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Nature Photonics

Integrated optical entangled quantum vortex emitters

Jieshan Huang, Jun Mao, Xudong Li, Jingze Yuan, Yun Zheng, Chonghao Zhai, Tianxiang Dai, Zhaorong Fu, Jueming Bao, Yan Yang, Daoxin Dai A, Yan Li, Qihuang Gong, Jianwei Wang

Published Feb 28, 2025• 37 citations
Publisher

Abstract

Abstract Quantum vortices of light carrying orbital angular momentum stand as essential resources for quantum photonic technologies. Recent advancements in integrated photonics offer the potential to create and control quantum vortices using fully integrated circuits, eliminating the needs for intricate free-space alignment, modulation, and stabilization of bulky optical elements. However, generating quantum vortices in planar optical waveguides and circuits poses challenges, owing to the complexities of confining and guiding twisted photons, and importantly, the difficulties in preparing quantum superposition and entanglement of vortex states. Here, we report entangled quantum vortex emitters leveraging programmable integrated nanophotonic circuits. These circuits enable the generation and arbitrary control of resilient vortex-entanglement in free space, coherently converting from on-chip path-entanglement by a chip-free space interfacing technology. The emitters are plug-and-play, enabling swift reconfiguration within mere microseconds. Validation of multidimensional genuine entanglement is achieved through quantum tomography and dimension witnesses. Our work demonstrates integrated quantum vortex devices that combine the versatility of on-chip processing quantum information with the robustness of transmitting quantum vortices in free space, opening new avenues for applications in quantum communication, quantum light detection and ranging, quantum computation and storage.

DOI
10.1038/s41566-025-01620-5

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Abstract Quantum vortices of light carrying orbital angular momentum stand as essential resources for quantum photonic technologies. Recent advancements in integrated photonics offer the potential to create and control quantum vortices using fully integrated circuits, eliminating the needs for intricate free-space alignment, modulation, and stabilization of bulky optical elements. However, generating quantum vortices in planar optical waveguides and circuits poses challenges, owing to the complexities of confining and guiding twisted photons, and importantly, the difficulties in preparing quantum superposition and entanglement of vortex states. Here, we report entangled quantum vortex emitters leveraging programmable integrated nanophotonic circuits. These circuits enable the generation and arbitrary control of resilient vortex-entanglement in free space, coherently converting from on-chip path-entanglement by a chip-free space interfacing technology. The emitters are plug-and-play, enabling swift reconfiguration within mere microseconds. Validation of multidimensional genuine entanglement is achieved through quantum tomography and dimension witnesses. Our work demonstrates integrated quantum vortex devices that combine the versatility of on-chip processing quantum information with the robustness of transmitting quantum vortices in free space, opening new avenues for applications in quantum communication, quantum light detection and ranging, quantum computation and storage.
Quantum mechanics endows light with properties that have no classical analogue - superposition, entanglement, and non-classical photon statistics, that can be harnessed as resources for computing, communication, sensing, and simulation. After decades of foundational research, quantum states of light can now be generated, manipulated, and measured with sufficient precision that their non-classical properties are no longer merely curiosities, but engineerable resources. Integrated photonics offers a compelling path forward. By confining light in lithographically defined waveguides on a chip, it replaces fragile bulk optical assemblies with compact, phase-stable, and reproducible circuits. Semiconductor quantum dots embedded in photonic nanostructures provide bright, on-demand single-photon emission compatible with waveguide integration, while superconducting nanowire single-photon detectors provide the efficiency and timing precision that quantum optical measurements demand. A particularly powerful frontier is reconfigurability: programmable photonic circuits whose functionality is defined in software can serve as versatile quantum photonic processors without any physical modification. This dissertation presents work on engineering quantum light across the full chain of generation, control, and detection using integrated photonic platforms. It covers coherent control of nanowire quantum dot emitters, generation of multipartite entangled states on a silicon nitride chip, and the use of programmable silicon-on-insulator interferometers as reconfigurable quantum optical processors for simulating quantum systems.
Very recently, the interest for quantum technologies by the scientific community and industry has strongly increased. Different types of implementations have been proposed as a practical implementation for a quantum bit as trapped atoms, superconducting qubits and single photons. In particular, we are interested in using single photons and single spins in solid state host matrices such as diamond (nanodiamonds or membranes). Integration of nanosources of light is currently a major bottleneck preventing the realisation of all-photonic chips for quantum technologies and nanophotonics applications. Nanophotonics and integrated optics are vast growing fields with huge market potentials in particular for quantum technologies. Ideally, one needs optical circuitry, on-chip photodetection and on-chip generation of quantum states of light (single photons, entangled photons…). We want to present our recent work on using integrated optics that can offer an easier and robust way to create fixed and compact quantum circuits that can be on chip and scalable. In this context, the coupling between waveguides and single photon emitters is critical. The goal of our research is to efficiently couple single photon emitters with a new platform made of optical glass waveguides. To achieve this goal, several paths are undertaken such as the use of dielectric and plasmonic structuration in order to increase the light interaction with the waveguide or to develop fabrication techniques to insert the emitters directly inside the guide (for nanodiamonds). We will show what is our current state of the art for placing single emitters at the right place on our optical waveguides made of ion-exchange in glass and in particular what can be done to improve our first promising results in order to get near unity coupling between the optical bus and single photon emitters. We will show first results with semiconductor nanocrystals (NCs) but also using nitrogen-vacancy defects in diamond either under nanodiamond form or in thin membranes.
Abstract High-dimensional quantum entanglement is an important resource for emerging quantum technologies such as quantum communication and quantum computation. The scalability of metres-long experimental setups limits high-dimensional entanglement in bulk optics. Advancements in quantum technology hinge on reproducible, and reconfigurable quantum devices—including photon sources, which are challenging to achieve in a scalable manner using bulk optics. Advances in nanotechnology and CMOS-compatible integration techniques have enabled the generation of entangled photons on millimeter-scale chips, significantly enhancing scalability, stability, replicability, and miniaturization for real-world quantum applications. In recent years we have seen several chip-scale demonstrations with different discrete degrees of freedom including path, frequency-bin, time-bin, and transverse modes, on many material platforms. A complete quantum photonic integrated circuit requires the generation, manipulation, and detection of quantum states, involving various active and passive quantum photonic components which further increase the degree of complexity. Here, we focus on the high-dimensional versions of qubits—qudits—and review the nonlinear optical processes that facilitate on-chip high-dimensional entangled photon sources, and the currently used material platforms. We discuss a range of current implementations of on-chip high-dimensional entangled photon sources and demonstrated applications. We comment on the current challenges due to the limitations of individual material platforms and present future opportunities in hybrid and heterogeneous integration strategies for the next generation of integrated quantum photonic chips.
Photonic quantum technologies require the integration of high-quality quantum light sources with programmable photonic circuitry to enable on-chip quantum information processing. Semiconductor quantum dots have emerged as a leading platform for quantum light generation, yet their monolithic integration with cryogenic-compatible, programmable photonic circuitry remains challenging. Here we demonstrate a programmable quantum photonic platform that enables simultaneous control of highly coherent quantum dot-based single photon emitters and reconfigurable optical elements at cryogenic temperatures. System-level integration enables individual electrical and optical addressing of active components on a single chip, allowing their concurrent operation while preserving coherent non-classical light emission. We demonstrate multiple quantum-photonic functionalities, including pure single-photon generation, two-photon interference, and resonant transmission and reflection measurements of integrated emitters. These results mark a step from isolated quantum-optical devices towards programmable quantum-photonic hardware platforms capable of combining coherent quantum emitters with large-scale photonic functionality.
In recent years, research on integrated quantum circuits has developed rapidly and exciting results have been achieved. The overarching goal of this emerging research direction in the field of modern quantum technology is the scalable integration of quantum functionality on robust chips. Such chips can work independently of one another, but it is even more interesting to develop them modularly for integration into larger quantum networks, thereby linking quantum computation and quantum communication in the same framework. In this context, the ongoing development and further optimization of integrated quantum circuits aim, inter alia, to achieve a quantum advantage in the area of quantum computing and to pave the way for multipartite quantum networks. The functionality of such chips is essentially based on single-photon operations, such as interference at beam splitters in combination with phase shifters in the field of linear optical quantum computing and Bell-state measurements for entanglement swapping in long-distance quantum networks. While individual functionalities such as CNOT gates and more complex quantum computing operations such as boson sampling in a combination of waveguide chips and external photon sources and detectors were successfully demonstrated, the field is currently facing the major challenge of integrating all necessary components monolithically on chip in order to exploit the full potential of integrated quantum nanophotonics. The present Perspective discusses the status and the present challenges of integrated quantum nanophotonics based on on-demand single-photon emitters and gives an outlook on required developments to enter the next level of fully functional quantum circuits for photonic quantum technology.
Twisted photons, carrying spin and orbital angular momentum (OAM) in an unbounded-dimensional Hilbert space, has recently sparked significant interest, leading to the discovery of new physics in both classical and quantum optics, furthering our understanding and incubating applications in classical and quantum communication. At the heart of this emerging field is the requirement for versatile, efficient, and robust generation of novel photonic spin-orbit states involving both spin and OAM degrees of freedom (DoFs). However, so far, the generation and manipulation of spin–orbit photons have primarily relied on free-space bulk optics, which, due to their lack of compactness and stability, are unsuitable for large-scale applications. In this work, we address this challenge by dynamically generating and manipulating the photonic spin-orbit states in both integrated microlaser and single photon source systems, leveraging non-Hermitian photonics and chiral quantum optics. We further investigated the generation and control of quantum entanglement between the spin and OAM DoFs of photons via integrated photonic circuits. Moreover, we successfully generated photonic spin-orbit states with intricate Skyrmionic topological structures and demonstrate the robustness of their topological properties during the quantum teleportation process. The integrated spin-orbit control toolbox for various structured photons, combined with the robustness of their topological properties, holds significant potential for developing large-channel capacity, noise-resilient information systems within a unique multidimensional space.