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Physical Review Applied

Hyperentangled-state generation in nanophotonic periodically poled lithium niobate waveguides

Yanghe Chen, Bo Ji, Tengfei Wu, Guangqiang He

Published Feb 12, 2025• 4 citations
Publisher

Abstract

Hyperentanglement is a promising resource in the realm of quantum communication, owing to its exploitation of multiple degrees of freedom. In this paper, we report the generation of a two-mode hyperentangled state using one nanophotonic periodically poled lithium niobate waveguide. Our approach encompasses the manipulation of polarization, energy-time, and quadrature amplitude-phase degrees of freedom. Theoretical calculations reveal that the magnitude of the Clauser-Horne-Shimony-Holt parameter $|S|$ can reach $2.375$ even considering the multi-photon-pair generation effect, which is indicative of the entanglement in the polarization degree of freedom. Further analysis involved computing the joint spectral amplitude of the two-mode state, followed by Schmidt decomposition and Fourier transformation. The resulting joint uncertainty product $\mathrm{\ensuremath{\Delta}}({\ensuremath{\omega}}_{s}+{\ensuremath{\omega}}_{i})\mathrm{\ensuremath{\Delta}}({t}_{s}\ensuremath{-}{t}_{i})=0.4113$, implying that high-quality energy-time entanglement is achieved. Notably, the von Neumann entropy ${S}_{r}$ of our source reaches 0.192, confirming the presence of quadrature amplitude-phase entanglement within the generated state. Moreover, we theoretically apply our source in a free-space quantum key distribution system to demonstrate its potential to increase secret key rates. Our proposed scheme is an efficient and practical approach for facilitating high-capacity quantum communication systems.

DOI
10.1103/physrevapplied.23.024030

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Hyperentanglement is a promising resource in the realm of quantum communication, owing to its exploitation of multiple degrees of freedom. In this paper, we report the generation of a two-mode hyperentangled state using one nanophotonic periodically poled lithium niobate waveguide. Our approach encompasses the manipulation of polarization, energy-time, and quadrature amplitude-phase degrees of freedom. Theoretical calculations reveal that the magnitude of the Clauser-Horne-Shimony-Holt parameter ∣S∣|S|∣S∣ can reach 2.3752.3752.375 even considering the multi-photon-pair generation effect, which is indicative of the entanglement in the polarization degree of freedom. Further analysis involved computing the joint spectral amplitude of the two-mode state, followed by Schmidt decomposition and Fourier transformation. The resulting joint uncertainty product \ensuremathΔ(\ensuremathωs+\ensuremathωi)\ensuremathΔ(ts\ensuremath−ti)=0.4113\mathrm{\ensuremath{\Delta}}({\ensuremath{\omega}}_{s}+{\ensuremath{\omega}}_{i})\mathrm{\ensuremath{\Delta}}({t}_{s}\ensuremath{-}{t}_{i})=0.4113\ensuremathΔ(\ensuremathωs​+\ensuremathωi​)\ensuremathΔ(ts​\ensuremath−ti​)=0.4113, implying that high-quality energy-time entanglement is achieved. Notably, the von Neumann entropy Sr{S}_{r}Sr​ of our source reaches 0.192, confirming the presence of quadrature amplitude-phase entanglement within the generated state. Moreover, we theoretically apply our source in a free-space quantum key distribution system to demonstrate its potential to increase secret key rates. Our proposed scheme is an efficient and practical approach for facilitating high-capacity quantum communication systems.
Here, we demonstrate the generation and manipulation of hyperentanglement in polarization and time-energy degrees of freedom. The hyperentangled photon pairs are generated by cascaded second-harmonic generation and spontaneous parametric down-conversion processes in a high-efficiency periodically poled lithium niobate (PPLN) waveguide in a fiber Sagnac loop. The states achieve the maximum value of Clauser-Horne-Shimony-Holt Bell inequality of $S=2.76\ifmmode\pm\else\textpm\fi{}0.03$ with two-photon interference visibility of higher than 99% for polarization entanglement and the Franson-type two-photon interference visibility of 98.5% for time-energy entanglement. In addition, the polarization maximally entangled states can be fast switched to each other by using a PPLN on insulator chip through the electro-optic effect. After the entanglement manipulation, the two-photon interference visibility for polarization entanglement is still higher than 97% while keeping the quantum characteristics of time-energy degrees of freedom maintained. Our system paves a way toward reducing the complexity of quantum systems and has potential applications in many quantum-information tasks like fast superdense coding and teleportation.
Hyperentanglement, as a high-dimensional quantum entanglement phenomenon with multiple degrees of freedom, plays a critical role in quantum communication, quantum computing, and high-dimensional quantum state manipulation. Unlike entangled states in a single degree of freedom, hyperentangled states establish entanglement relationships simultaneously in multiple degrees of freedom, such as polarization, path, and orbital angular momentum. Through entanglement-based distribution techniques, high-dimensional quantum information networks can be constructed. On this basis, a fully connected quantum network with hyperentanglement is constructed in this work, and the polarization and time-bin degree-of-freedom hyperentanglement is realized through the process of second-harmonic generation and spontaneous parametric down-conversion in periodically poled lithium niobate (PPLN) waveguide cascades. The hyperentangled state is then multiplexed into a single-mode fiber by using dense wavelength division multiplexing (DWDM) technology for transmission to terminal users. The quality of the entangled states in the two degrees of freedom is characterized using Franson-type interference and photon-pair coincidence measurement techniques. Polarization entangled states are subjected to quantum state tomography, and entanglement distribution technology is employed to achieve long-distance distribution and quantum key transmission within the network. Experimental results show that the two-photon interference visibility of both polarization and time-bin entanglement is greater than 95%, demonstrating the high quality of the hyperentanglement in the network. After 100-km-entanglement distribution, the fidelity of the quantum states in both degrees of freedom remains above 88%, indicating the effectiveness of long-distance entanglement distribution in this network. Additionally, it is verified that this network supports the distribution of quantum keys over a distance of more than 50 km between users. These results confirm the feasibility of a fully connected quantum network with hyperentanglement and demonstrate the potential for constructing large-scale metropolitan networks by using hyperentanglement. As a higher-dimensional entanglement, hyperentangled states can significantly enhance the capacity and efficiency of quantum information processing. Although the quantum communication is still in its early stages of development, achieving stable storage and transmission of entangled states in large-scale metropolitan networks remains a great challenge. By utilizing the frequency conversion properties and high integration characteristics of the periodically poled lithium niobate waveguides, the three-user hyperentangled quantum network constructed in this work provides a new solution for developing the large-scale metropolitan networks with high-dimensional quantum information networks. It is expected to provide a new platform for quantum tasks such as superdense coding and quantum teleportation.
Generation of hyperentangled photon pairs is investigated based on the lithium niobate straight waveguide. We propose to use the nonlinear optical process of spontaneous parametric down-conversion (SPDC) and a well-designed lithium niobate waveguide structure to generate a hyperentangled (in the polarization dimension and the energy-time dimension) two-photon state. By performing numerical simulations of the waveguide structure and calculating the possible polarization states, joint spectral amplitudes (JSA), and joint temporal amplitudes (JTA) of the generated photon pair, we show that the generated photon pair is indeed hyperentangled in both the polarization dimension and the energy-time dimension.
In this paper, we propose the generation of hyperentangled photon pairs using type-II spontaneous parametric down-conversion in a biperiod, 5% MgO-doped lithium-niobate ridge waveguide. The photon pairs are entangled in spatial mode and polarization degrees of freedom. A pulsed laser source at 687 nm, having an antisymmetric Hermite-Gaussian HG (1,0) spatial mode, is considered as the pump. Down-converted photon pairs, with the signal being at the telecommunication wavelength of 1550 nm, are characterized through a joint spectral amplitude analysis of their biphoton state.
Reliable generation of single photons is of key importance for fundamental physical experiments and quantum protocols.The periodically poled lithium niobate (LN) waveguide has shown promise for an integrated quantum source due to its large spectral tunability and high efficiency, benefiting from the quasi-phase-matching.Here we demonstrate photon-pair sources based on an LN waveguide periodically poled by a tightly focused femtosecond laser beam.The pair coincidence rate reaches ∼8000 counts per second for average pump power of 3.2 mW (peak power is 2.9 kW).Our results prove the possibility of application of the nonlinear photonics structure fabricated by femtosecond laser to the integrated quantum source.This method can be extended to three-dimensional domain structures, which provide a potential platform for steering the spatial degree of freedom of the entangled two-photon states.