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Applied Physics Letters

Inter-frequency all-optical transfer of structured light information in Rb vapor based on spatial cross-phase modulation

Junfei Chen, Zhiping Wang, Hamid Reza Hamedi, Benli Yu

Published Apr 14, 2025• 1 citation
Publisher

Abstract

High-dimensional all-optical information transfer facilitates large-capacity, high-speed, and energy-efficient optical communication, playing a pivotal role in advancing modern photonic technologies. Here, we demonstrate the all-optical transfer of structured information between two beams with different frequencies via spatial cross-phase modulation in a hot 85Rb vapor. A high-power pump beam, characterized by a structured light, induces a refractive index change in the rubidium vapor. A low-power, initially Gaussian probe beam counter-propagates through the rubidium vapor cell, undergoing a nonlinear phase shift induced by the pump beam. This enables the transfer of the spatial characteristics imprinted by the pump beam onto the probe beam with maximum structural integrity and similarity. The spatial evolution of the transverse intensity of the probe beam vs frequency detunings of the pump and probe beams, pump beam power, and cell temperature is studied. We have further shown that the structural similarity can be manipulated by changing the pump beam power and temperature of the vapor cell. Our findings may reveal a way to manipulate light fields, offering potential applications in optical communication, all-optical data processing, and advanced photonic devices.

DOI
10.1063/5.0256568

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High-dimensional all-optical information transfer facilitates large-capacity, high-speed, and energy-efficient optical communication, playing a pivotal role in advancing modern photonic technologies. Here, we demonstrate the all-optical transfer of structured information between two beams with different frequencies via spatial cross-phase modulation in a hot 85Rb vapor. A high-power pump beam, characterized by a structured light, induces a refractive index change in the rubidium vapor. A low-power, initially Gaussian probe beam counter-propagates through the rubidium vapor cell, undergoing a nonlinear phase shift induced by the pump beam. This enables the transfer of the spatial characteristics imprinted by the pump beam onto the probe beam with maximum structural integrity and similarity. The spatial evolution of the transverse intensity of the probe beam vs frequency detunings of the pump and probe beams, pump beam power, and cell temperature is studied. We have further shown that the structural similarity can be manipulated by changing the pump beam power and temperature of the vapor cell. Our findings may reveal a way to manipulate light fields, offering potential applications in optical communication, all-optical data processing, and advanced photonic devices.
All-optical information conversion, conveying optical signals without electro-optical transformation, plays a vital role in the all-optical devices and optical communication. We achieve the all-optical information conversion in Rb vapor by utilizing the spatial cross-phase modulation. The refractive index of atomic medium is spatially modulated by the strong switch laser beam, which makes it as a nonlinear focusing lens for the weak signal laser beam. As a result, the far-field diffraction ring patterns of the signal laser beam interacted with atoms can effectively carry the nonlinear phase shift information of the switch laser beam. The channel numbers, channel capacities and channel storage densities of information transmission from switch laser beam to signal laser beam are investigated in the terms of switch laser intensity and vapor temperature. Finally, a special "sxu" alphabetic string, encoded by ASCII code, is introduced to verify this all-optical information conversion scheme. This work paves the way for studying optical information processing and all-optical networking with atomic ensembles.
Airy vortex beams, which integrate orbital angular momentum with diffraction-resistant and self-accelerating characteristics of Airy beams, offer unique capabilities for high-capacity optical communication and high-resolution imaging. Here, we experimentally demonstrate the generation and manipulation of frequency-converted Airy vortex beams through four-wave mixing in hot Rb vapor. A 780 nm vortex beam and a 776 nm two-dimensional Airy beam coherently participate in the four-wave mixing process, generating a 420 nm output beam that combines the orbital angular momentum of the vortex beam with the spatial structure of the Airy beam. The generated beam exhibits pronounced quasi-nondiffracting propagation and self-acceleration, with an intensity decay rate reduced by a factor of ∼1.88 relative to the input vortex beam and a transverse acceleration ∼1.84 times that of the input Airy beam. Moreover, both the intensity and the spatial profile of the generated beam are flexibly manipulated by varying the Rb vapor temperature and the pump beam power. This work provides a versatile approach for generating and controlling structured light at what we believe are new wavelengths, opening opportunities for short-wavelength optical manipulation and optical information processing.
Nonlinear atomic media are promising substitutes for spatial light modulators (SLMs) owing to the high tunability and fast response. We demonstrate the generation of high-order Bessel-like beam based on cross-phase modulation in 85 Rb atoms. The atomic medium, whose refractive index is spatially modulated by the focused Gaussian pump beam, acts as a nonlinear focusing lens for the Laguerre-Gaussian probe beam. As a result, the probe beam carries the nonlinear phase shift and is converted into a Bessel-like mode in far-field diffraction. The superior self-healing ability of the generated high-order Bessel-like beam is verified by inserting an obstruction in the beam path, and its high tunability is investigated in terms of the pump beam power and vapor temperature. Furthermore, this novel beam is used in an obstruction-immune rotation sensor to measure the angular velocity. Nonlinear atomic medium as a novel SLM promises considerable application prospects in modulating the light field structure.
The effect of self-focusing and defocusing of the optical beam, which is caused by the interaction between a strong light field and medium, plays an important role in nonlinear optics. The difference in the spatial structure of the strong control beam with orbital angular momentum (OAM) and the Gaussian mode will have different effects on self-focusing and defocusing, which has the potential for realizing the modulation of the self-focusing and the defocusing process of the probe light with OAM. In this work, we report the influence of the spatial structure of the control beam on the self-focusing and defocusing process of the probe beam in a hot rubidium vapor cell with a lambda-type configuration. Under the same experimental condition, the control beam with the Laguerre-Gaussian mode contributes more to self-defocusing, while the Gaussian mode promotes the defocusing effect. The result is promising for manipulating the optical beam with OAM.
The ability to control light with light at ultralow powers has been a major avenue of research in photonics with applications to optical communications, computation, and signal processing. Such light-by-light scattering is achieved in a medium with a strong light-matter interaction, and for the development of quantum information networks it is important to demonstrate such effects near the single-photon level. Alkali-metal vapors such as rubidium (Rb) enable strong light-matter interactions due to the large cross section per atom and well-defined energy level structure, while the use of optical fibers offers the advantage of possible integration with modern optical communication systems. Hollow-core photonic band-gap fibers (PBGFs) can combine both these technologies such that both the atoms and the optical fields are transversely confined to a region that is a few wavelengths in size, which offers the prospect of exploring few-photon nonlinear interactions. We generate large optical depths in such a Rb-PBGF system, and the tight light confinement, high vapor density and long interaction length allow us to perform nonlinear optics at ultralow power. We demonstrate large signal amplification (>100) and frequency conversion using a four-wave mixing process with only microwatts of pump power. This is, to our knowledge, the largest gain observed at such low power. We perturb the coherence of this four-wave mixing to demonstrate all-optical modulation at unprecedented bandwidths (~300 MHz) for an atomic-vapor system, with an energy density of only tens of pho- tons per atomic cross-section, comparable to that achieved in more elaborate setups based on cold-atomic clouds. We then demonstrate an enhancement of several orders of magnitude in degenerate two-photon absorption in our RbPBGF system over that achieved in bulk vapor cells in a focused beam geometry. This allows us to directly measure two-photon absorption from a beam by detecting its intensity on a photodiode. Further, employing a near-resonant, non-degenerate two-photon transition in Rb, we demonstrate all-optical intensity modulation with just a few photons (<20), or only a few attojoules of energy, at relatively large bandwidths (~50 MHz) for such a sensitive scheme. This result takes us to within an order of magnitude of single-photon switching, and improves upon previous experiments for freely propagating optical fields, including those in cold-atoms. Finally, we produce relatively large cross-phase shifts of a few milliradians on a meter beam with <20 signal photons by tuning slightly away from resonance on the same non-degenerate two-photon transition. This corresponds to a phase shift of 0.3 milliradian per photon, with a fast response time of <5 ns. This represents, to our knowledge, the largest such nonlinear phase shift induced in a single-pass through a room temperature medium. Our Rb-PBGF system can thus potentially be employed to realize weak-nonlinearity based quantum computation and quantum non-demolition measurement of photon number. Through these experiments, we show the potential of a Rb-PBGF system for exploring quantum nonlinear optics at ultralow powers. Moreover, our system is simpler and easier to control and manipulate than setups based on cold atomic clouds and/or high-finesse cavities, and holds promise for integration with fiber-optic communication networks.
Abstract We investigate the nonlinear frequency conversion of non-diffracting optical modes via non-degenerate four-wave mixing(FWM) process in rubidium vapor. In this process, two strong control fields and a weak probe field mutually interact via afour-level double-Λ type atomic system to produce a new frequency weak Stokes field which is a phase conjugate to probe. We show that any arbitrary mode such as Airy, Bessel, Mathieu, and Weber beams encoded initially in the spatial envelope of probe field are efficiently transferred to FWM Stokes field by satisfying the phase matching condition. Interestingly, we found that the transmitted intensity profiles of Stokes beam are identical to that of probe beam while phase profile is complimentary.The phase conjugation property of output beams is revealed by interfering them with a copropagating plane wave. We further found the fidelity in terms of structural similarity between two transmitted modes of about 99%, which substantiates the high efficiency of FWM process. The efficient transfer and frequency conversion of such diffraction-free beams may have potential applications in nonlinear optical and quantum technologies.