum mechanics. In coupled systems of light and matter, entanglement manifests itself in the linear superposition of multipartite quantum states (e.g., parametrized by multiple spatial, spectral, or temporal degrees of freedom of a light field). In bipartite systems, the Schmidt decomposition provides a modal decomposition of the entanglement structure over independent, separable states. Although ubiquitous as a mathematical tool to describe and measure entanglement, there exists no general efficient experimental method to decompose a bipartite quantum state onto its Schmidt modes. Here, we propose a method that relies on bipartite self-configuring optics that automatically “learns” the Schmidt decomposition of an arbitrary pure quantum state. Our method is designed for entanglement distributed over spatial or spectral degrees of freedom of a light field and can reconstruct the Schmidt modes and values by variational optimization of the network’s output powers or coincidences. We illustrate our method with numerical examples of spectral entanglement analysis for biphotons generated via spontaneous parametric down conversion and provide experimental guidelines for its realization and generalization to other degrees of freedom of light, including the influence of losses and impurities. Our method provides a versatile and scalable way of analyzing entanglement in bipartite integrated quantum photonic systems.

DOI
10.1021/acsphotonics.5c00813

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Entanglement is a unique feature of quantum mechanics. In coupled systems of light and matter, entanglement manifests itself in the linear superposition of multipartite quantum states (e.g., parametrized by multiple spatial, spectral, or temporal degrees of freedom of a light field). In bipartite systems, the Schmidt decomposition provides a modal decomposition of the entanglement structure over independent, separable states. Although ubiquitous as a mathematical tool to describe and measure entanglement, there exists no general efficient experimental method to decompose a bipartite quantum state onto its Schmidt modes. Here, we propose a method that relies on bipartite self-configuring optics that automatically “learns” the Schmidt decomposition of an arbitrary pure quantum state. Our method is designed for entanglement distributed over spatial or spectral degrees of freedom of a light field and can reconstruct the Schmidt modes and values by variational optimization of the network’s output powers or coincidences. We illustrate our method with numerical examples of spectral entanglement analysis for biphotons generated via spontaneous parametric down conversion and provide experimental guidelines for its realization and generalization to other degrees of freedom of light, including the influence of losses and impurities. Our method provides a versatile and scalable way of analyzing entanglement in bipartite integrated quantum photonic systems.
Spontaneous parametric down-conversion (SPDC) is the most widely-used source of high-dimensional entangled two-photon states, and the entanglement in the spatial degree of freedom is considered best suited for harnessing high-dimensional advantages. Although the Schmidt basis provides a natural choice for state characterisation of entangled two-photon states in any degree of freedom, there is currently no technique that can measure the Schmidt basis of an entangled two-photon field. The existing techniques can only reconstruct the Schmidt spectrum when the Schmidt basis is known a priori. In contrast, we present a technique that measures the complete set of spatial Schmidt modes without any prior knowledge. Using this technique, we report measurement of states with over 3000 Schmidt modes -- highest reported yet -- with up to 98%\%% fidelity. We expect our work to significantly advance the harnessing of high-dimensional advantages in SPDC-based systems.
We introduce a new class of self-configuring photonic architectures called variational optical processors (VOPs). These devices tackle the problem of decomposing and measuring multimode light fields, both partially coherent and quantum, without requiring prior knowledge of the modes involved. Classical strategies for modal decomposition—such as Karhunen-Loève expansions [1] for partially coherent beams or Schmidt decompositions [2] for bipartite quantum states—often rely on comprehensive tomography and complex data processing. By contrast, VOPs discover the relevant modes in situ through a simple optimization of detection signals at their outputs (e.g., measured optical power or coincidence counts), eliminating the overhead usually associated with scanning and reconstruction. Prior demonstrations of self-configuring photonic networks have proven the feasibility of such approaches for analyzing and generating multimode coherent optical fields [3].
Entanglement plays a crucial role in quantum physics and is the key resource in quantum information processing. In entanglement theory, Schmidt decomposition is a powerful tool to analyze the fundamental properties and structure of quantum entanglement. This work introduces a hybrid quantum-classical algorithm for Schmidt decomposition of bipartite pure states on near-term quantum devices. First, we show that the Schmidt decomposition task could be accomplished by maximizing a cost function utilizing bi-local quantum neural networks. Based on this, we propose a variational quantum algorithm for Schmidt decomposition (named VQASD) of which the cost function evaluation notably requires only one estimate of expectation with no extra copies of the input state. In this sense, VQASD outperforms existent approaches in resource cost and hardware efficiency. Second, by further exploring VQASD, we introduce a variational quantum algorithm to estimate the logarithm negativity, which can be applied to efficiently quantify entanglement of bipartite pure states. Third, we experimentally implement our algorithm on Quantum Leaf using the IoP CAS superconducting quantum processor. Both experimental implementations and numerical simulations exhibit the validity and practicality of our methods for analyzing and quantifying entanglement on near-term quantum devices.
High-dimensional spatially entangled two-photon state generated by spontaneous parametric down-conversion process (SPDC) has become a promising resource for several quantum information science applications. For harnessing high-dimensional entanglement advantages, detection capability in the Schmidt basis is a necessity. Spatial entanglement has been explored in several modal bases, such as pixel, azimuthal, and radial modes. Among them, pixel and azimuthal entanglement have been widely utilized due to efficient access to their Schmidt modes, while radial-mode entanglement remains underexploited. This is because for radial coordinates, there is neither a Schmidt-decomposed form for the SPDC photons nor is there a technique for measuring high-dimensional radial Schmidt modes, which is a major roadblock in harnessing radial mode advantages. In this work, we first theoretically show that the azimuthal averaging of SPDC two-photon state yields a radial Schmidt-decomposed form under typical experimental situations. We then demonstrate an innovative approach for extracting the radial Schmidt modes and their spectrum by characterizing the density matrix in the radial basis of one of the SPDC photons. Finally, we report the first-ever measurement of radial Schmidt spectrum of upto 50 radial Schmidt modes with about 98\% fidelity.
We study entanglement in a system of three coupled quantum harmonic oscillators. Specifically, we use the Schmidt decomposition to analyze how the entanglement is distributed among the three subsystems. The Schmidt decomposition is a powerful mathematical tool for characterizing bipartite entanglement in composite quantum systems. It allows to write a multipartite quantum state as a sum of product states between the subsystems, with coefficients known as Schmidt coefficients. We apply this decomposition to the general quantum state of three coupled oscillators and study how the Schmidt coefficients evolve as the interaction strengths between the oscillators are varied. This provides insight into how entanglement is shared between the different bipartitions of the overall three-particle system. Our results advance the fundamental understanding of multipartite entanglement in networked quantum systems. They also have implications for quantum information processing using multiple entangled nodes.
We address the problem of the persistence of entanglement of quantum light under mode transformations, where orthogonal modes define the parties between which quantum correlations can occur. Since the representation of a fixed photonic quantum state in different optical mode bases can substantially influence the entanglement properties of the said state, we devise a constructive method to obtain families of states with the genuine feature of remaining entangled for any choice of mode decomposition. In the first step, we focus on two-photon states in a bipartite system and optimize their entanglement properties with respect to unitary mode transformations. Applying a necessary and sufficient entanglement witness criteria, we are then able to prove that the class of constructed states is entangled for arbitrary mode decompositions. Furthermore, we provide optimal bounds to the robustness of the mode-independent entanglement under general imperfections. In the second step, we demonstrate the power of our technique by showing how it can be straightforwardly extended to higher-order photon numbers in multipartite systems, together with providing a generally applicable and rigorous definition of mode-independent separability and inseparability for mixed states.