In the context of spin systems, exchange interactions play a crucial role in generating quantum entanglement within the ground and thermal states. This entanglement has been identified as a valuable reserve for Quantum Information and Computation protocols. In our study, we focus on a spin tetramer composed of spins with a magnitude of 1/2. These spins interact with each other through pairwise nearest-neighbour and diagonal interactions denoted as J1 and J2, respectively, as well as arm-wise and diagonal-wise 4-spin interactions of strengths K1 and K2 respectively . The geometric arrangement of the tetramer leads to frustration – a phenomenon observed in physical systems. By performing analytical calculations, we explore the quantum correlation properties of the tetramer in both its ground and thermal states. Our investigation includes the study of bipartite and multipartite entanglements, Quantum Discord and Fidelity. Notably, we identify signatures of quantum critical transition lines, which can be referred as the ‘entanglement transition lines’ signalled differently by different measures.
Exchange interactions in spin systems can give rise to quantum entanglement in the ground and thermal states of the systems. We consider a spin tetramer, with spins of magnitude
21, in which the spins interact via nearest-neighbor, diagonal, and four-spin interactions of strength
J1,
J2, and
K, respectively. The ground- and thermal-state entanglement properties of the tetramer are calculated analytically in the various limiting cases. Both bipartite and multipartite entanglements are considered and a signature of the quantum phase transition (QPT), in terms of the entanglement ratio, is identified. The first-order QPT is accompanied by discontinuities in the nearest-neighbor and diagonal concurrences. The magnetic properties of a
S=21 antiferromagnetic polyoxovanadate compound V12 are well explained by tetramers, with
J2=0,
K=0, in which the spins interact via the isotropic Heisenberg exchange interaction Hamiltonian. Treating the magnetic susceptibility $\ensuremath{\chi}$ as an entanglement witness (EW), an estimate of the lower bound of the critical entanglement temperature
Tc below which entanglement is present in the experimental compound, is determined. Two other cases considered include the symmetric tetramer---i.e., tetrahedron
(J1=J2,K=0)---and the symmetric trimer. In both the cases, there is no entanglement between a pair of spins in the thermal state but multipartite entanglement is present. A second EW based on energy provides an estimate of the entanglement temperature
TE below which the thermal state is definitely entangled. This EW detects bipartite entanglement in the case of the tetramer describing a square of spins (the case of V12 ) and multipartite entanglement in the cases of the tetrahedron and symmetric trimer.
Quantum simulators are capable of calculating properties of quantum systems unfeasible for classical computers. Here we report the analog quantum simulation of arbitrary Heisenberg-type interactions among four spin-1/2 particles. This spin-1/2 tetramer is the two-dimensional archetype system whose ground state belongs to the class of valence-bond states. Depending on the interaction strength, frustration within the system emerges such that the ground state evolves from a localized to a resonating valence-bond state. This spin-1/2 tetramer is created using the polarization states of four photons. We utilize the particular advantages of the precise single-particle addressability and a tunable measurement-induced interaction to obtain fundamental insights into entanglement dynamics among individual particles. We also directly extract ground-state energies and pair-wise quantum correlations, which enable our quantum simulator to investigate the frustration of entanglement. Remarkably, the pair-wise correlations are restricted by quantum monogamy.
Quantum discord (QD) is a general measure of bipartite quantum correlations with a potential role in quantum information processing tasks. Spin clusters serve as ideal candidates for the implementation of some of the associated protocols. In this paper, we consider a symmetric spin trimer and a tetramer which describe a number of known molecular magnets and compute the QD in the ground and thermal states of the clusters. The variations of the QD as a function of an anisotropy parameter, magnetic field and temperature are investigated. We obtain a number of interesting results such as a finite value of the QD in the trimer ground state for which the pairwise entanglement is known to be zero, differences in the nature of some of the variations in the ferromagnetic and antiferromagnetic cases, and discontinuous jumps in the magnitude of the QD at first-order quantum phase transition points. A remarkable feature that is observed is that the QD completely vanishes only in the asymptotic limit of temperature T → ∞. We further study the dynamics of the QD and the pairwise entanglement at T = 0 under the effect of a dephasing channel describing the interaction of the reduced spin cluster state with independent local environments. The QD is found to vanish asymptotically as t → ∞. In the case of the spin trimer, the pairwise entanglement has a zero value at all times and reaches a zero value in a finite time in the case of the tetramer.
Quantum discord (QD) is a general measure of bipartite quantum correlations with a potential role in quantum information processing tasks. Spin clusters serve as ideal candidates for the implementation of some of the associated protocols. In this paper, we consider a symmetric spin trimer and a tetramer which describe a number of known molecular magnets and compute the QD in the ground and thermal states of the clusters. The variations of the QD as a function of an anisotropy parameter, magnetic field and temperature are investigated. We obtain a number of interesting results such as a finite value of the QD in the trimer ground state for which the pairwise entanglement is known to be zero, differences in the nature of some of the variations in the ferromagnetic and antiferromagnetic cases, and discontinuous jumps in the magnitude of the QD at first-order quantum phase transition points. A remarkable feature that is observed is that the QD completely vanishes only in the asymptotic limit of temperature T → ∞. We further study the dynamics of the QD and the pairwise entanglement at T = 0 under the effect of a dephasing channel describing the interaction of the reduced spin cluster state with independent local environments. The QD is found to vanish asymptotically as t → ∞. In the case of the spin trimer, the pairwise entanglement has a zero value at all times and reaches a zero value in a finite time in the case of the tetramer.
We study here different regions in phase diagrams of the spin-1/2, spin-1 and spin-3/2 one-dimensional antiferromagnetic Heisenberg systems with frustration (next-nearest-neighbor interaction J2) and dimerization (δ). In particular, we analyze the behaviors of the bipartite entanglement entropy and fidelity at the gapless to gapped phase transitions and across the lines separating different phases in the J2-δ plane. All the calculations in this work are based on numerical exact diagonalizations of finite systems.
Multipartite entanglement and the maximum violation of Bell inequalities are studied in finite clusters of spins in an extended J1–J2 Heisenberg model at zero temperature. The ensuing highly frustrated states will unveil a rich structure for different values of the corresponding spin–spin interaction strengths. The interplay between nearest-neighbors, next-nearest neighbors and further couplings will be explored using multipartite correlations. The model is relevant to certain quantum annealing computation architectures where an all-to-all connectivity is considered.