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Physical review. B./Physical review. B

Nonlocal quench spectroscopy of fermionic excitations in quantum spin chains

Saverio Bocini, Filippo Caleca, Fabio Mezzacapo, Tommaso Roscilde

Published Mar 25, 2025• 4 citations
Publisher

Abstract

The elementary excitations of quantum spin systems have generally the nature of weakly interacting bosonic quasiparticles, generated by local operators acting on the ground state. Nonetheless in one spatial dimension the nature of the quasiparticles can change radically, since many relevant one-dimensional $S=1/2$ Hamiltonians can be exactly mapped onto models of spinless fermions with local hopping and interactions. Due to the nonlocal nature of the spin-to-fermion mapping, observing directly the fermionic quasiparticle excitations is impossible using local probes, which are at the basis of all the forms of spectroscopy (such as neutron scattering) traditionally available in condensed-matter physics. Here, we show theoretically that quench spectroscopy for synthetic quantum matter---which probes the excitation spectrum of a system by monitoring the nonequilibrium dynamics of its correlation functions---can reconstruct accurately the dispersion relation of fermionic quasiparticles in spin chains. This possibility relies on the ability of quantum simulation experiments to measure nonlocal spin-spin correlation functions, corresponding to elementary fermionic correlation functions. Our analysis is based on exact results for the quench dynamics of quantum spin chains, and it opens the path to probe arbitrary quasiparticle excitations in synthetic quantum matter.

DOI
10.1103/physrevb.111.l121114

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The elementary excitations of quantum spin systems have generally the nature of weakly interacting bosonic quasiparticles, generated by local operators acting on the ground state. Nonetheless in one spatial dimension the nature of the quasiparticles can change radically, since many relevant one-dimensional S=1/2S=1/2S=1/2 Hamiltonians can be exactly mapped onto models of spinless fermions with local hopping and interactions. Due to the nonlocal nature of the spin-to-fermion mapping, observing directly the fermionic quasiparticle excitations is impossible using local probes, which are at the basis of all the forms of spectroscopy (such as neutron scattering) traditionally available in condensed-matter physics. Here, we show theoretically that quench spectroscopy for synthetic quantum matter---which probes the excitation spectrum of a system by monitoring the nonequilibrium dynamics of its correlation functions---can reconstruct accurately the dispersion relation of fermionic quasiparticles in spin chains. This possibility relies on the ability of quantum simulation experiments to measure nonlocal spin-spin correlation functions, corresponding to elementary fermionic correlation functions. Our analysis is based on exact results for the quench dynamics of quantum spin chains, and it opens the path to probe arbitrary quasiparticle excitations in synthetic quantum matter.
The elementary excitations of quantum spin systems have generally the nature of weakly interacting bosonic quasi-particles, generated by local operators acting on the ground state. Nonetheless in one spatial dimension the nature of the quasiparticles can change radically, since many relevant one-dimensional S=1/2S=1/2S=1/2 Hamiltonians can be exactly mapped onto models of spinless fermions with local hopping and interactions. Due to the non-local nature of the spin-to-fermion mapping, observing directly the fermionic quasiparticle excitations is impossible using local probes, which are at the basis of all the forms of spectroscopy (such as neutron scattering) traditionally available in condensed matter physics. Here we show theoretically that \emph{quench spectroscopy} for synthetic quantum matter -- which probes the excitation spectrum of a system by monitoring the nonequilibrium dynamics of its correlation functions -- can reconstruct accurately the dispersion relation of fermionic quasiparticles in spin chains. This possibility relies on the ability of quantum simulation experiments to measure non-local spin-spin correlation functions, corresponding to elementary fermionic correlation functions. Our analysis is based on new exact results for the quench dynamics of quantum spin chains; and it opens the path to probe arbitrary quasiparticle excitations in synthetic quantum matter.
The elementary excitation spectrum of a many-body quantum system encodes many key properties, including phenomena as diverse as transport, thermalisation and ground state structure. Excitation spectra of strongly correlated systems are typically encoded in dynamical structure factors, which are demanding to measure experimentally and challenging to compute classically. Here we use quench spectroscopy on a superconducting quantum processor to extract excitation spectra of spin chains of L=101L=101L=101 spins. By tailoring the combination of quench protocol and observable, we selectively access distinct excitation sectors across several phases of the spin-1/21/21/2 XXZ chain, resolving free magnons, multi-magnon bound states, and two-spinon continua. Notably, we demonstrate that the protocol does not rely on ground state preparation: in the classically challenging gapless regime, we extract spectra directly from the quench dynamics of easily prepared product states, a procedure that is natural and straightforward on quantum hardware. Our work establishes quench spectroscopy as a fast and flexible probe of many-body excitation spectra on digital quantum hardware, introduces a novel quench protocol that does not require costly state preparation routines, and provides a scalable route towards regimes where classical simulation may become intractable.
The nature and spectrum of elementary excitations are defining features of a many-body system. In this study, we used a Rydberg quantum simulator to demonstrate a form of spectroscopy, called quench spectroscopy, that probes these low-energy excitations. We illustrated the method on a two-dimensional simulation of the spin-1/2 dipolar XY model. Through microscopic measurements of the spatial spin correlation dynamics following a quench, we extracted the dispersion relation of the elementary excitations for both ferro- and antiferromagnetic couplings. The ferromagnet exhibits elementary excitations behaving as linear spin waves, whereas in the antiferromagnet, spin waves appear to decay, suggesting the presence of strong nonlinearities. Our demonstration highlights the importance of power-law interactions on the excitation spectrum of a many-body system.
Quantum simulation platforms such as cold atoms, superconducting circuits, and trapped ions enable the experimental investigation of quantum many-body systems, with important implications for quantum technologies. In this thesis, we investigate how entanglement and correlations develop in such systems and how they can be harnessed both for the theoretical study of models relevant to condensed matter physics and for practical applications in quantum metrology. We begin by focusing on the adiabatic preparation of quantum many-body ground states. In particular, we show that quantum simulators can probe the link between spectral degeneracy and Spontaneous Symmetry Breaking, as pioneered by P.W. Anderson. We prove that odd-sized spin-½ systems exhibiting time-reversal symmetry sustain a net magnetization even away from the thermodynamic limit, thanks to an exact spectral degeneracy. Moreover, the symmetry-broken state exhibits scalable spin squeezing, a key resource for quantum metrology. We then turn to a different paradigm of evolution: quench dynamics. In particular, we show that monitoring the real-time evolution of correlations allows for the experimental measurement of the dispersion relation of fundamental excitations. In the case of two-dimensional long-range ordered systems, such as the dipolar XY model, these excitations are spin waves, leading to sharp features in the evolution of two-point correlation functions. Conversely, in one-dimensional systems, fundamental excitations have a fermionic nature, and their detection requires the measurement of non-local correlation functions. The latter, while inaccessible in condensed matter, are instead well suited to quantum simulators with individually addressable degrees of freedom.
The simulation of quantum many-body systems, relevant for quantum chemistry and condensed matter physics, is one of the most promising applications of near-term quantum computers before fault-tolerance. However, since the vast majority of quantum computing technologies are built around qubits and discrete gate-based operations, the translation of the physical problem into this framework is a crucial step. This translation will often be device specific, and a suboptimal implementation will be punished by the exponential compounding of errors on real devices. The importance of an efficient mapping is already revealed for models of spinful fermions in two or three dimensions, which naturally arise when the relevant physics relates to electrons. Using the most direct and well-known mapping, the Jordan-Wigner transformation, leads to a nonlocal representation of local degrees of freedom, and necessities efficient decompositions of nonlocal unitary gates into a sequence of hardware accessible local gates. In this paper, we provide a step-by-step recipe for simulating the paradigmatic two-dimensional Fermi-Hubbard model on a quantum computer using only local operations. To provide the ingredients for such a recipe, we briefly review the plethora of different approaches that have emerged recently but focus on the Derby-Klassen compact fermion mapping to make our discussion concrete. We provide a detailed recipe for an end-to-end simulation including embedding on a physical device, preparing initial states such as ground states, simulation of unitary time evolution, and measurement of observables and spectral functions. We explicitly compute the resource requirements for simulating a global quantum quench and conclude by discussing the challenges and future directions for simulating strongly correlated fermionic matter on quantum computers.
Quantum simulation with ultracold atoms has become a powerful technique to gain insight into interacting many-body systems. In particular, the possibility to study nonequilibrium dynamics offers a unique pathway to understand correlations and excitations in strongly interacting quantum matter. So far, coherent nonequilibrium dynamics has exclusively been observed in ultracold many-body systems of bosonic atoms. Here we report on the observation of coherent quench dynamics of fermionic atoms. A metallic state of ultracold spin-polarized fermions is prepared along with a Bose–Einstein condensate in a shallow three-dimensional optical lattice. After a quench that suppresses tunnelling between lattice sites for both the fermions and the bosons, we observe long-lived coherent oscillations in the fermionic momentum distribution, with a period that is determined solely by the Fermi–Bose interaction energy. Our results show that coherent quench dynamics can serve as a sensitive probe for correlations in delocalized fermionic quantum states and for quantum metrology. In ultracold quantum gases, coherent nonequilibrium dynamics has been observed for bosons, but remained elusive in fermionic systems. Here, Will et al. demonstrate coherent quench dynamics in a hybrid quantum system composed of a metallic state of fermionic atoms and a Bose–Einstein condensate.