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Suppression of local decay rate through energy quantum confinement effect in non-Markovian waveguide QED

Yuan Liu, Hong‐Bo Sun, Linhan Lin

Published Mar 31, 2025• 3 citations
Publisher

Abstract

Abstract Waveguide quantum electrodynamics (QED) system manifests an ideal platform for studying many-body physics. When multiple emitters are coupled to a common waveguide, subradiant states may arise because of the waveguide-mediated interaction, leading to a long lifetime because of their immunity to the waveguide mode-induced dissipation. However, they can still be influenced by local environments, which are incoherent for different emitters and cannot be canceled out through interference. Herein, a new mechanism termed energy quantum confinement effect (EQCE) is proposed in a non-Markovian waveguide QED system to suppress the local dissipation. The energy quantum is confined in the waveguide by emitters, suppressing spontaneous decay of the emitters. The EQCE makes the system partly free from local dissipation of emitters, leading to a total decay rate lower than the local decay rate. We further show that similar effect occurs spontaneously by self-interference and can be stressed by cooperative coupling, relaxing the requirement for initializing the emitters into a remotely entangled state.

DOI
10.1186/s43074-025-00167-6

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Abstract Waveguide quantum electrodynamics (QED) system manifests an ideal platform for studying many-body physics. When multiple emitters are coupled to a common waveguide, subradiant states may arise because of the waveguide-mediated interaction, leading to a long lifetime because of their immunity to the waveguide mode-induced dissipation. However, they can still be influenced by local environments, which are incoherent for different emitters and cannot be canceled out through interference. Herein, a new mechanism termed energy quantum confinement effect (EQCE) is proposed in a non-Markovian waveguide QED system to suppress the local dissipation. The energy quantum is confined in the waveguide by emitters, suppressing spontaneous decay of the emitters. The EQCE makes the system partly free from local dissipation of emitters, leading to a total decay rate lower than the local decay rate. We further show that similar effect occurs spontaneously by self-interference and can be stressed by cooperative coupling, relaxing the requirement for initializing the emitters into a remotely entangled state.
Atoms coupled to the same environment interfere with each other to yield super- or sub-radiance. Specifically, atoms in subradiant states are promising candidates for long-lifetime qubits and quantum memory because of the immunity to the common environment. However, subradiant states can still be influenced by local environments, which are incoherent for different atoms and cannot be canceled out through interference. Here we propose to break this limit by preparing a waveguide QED system in the non-Markovian regime, where the ultra-small decay rate arises because of the retarded interaction. We further show that similar effect occurs spontaneously by self-interference and can be stressed by cooperative coupling.
Spontaneous emission of a quantum emitter, such as an excited atom, is a fundamental process in quantum electrodynamics (QED), typically associated with exponential decay to the ground state accompanied by irreversible photon emission. This simple Markovian picture, however, is profoundly modified in the presence of time-delayed feedback, structured continua, or cooperative emission, as occurs when an emitter radiates in front of a mirror, when several emitters radiate collectively, or in the case of a giant atom. In such regimes, strong non-Markovian dynamics arise from photon reabsorption and interference effects, leading to pronounced deviations from exponential decay. Here we demonstrate the emergence of exceptional points (EPs) in these highly non-Markovian waveguide-QED environments, i.e., non-Markovian EPs. These EPs appear directly in the relaxation dynamics as sharp transitions to oscillatory behavior, manifested by the appearance of real zeros in the excited-state amplitude. We analyze in detail the spontaneous emission of giant atoms with two or more coupling points, highlighting the mechanisms leading to non-Markovian EPs, and show that similar phenomena arise in other waveguide-QED settings, such as the collective spontaneous emission of spatially separated point-like emitters. Our results reveal waveguide-QED systems as experimentally accessible platforms for realizing and exploring non-Markovian EP physics.
Waveguide quantum electrodynamics platforms have emerged as promising candidates for exploring and implementing non-Markovian quantum phenomena. In this work, we investigate the formation and dynamics of superpositions of bound states in a cavity array waveguide coupled to two spatially separated quantum emitters. By tuning the system parameters, we show that spontaneous emission can drive the system into non-local equilibrium states in which both photonic and emitter populations exhibit persistent oscillations. These states arise from the coexistence of bound states embedded in the energy continuum and bound states outside it, leading to hybrid oscillatory modes. We analytically derive the conditions required for the emergence of these states, numerically simulate their formation through spontaneous emission, and predict their long-time behaviour. Our results demonstrate that such bound-state superpositions enable the generation of emitter-emitter interaction through free evolution, while supporting oscillatory breathing modes of the photon density between the emitters.
Quantum systems are invariably coupled to a surrounding environment. A common theoretical method to simplify the problem is to trace over the environment under a Markov approximation, which assumes that the environment holds no memory over the timescales that the system evolves under. In interacting many-body systems, it is often not trivial to extract which of the multiple collective timescales are relevant. We consider a time-delayed waveguide QED setup with a single excitation. By fixing the maximum propagation time and increasing the number of emitters, we show that, even for small delay times, collective effects are sufficient to cause non-Markovianity. The impact of memory is intrinsically state-dependent. For superradiant states, the relevant system timescale is the superradiant lifetime while the relevant bath timescale is the end-to-end delay time. For subradiant states, both timescales depend on the structure of the specific state. Our results demonstrate the importance of prudently making Markov approximations in quantum many-body systems, and highlight potential pitfalls to avoid in scaling up quantum devices to large system sizes.
Waveguide quantum electrodynamics (QED) has opened a new frontier in quantum optics, which enables the radiative coupling of distantly located emitters via the spatially extended waveguide mode. This coupling leads to modified emission dynamics and previous work has reported the observation of increased intensity correlations (an antidip) when probing the resonance response of multiple emitters. However, the interference between independent emitters has been shown to lead to a similar response. Here, we directly observe resonant energy transfer between two distant quantum emitters by recording an antidip in the intensity correlations, g ( 2 ) ( τ ) , while driving only one of the emitters. Under the condition that only a single emitter is driven, the antidip in photon coincidences is a distinctive signature of emitter-emitter coupling, which enables the transfer of energy from the driven to the undriven emitter. Interestingly, the observed mechanism is a long-range and waveguide-engineered version of resonant Förster transfer, which is responsible for the transport of energy between chlorophylls in the photosynthesis. Building on the established coupling, we demonstrate collective driving of the coupled emitter pair. Specifically, we control the relative driving phase and amplitude of the emitters and apply this collective excitation scheme to selectively populate the long-lived subradiant state. This results in suppressed emission, i.e., the peculiar situation where driving two emitters as opposed to one effectively reduces the probability of photon emission. Our work presents novel emission regimes and excitation schemes for a multiemitter waveguide QED system. These can be exploited to deterministically generate emitter-emitter entanglement and advanced photonic states providing robustness against losses for photonic quantum computation and quantum communication.
An array of initially excited emitters coupled to a one-dimensional waveguide exhibits superradiant decay under the Born-Markov approximation, manifested as a coherent burst of photons in the output field. In this work, we employ tensor-network methods to investigate its non-Markovian dynamics induced by finite time delays in photon exchange among the emitters. We find that the superradiant burst breaks into a structured train of correlated photons, each intensity peak corresponding to a specific photon number. We quantify the emitter-photon and emitter-emitter entanglement generated during this process and show that the latter emerges in the long-time limit, as part of the excitation becomes trapped within the emitters' singlet subspace. We finally consider the decay of the system's most radiant state, the symmetric Dicke state, and show that time delay can lead to decay rates exceeding those predicted by the Markovian approximation.