Complex quantum states of light are not only central to advancing our understanding of quantum mechanics, but are also necessary for a variety of quantum protocols. High-dimensional, or multipartite, quantum states are of specific interest, as they can exhibit unique properties both fundamentally and in application. The synthesis of high-dimensional, entangled photonic states can take the form of various schemes, which result in varying forms of entanglement. Frequency entanglement is specifically attractive due to compatibility with integrated systems and resistance to decoherence in fiber transportation; however, increasing the dimension of frequency-entangled states requires a system that offers quantum interactions between a large set of distinct frequencies. Here, we show how the phonon-photon interactions of forward Brillouin scattering, which offer access to a ladder of optical resonances permitted by a single mechanical mode, can be used for fast synthesis of frequency-entangled, single-photon $W$ states. In our proposed system, simultaneous laser pulses of different frequencies dynamically evolve either an injected single photon or a heralded single phonon, generating $W$ states of selected dimension and output frequency. This method enables the synthesis of ``perfect'' $W$ states by adjusting the pulse amplitudes. In addition, we show how this system can be used for quantum frequency translation.
Complex quantum states of light are not only central to advancing our understanding of quantum mechanics, but are also necessary for a variety of quantum protocols. High-dimensional, or multipartite, quantum states are of specific interest, as they can exhibit unique properties both fundamentally and in application. The synthesis of high-dimensional, entangled photonic states can take the form of various schemes, which result in varying forms of entanglement. Frequency entanglement is specifically attractive due to compatibility with integrated systems and resistance to decoherence in fiber transportation; however, increasing the dimension of frequency-entangled states requires a system that offers quantum interactions between a large set of distinct frequencies. Here, we show how the phonon-photon interactions of forward Brillouin scattering, which offer access to a ladder of optical resonances permitted by a single mechanical mode, can be used for fast synthesis of frequency-entangled, single-photon W states. In our proposed system, simultaneous laser pulses of different frequencies dynamically evolve either an injected single photon or a heralded single phonon, generating W states of selected dimension and output frequency. This method enables the synthesis of ``perfect'' W states by adjusting the pulse amplitudes. In addition, we show how this system can be used for quantum frequency translation.
Complex quantum states of light are not only central to advancing our understanding of quantum mechanics, but are also necessary for a variety of quantum protocols. High-dimensional, or multipartite, quantum states are of specific interest, as they can exhibit unique properties both fundamentally and in application. The synthesis of high-dimensional, entangled photonic states can take the form of various schemes, which result in varying forms of entanglement. Frequency-entanglement is specifically attractive due to compatibility with integrated systems and resistance to decoherence in fiber transportation; however, increasing the dimension of frequency-entangled states requires a system that offers quantum interactions between a large set of distinct frequencies. Here, we show how the phonon-photon interactions of forward Brillouin scattering, which offer access to a ladder of optical resonances permitted by a single mechanical mode, can be used for fast-synthesis of frequency-entangled, single-photon W states. In our proposed system, simultaneous laser pulses of different frequencies dynamically evolve either an injected single photon or a heralded single phonon, generating W states of selected dimension and output frequency. This method enables the synthesis of `perfect' W states by adjusting the pulse amplitudes. In addition, we show how this system can be used for quantum frequency translation.
Frequency modes of light are one of the most promising platforms that provide access to high-dimensional quantum states amongst different photonic degrees of freedom capable of high-dimensionality, enabling robust, error-tolerant, and scalable quantum optical information systems. We demonstrate engineering of precisely controlled two-photon high-dimensional states entangled in frequency through time-domain Fourier optical synthesis. We generate and convert a continuous broadband frequency-entangled state into a large range of discrete frequency bins suitable for ITU standards, with spacings ranging from 12.5 GHz to 750 GHz, and observe spectral anticorrelations over 38 frequency bins, including intra-bin pure states at a 100 GHz bin spacing. We characterize the full quantum state dimensionality via Schmidt decomposition and observe lower bounds on the frequency-binned Hilbert-space dimensionalities of at least 289, formed by two entangled qudits with dimension 17. Furthermore, we demonstrate quantum nonlocality via frequency correlations in a transmission experiment over a campus-scale two-node fiber network. This work represents a crucial step towards building a versatile and relatively simple way of generating precisely controlled high-dimensional spectral qudits, with the potential of harnessing in wavelength-multiplexed quantum networks, high-dimensional information processing, and communication of quantum states specifically, and fiber-optic quantum remote sensing.
Recognized as a potential resource for quantum technologies and a possible test bed for fundamental physics, the control and preparation of nonclassical states of mechanical oscillators have been explored extensively. Within optomechanics, quantum state synthesis can be realized by entangling photonic and phononic degrees of freedom followed by optical detection. Single-photon detection enables one of the most powerful forms of such heralded quantum state preparation, permitting the creation of single-phonon states when applied to conventional cavity optomechanical systems. As the complexity of optomechanical systems increases, single-photon detection may provide heralded access to a larger class of exotic quantum states. Here, we examine the quantum dynamics of optomechanical systems that permit forward Brillouin scattering, where a single-phonon mode mediates transitions between a collection of equally spaced optical resonances. Solving both the Schrodinger equation and the Lindblad master equation for this system, we find that initial states comprised of single photons or weak laser pulses evolve into complex quantum states where the frequency of single-photon states and the phonon occupation number are entangled. Physically, these interactions permit a single photon to scatter to lower frequencies, where phonon excitation occurs for each scattering event. Combining this result with frequency filtering, we show how single-photon detection can herald selected multiphonon Fock states, even in the presence of optical losses. We also present an approach for quantum tomography of the heralded phonon states, which in the form of a state swap from the phononic to photonic domain enables on-demand generation of multiphoton Fock states.
The exploitation of quantum mechanics has the potential to solve important challenges and \nintroduce novel technologies enabling, among others, powerful computation (which can solve \ncertain problems exponentially faster than classical computers), perfectly secure communications, \nas well as sensing and imaging with precision and resolutions not achievable by classical means. \nIn order to make use of the unique properties of quantum physics, experimental platforms \nthat provide access to, and allow the control of quantum states, need to be developed. In \nparticular, quantum systems composed of multiple parties are required, where each party is in a \ncoherent superposition of states, and where multiples of such parties are in a coherent \nsuperposition with each other (e.g. being entangled). Additionally, in order to make use of such \nentangled quantum systems, it is required that each individual party can be coherently controlled \nand measured. The usability and available quantum resources of the entangled system is related \nto its size, which is proportional to the number of entangled parties, as well as the dimensionality \nof the superposition each party is in. For this reason, there is a imminent demand to achieve, \ninvestigate, and improve the generation and control of large quantum systems, comprised of as \nmany entangled parties as possible, where each party is in an ideally high-dimensional \nsuperposition. \nMany quantum platforms are currently subject to extensive research, such as trapped ions, \nsuperconducting circuits, defect centers in solid-state crystals, mechanical oscillators, and optical \nquantum states (i.e. photons). While all platforms provide distinct advantages (as well as \nchallenges), optical photon states are of particular interest, because they can interact with other \nquantum systems, and can be transmitted over long distances while preserving their quantum \ncoherence without the need for extensive shielding. A large variety of sources for optical \nquantum states has been demonstrated, however most such implementations suffer from high \ncomplexity, ultimately limiting their scalability. Integrated photonics has recently become a \nleading platform for the compact, cost-efficient, and stable generation and processing of optical \nquantum states. However, to date, integrated quantum sources have only been able to generate \nphoton pairs, which operated on single channels, and single polarization modes. Furthermore, in \nthe few realizations of on-chip entanglement, they were limited to two entangled parties, where \neach party was in a two-dimensional superposition. These limitations of current integrated photon sources arise in large part from the concepts currently exploited to generate and control these \nstates. In particular, path-entangled sources are the most commonly used, but increasing the \nquantum state complexity requires a significant, and very challenging, increase in device \ncomplexity. There is therefore an urgent need to develop new concepts that can achieve the onchip \ngeneration of large and complex photon states without increasing source complexity, while \nstill enabling coherent quantum state control and detection. \nIn this work, we aim to address these limitations by making use of multiple frequency and \ntemporal modes within a single spatial waveguide mode (therefore readily compatible with \nstandard optical fibers) of an on-chip microring resonator. This approach is in contrast to more \ncommonly used techniques relying on path entanglement, which exploits multiple spatial modes \nand generates entanglement by means of complex waveguide structures. Working within a single \nspatial mode, we achieve the first demonstration of pure heralded single photons and entangled \nphoton pairs, which are emitted on multiple frequency modes from a single source. We then \ndemonstrate the first generation of multi-photon entangled quantum states on a photonic chip. \nFinally, by making use of the spectral multi-mode nature of optical frequency combs, we achieve \nthe generation of photon pairs in a coherent superposition of multiple frequency modes, \nrepresenting the first generation of high-dimensional entangled states on a photonic chip. \nOur work represents a significant step forward in the generation of complex quantum \nstates on a photonic chip and in a single spatial mode compatible with standard optical fibers. In \naddition, we demonstrated coherent quantum state control and manipulation for all generated \nstates by means of standard telecommunications components, which could in the future be also \nintegrated on single, monolithic chip. Our results indicate that the exploitation of integrated \noptical frequency comb sources for the generation of optical quantum states can provide a \nscalable and practical platform for quantum technologies.
Generation and control of entanglement are fundamental tasks in quantum information. In this paper, we propose a novel approach to generating controllable frequency-entangled photons using the concept of synthetic frequency dimension in an optical system. This system consists of a ring resonator made of tailored third-order nonlinear media to induce photon-photon interactions and a periodic modulator to manipulate coupling between different frequency modes. We show that this system provides a unique platform for the exploration of distinct few- or many-body quantum phases including chaos, localization, and integrability in a highly integrable photonics platform. In particular, we develop a proposal to calculate the spectral form factor, which characterizes the degree of chaos in the system and differentiates between these phases based on observable measurements. Then, the switching of the quench dynamics from an intermediate phase between integrable and chaotic to the Stark many-body phase can generate and sustain stable frequency-entangled multiphoton states. This work is the first to explore rich and controllable quantum phases beyond single-particle physics in a synthetic dimension.
We present a method for the generation and coherent manipulation of pulsed quantum frequency combs. Until now, methods of preparing high-dimensional states on-chip in a practical way have remained elusive due to the increasing complexity of the quantum circuitry needed to prepare and process such states. Here, we outline how high-dimensional, frequency-bin entangled, two-photon states can be generated at a stable, high generation rate by using a nested-cavity, actively mode-locked excitation of a nonlinear micro-cavity. This technique is used to produce pulsed quantum frequency combs. Moreover, we present how the quantum states can be coherently manipulated using standard telecommunications components such as programmable filters and electro-optic modulators. In particular, we show in detail how to accomplish state characterization measurements such as density matrix reconstruction, coincidence detection, and single photon spectrum determination. The presented methods form an accessible, reconfigurable, and scalable foundation for complex high-dimensional state preparation and manipulation protocols in the frequency domain.