Trapping photons in a dye high-Q microcavity comprising two dielectric mirrors allows for studying Bose-Einstein condensation (BEC) of the two-dimensional photon gas under ambient conditions. Adding polymer nanostructures on the surface of the mirrors by direct laser writing provides additional trapping potentials for the photon gas. As the dimensionality of a system profoundly influences its physical behavior, trapping potentials with different effective dimensionality allow to study the modifications of the behavior for the 2d-1d transition. Here, we experimentally study the properties of a harmonically trapped photon gas undergoing Bose-Einstein condensation along this dimensional crossover. By varying the aspect ratio of the harmonic trap, we tune from an isotropic two-dimensional confinement to an anisotropic, highly elongated one-dimensional trapping potential. We discuss the fabrication of the micro potential on the highly reflective dielectric mirrors and determine the caloric properties of the photon gas and discuss prospects of our polymer-based potential landscapes.
Trapping photons in a dye high-Q microcavity comprising two dielectric mirrors allows for studying Bose-Einstein condensation (BEC) of the two-dimensional photon gas under ambient conditions. Adding polymer nanostructures on the surface of the mirrors by direct laser writing provides additional trapping potentials for the photon gas. As the dimensionality of a system profoundly influences its physical behavior, trapping potentials with different effective dimensionality allow to study the modifications of the behavior for the 2d-1d transition. Here, we experimentally study the properties of a harmonically trapped photon gas undergoing Bose-Einstein condensation along this dimensional crossover. By varying the aspect ratio of the harmonic trap, we tune from an isotropic two-dimensional confinement to an anisotropic, highly elongated one-dimensional trapping potential. We discuss the fabrication of the micro potential on the highly reflective dielectric mirrors and determine the caloric properties of the photon gas and discuss prospects of our polymer-based potential landscapes.
For many-body quantum systems, dimensionality is known to exert a profound influence on the physical behaviour, allowing for the shaping of distinct phases of matter. In general, for lower dimensions, enhanced fluctuations serve to suppress long range order. For bosonic gases, for example, Bose-Einstein condensation in one dimension requires confinement that is stronger than linear in order to occur, in contrast to two-dimensional systems where harmonic confinement can suffice. In this thesis, the dimensional crossover between one and two dimensions in a harmonically trapped photon gas has been experimentally investigated. The photons were confined within a dye filled optical microcavity, where polymer nanostructures produced by direct laser writing defined the trapping potential. By systematically adjusting the aspect ratio of the harmonic trap, the confinement was varied from an isotropic two dimensional regime to a highly anisotropic one dimensional regime. The caloric properties of the photon gas were characterised across this transition, revealing that the sharp phase transition observed in two dimensions evolves into a smooth crossover in one dimension. This work enhances understanding of thermodynamic behaviour in photon Bose gases under confinement and demonstrates that here dimensionality can be used to tailor phase transition phenomena. Furthermore, polymer cavities fabricated via direct laser writing afforded precise control over the confinement geometry, enabling exploration of variable potential landscapes. Proof of concept studies of advanced geometries, previously inaccessible, are presented, opening new directions for research in driven dissipative Bose gases and photonic quantum simulation platforms.
Abstract Since the advent of experiments with photon Bose–Einstein condensates (phBECs) in dye-filled microcavities in 2010, many investigations have focussed upon the emerging effective photon–photon interaction. Despite its smallness, it can be identified to stem from two physically distinct mechanisms. On the one hand, a Kerr nonlinearity of the dye medium yields a photon–photon contact interaction. On the other hand, a heating of the dye medium leads to an additional thermo-optic interaction, which is both delayed and non-local. The latter turns out to represent the leading contribution to the effective interaction for the current 2D experiments. Here we analyse theoretically how the effective photon–photon interaction increases when the system dimension is reduced from 2D to 1D. To this end, we consider an anisotropic harmonic trapping potential and determine via a variational approach how the properties of the phBEC in general, and both aforementioned interaction mechanisms in particular, change with increasing anisotropy. We find that the thermo-optic interaction strength increases at first linearly with the trap aspect ratio and later on saturates at a certain value of the trap aspect ratio. Furthermore, in the strong 1D limit the roles of both interactions get reversed as the thermo-optic interaction remains saturated and the contact Kerr interaction becomes the leading interaction mechanism. Finally, we discuss how the predicted effects can be measured experimentally.
Bose-Einstein condensation (BEC) is the transition to a macroscopic occupation of the ground state of a system of bosonic particles. In 1995 the first experimental realization of BEC was achieved by condensing a dilute atomic gas [1,2]. It was long thought only massive particles could undergo BEC. However, in 2010 it was shown that photon BEC was achieved in an optical dye-filled microcavity [3]. In 2015, we became the second group to successfully repeat these experiments.\n\nBEC is a phase transition and thus it occurs at thermal equilibrium. To achieve a thermal photon gas the cavity is filled with a fluorescent dye solution. The dye molecules thermalize the photons by means of repeated absorption-emission cycles. We optically pump the cavity. With the pump we determine the number of photons absorbed by the dye, consequently defining a nonvanishing chemical potential. This ensures a conserved photon number. The photons are trapped by the harmonic potential induced by the concave cavity mirrors. Due to the cutoff energy determined by the cavity length, the trapped photons have a dispersion similar to that of a massive particle in a quantum harmonic oscillator. The cavity length is tuned such that the free spectral range is larger than the bandwidth of the dye. Therefore, only one longitudinal mode fits inside the cavity, making the photon gas effectively two-dimensional. We end up with a thermalized two-dimensional photon gas that has the eigenenergies of a quantum harmonic oscillator. The Bose-Einstein distribution function predicts a critical photon number. Pumping the thermal photon gas beyond this critical number will lead to photon BEC.\n\nWe measure the spectral- and spatial distributions of our two-dimensional photon gas. In both distributions we observe photon BEC. Results show the characteristics of a phase transition: the appearance of a sharp peak on top of the thermal cloud that coincides with a converging chemical potential to zero. Both the spectral- and spatial distribution are in agreement with the theoretical distribution of photons with an effective mass in a quantum harmonic oscillator. Expansion of the condensate has been measured. This could indicate nonlinear optical effects such as thermal lensing or repulsive photon-photon interactions.
We consider a microcavity made by a graded-index glass, doped with dye molecules, placed within two planar mirrors and study Bose-Einstein condensation of photons. The presence of the mirrors leads to an effective photon mass, and the index grading provides an effective trapping frequency; the photon gas becomes formally equivalent to a two-dimensional Bose gas trapped in an isotropic harmonic potential. The inclusion of nonlinear effects provides an effective interaction between photons. We discuss, in particular, thermal lensing effects and nonlocal nonlinearity, and quantitatively compare our results with the reported experimental data.
Abstract Photon Bose–Einstein condensates are characterised by a quite weak interaction, so they behave nearly as an ideal Bose gas. Moreover, since the current experiments are conducted in a microcavity, the longitudinal motion is frozen out and the photon gas represents effectively a two-dimensional trapped gas of massive bosons. In this paper we focus on a harmonically confined ideal Bose gas in two dimensions, where the anisotropy of the confinement allows for a dimensional crossover. If the confinement in one direction is strong enough so that this squeezed direction is frozen out, then only one degree of freedom survives and the system can be considered to be quasi-one dimensional. In view of an experimental set-up we work out analytically the thermodynamic properties for such a system with a finite number of photons. In particular, we focus on examining the dimensional information which is contained in the respective thermodynamic quantities.
We investigate thermodynamic properties of a two-dimensional photon gas confined by a dye-filled optical microcavity. A thermally equilibrated state of the photon gas is achieved by radiative coupling to a heat bath that is realized with dye molecules embedded in a polymer at room temperature. The chemical potential of the gas is freely adjustable. The optical microcavity consisting of two curved mirrors induces both a non-vanishing effective photon mass and a harmonic trapping potential for the photons. While previous experiments of our group have used liquid dye solutions, the measurements described here are based on dye molecules incorporated into a polymer host matrix. The solid state material allows a simplified operation of the experimental scheme. We furthermore describe studies of fluorescence properties of dye-doped polymers, and verify the applicability of Kennard–Stepanov theory in this system. In the future, dye-based solid state systems hold promise for the realization of single-mode light sources in thermal equilibrium based on Bose–Einstein condensation of photons, as well as for solar energy concentrators.